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Nonlinear spectroscopic techniques using entangled photon pairs can provide an opportunity to exploit non-classical correlations encoded in two-photon wavefunctions to manipulate two-exciton wavefunctions. We propose an entangled photon…

Quantum Physics · Physics 2026-04-10 Arunangshu Debnath , Shaul Mukamel

We report on an experiment demonstrating entanglement swapping of time-frequency entangled photons. We perform a frequency-resolved Bell-state measurement on the idler photons from two independent entangled photon pairs, which projects the…

Quantum Physics · Physics 2019-10-16 Sofiane Merkouche , Valérian Thiel , Alex O. C. Davis , Brian J. Smith

Entanglement is a fundamental feature of quantum mechanics, considered a key resource in quantum information processing. Measuring entanglement is an essential step in a wide range of applied and foundational quantum experiments. When a…

Pairs of entangled vortex photons can promise new prospects of application in quantum computing and cryptography. We investigate the possibility of generating such states via two-level atom emission induced by a single photon wave packet…

Quantum Physics · Physics 2025-09-30 D. V. Grosman , G. K. Sizykh , E. O. Lazarev , G. V. Voloshin , D. V. Karlovets

Frequency non-degenerate entangled photon pairs have been employed in quantum communication, imaging, and sensing. To characterize quantum entangled state with long-wavelength (infrared, IR or even terahertz, THz) photon, one needs to…

Quantum Physics · Physics 2021-01-27 Yiquan Yang , Peiyu Zhang , Xiao-Song Ma

Path-entangled N-photon states can be obtained through the coalescence of indistinguishable photons inside linear networks. They are key resources for quantum enhanced metrology, quantum imaging, as well as quantum computation based on…

Spectroscopy is an important tool for probing the properties of materials, chemicals and biological samples. We design a practical transmitter-receiver system that exploits entanglement to achieve a provable quantum advantage over all…

Quantum Physics · Physics 2020-11-03 Haowei Shi , Zheshen Zhang , Stefano Pirandola , Quntao Zhuang

Entangled two-photon spectroscopy is expected to provide advantages compared with classical protocols. It is achieved by coherently controlling the spectral properties of energy-entangled photons. We present here an experimental setup that…

Quantum Physics · Physics 2021-08-25 Stefan Lerch , André Stefanov

Ultrafast optical spectroscopy is a powerful technique for studying the dynamic processes of molecular systems in condensed phases. However, in molecular systems containing many dye molecules, the spectra can become crowded and difficult to…

Chemical Physics · Physics 2025-02-05 Yuta Fujihashi , Akihito Ishizaki , Ryosuke Shimizu

Path-entangled multi-photon states allow optical phase-sensing beyond the shot-noise limit, provided that an efficient parity measurement can be implemented. Realising this experimentally is technologically demanding, as it requires…

Entangled two-photon absorption (ETPA) may be a viable technique to continuously drive an excited state population in plasma for high-bandwidth spectroscopy measurements of localized plasma turbulence or impurity density. Classical…

The ability to use the temporal and spatial degrees of freedom of quantum states of light to encode and transmit information is crucial for the implementation of a robust and efficient quantum network. In particular, the large…

Quantum Physics · Physics 2023-10-31 Gaurav Nirala , Siva T. Pradyumna , Ashok Kumar , Alberto M. Marino

Entangled photons can be used to make measurements with an accuracy beyond that possible with classical light. While most implementations of quantum metrology have used states made up of a single colour of photons, we show that entangled…

Twin entangled beams produced by single-pass parametric down-conversion (PDC) offer the opportunity to detect weak amount of absorption with an improved sensitivity with respect to standard techniques which make use of classical light…

Quantum Physics · Physics 2009-11-13 E. Brambilla , L. Caspani , O. Jedrkiewicz , L. A. Lugiato , A. Gatti

We present a scheme to produce an entangled four-photon state from two pairs of entangled two-photon states. Such entangled four-photon states are equivalent to the quantum state of two maximally entangled spin-1 particles. The scheme can…

Quantum Physics · Physics 2007-05-23 XuBo Zou , K. Pahlke , W. Mathis

When a low flux of time-frequency-entangled photon pairs (EPP) illuminates a two-photon transition, the rate of two-photon absorption (TPA) can be enhanced considerably by the quantum nature of photon number correlations and frequency…

While two-photon absorption (TPA) and other forms of nonlinear interactions of molecules with isolated time-frequency-entangled photon pairs (EPP) have been predicted to display a variety of fascinating effects, their potential use in…

Joint spectral measurements are a powerful tool for characterising biphoton spectral correlation, which is crucial for quantum information and communication technologies. In these applications, highly pure biphoton states are essential in…

This paper presents simulations of the state vector dynamics for a pair of atomic samples which are being probed by phase shift measurements on an optical beam passing through both samples. We show how measurements, which are sensitive to…

Quantum Physics · Physics 2016-09-08 Antonio Di Lisi , Klaus Moelmer

We use a non-perturbative theoretical approach to the parametric down-conversion (PDC) process, which generates entangled-photon field for an arbitrarily strong pump-pulse. This approach can be used to evaluate multi-point field correlation…

Chemical Physics · Physics 2025-10-22 Deependra Jadoun , Upendra Harbola , Vladimir Y. Chernyak , Shaul Mukamel