Related papers: Virtual-State Spectroscopy with Frequency-Tailored…
An entangled quantum state is considered by applying a local photon excitation to each mode of an entangled coherent state. The entanglement property is investigated in terms of the entropy of entanglement. It is shown that applying a…
In molecular aggregates, multiple delocalized exciton states interact with phonons, making the state-resolved spectroscopic monitoring of dynamics challenging. We propose a protocol that combines photon-entanglement-enhanced narrowband…
We demonstrate a new technique for characterizing two-photon quantum states based on joint temporal correlation measurements using time resolved single photon detection by femtosecond upconversion. We measure for the first time the joint…
It has been claimed that ``the use of entangled photons in an imaging system can exhibit effects that cannot be mimicked by any other two-photon source, whatever strength of the correlations between the two photons'' [A. F. Abouraddy, B. E.…
We propose a new approach to the generation of entangled states, both hybrid and consisting exclusively of continuous variable (CV) states. A single mode squeezed vacuum is mixed with a delocalized single photon on arbitrary beam splitter…
Two-photon processes are crucial in applications like microscopy and microfabrication, but their low cross-section requires intense illumination and limits, e.g., the penetration depth in nonlinear microscopy. Entangled states have been…
We discuss an expansion of the detection probabilities of biphoton states in terms of increasing orders of the joint spectral amplitude. The expansion enables efficient time- or frequency-resolved numerical simulations involving quantum…
Entangled quantum states play an important role in quantum information science and also in quantum mechanics fundamental investigations. Implementation and characterization of techniques allowing for easy preparation of entangled states are…
We closely replicated and extended a recent experiment ("Spatial properties of entangled two-photon absorption," Phys. Rev. Lett. 129, 183601, 2022) that reportedly observed enhancement of two-photon absorption rates in molecular samples by…
We consider a scheme of multiplexed cold atomic ensembles that generate a frequency-entangled biphoton state with controllable entropy of entanglement. The biphoton state consists of a telecommunication photon (signal) immediately followed…
Quantum entanglement has emerged as a great resource for interactions between molecules and radiation. We propose a new paradigm of stimulated Raman scattering with entangled photons. A quantum ultrafast Raman spectroscopy is developed for…
Integrated photonic circuits offer the possibility for complex quantum optical experiments in higher-dimensional photonic systems. However, the advantages of integration and scalability can only be fully utilized with the availability of a…
Entangled photon spectroscopy is a nascent field that has important implications for measurement and imaging across chemical, biology, and materials fields. Entangled photon spectroscopy potentially offers improved spatial and…
We theoretically study the optical tomography of maximally entangled states generated at the output modes of a beam splitter. We consider even and odd coherent states in one of the input modes and vacuum state in the other input mode of the…
Two-photon excited fluorescence (TPEF) is a standard technique in modern microscopy but still affected by photo-damage of the probe. It was proposed that TPEF can be enhanced by using entangled photons, but has proven to be challenging.…
Two-photon excitation spectroscopy is a nonlinear technique that has gained rapidly in interest and significance for studying the complex energy-level structure and transition probabilities of materials. While the conventional spectroscopy…
We experimentally demonstrate amplitude and phase modulation of a time-energy entangled two-photon wave function. The entangled photons are produced by spontaneous parametric down-conversion, spectrally dispersed in an prism compressor,…
Classical time-resolved optical spectroscopy experiments are performed using sequences of ultrashort light pulses, with photon fluxes incident on the sample which are many orders of magnitude higher than real-world conditions corresponding…
We describe and demonstrate a quantum state tomography for measuring the complex temporal waveform of narrowband biphotons. Through six sets of two-photon interference measurements projected in different polarization subspaces, we can…
Enhancing quantum entanglement is important for many quantum information processing applications. In this paper, we consider a protocol for entanglement enhancing in a two-mode squeezed vacuum state (TMSVS), attained based on photon…