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Photosynthetic organisms use networks of chromophores to absorb sunlight and deliver the energy to reaction centres, where charge separation triggers a cascade of chemical steps to store the energy. We present a detailed model of the…

Until recently it was believed that photosynthesis, a fundamental process for life on earth, could be fully understood with semi-classical models. However, puzzling quantum phenomena have been observed in several photosynthetic…

We analytically derive transfer probabilities and efficiencies for an artificial light-harvesting photosynthetic system, which consists of a ring coupled to a central acceptor. For an incident photon pair, we find near-perfect single…

Chemical Physics · Physics 2025-04-22 Stephon Alexander , Roger Andrews , Oliver Fox , Sarben Sarkar

Removing exactly one photon from an arbitrary input pulse is an elementary operation in quantum optics and enables applications in quantum information processing and quantum simulation. Here we demonstrate a deterministic single-photon…

The phenomenon of upconversion, in which a system sequentially absorbs two or more photons and emits a photon of a higher frequency, has been used in numerous applications. These include high-resolution non-destructive bioimaging,…

The interaction between molecules and surface plasmons in defined geometries can lead to new light mater hybrid states where light propagation is strongly influenced by molecular photon absorption. Their application range from lasing LEDs…

Interfaced single-photon sources and quantum memories for photons together form a foundational component of quantum technology. Achieving compatibility between heterogeneous, state-of-the-art devices is a long-standing challenge. We built…

Quantum Physics · Physics 2022-10-04 Gianni Buser , Roberto Mottola , Björn Cotting , Janik Wolters , Philipp Treutlein

The ability to detect single photons has become increasingly essential due to the rise of photon-based quantum computing. In this theoretical work, we propose a system consisting of a quantum dot (QD) side-coupled to a superconducting…

Mesoscale and Nanoscale Physics · Physics 2023-01-05 Eric Chatterjee , Wei Pan , Daniel Soh

Single photon detectors have historically consisted of macroscopic-sized materials but recent experimental and theoretical progress suggests new approaches based on nanoscale and molecular electronics. Here we present a theoretical study of…

Mesoscale and Nanoscale Physics · Physics 2019-09-04 Catalin D. Spataru , François Léonard

We propose a new approximation for the cyclo-synchrotron emissivity of a single electron. In the second part of this work, we discuss a simple application for our approximation, and investigate the heating of electrons through the…

Astrophysics · Physics 2009-11-11 K. Katarzynski , G. Ghisellini , R. Svensson , J. Gracia

Single photon detection generally consists of several stages: the photon has to interact with one or more charged particles, its excitation energy will be converted into other forms of energy, and amplification to a macroscopic signal must…

Quantum Physics · Physics 2019-10-09 Tzula B. Propp , S. J. van Enk

We propose a method for producing on-demand single-photon states based on collision-induced exchanges of photons and unbalanced linear absorption between two single-mode light fields. These two effects result in an effective nonlinear…

Quantum Physics · Physics 2009-11-10 Tao Hong , Michael W. Jack , Makoto Yamashita

We investigate for optimal photon absorption a quantum electrodynamical model of an inhomogeneously-broadened spin ensemble coupled to a single-mode cavity. Solutions to this problem under experimental assumptions are developed in the…

Light harvesting as the first step in photosynthesis is of prime importance for life on earth. For a theoretical description of photochemical processes during light harvesting, spectral densities are key quantities. They serve as input…

Chemical Physics · Physics 2021-08-25 Sayan Maity , Pooja Sarngadharan , Vangelis Daskalakis , Ulrich Kleinekathöfer

We demonstrate a spectrally broadband and effcient technique for collecting photoluminescence from a single InAs quantum dot directly into a standard single mode optical fiber. In this approach, an optical fiber taper waveguide is placed in…

Optics · Physics 2015-05-27 M. Davanco , M. T. Rakher , W. Wegscheider , D. Schuh , A. Badolato , K. Srinivasan

We report on a single-photon-to-single-atom interface, where a single photon generated by Spontaneous Parametric Down Conversion (SPDC) is absorbed by a single trapped ion. The photon is heralded by its time-correlated partner generated in…

Quantum Physics · Physics 2016-03-23 José Brito , Stephan Kucera , Pascal Eich , Philipp Müller , Jürgen Eschner

Multi-photon absorption processes have a nonlinear dependence on the amplitude of the incident optical field i.e. the number of photons. However, multi-photon absorption is generally weak and multi-photon events occur with extremely low…

We examine computational techniques and methodologies currently in use to explore electronic excitation energy transfer in the context of light-harvesting complexes in photosynthetic antenna systems, and comment on some new insights into…

Chemical Physics · Physics 2012-07-05 Leonardo A. Pachon , Paul Brumer

We present a theoretical analysis of two-photon absorption of classical and squeezed light valid when one-photon absorption to an intermediate state is either resonant or far-detuned from resonance, and in both the low and high intensity…

Quantum Physics · Physics 2022-09-14 Christian Drago , John Sipe

In this paper we consider dynamics of a molecular system subjected to external pumping by a light source. Within a completely quantum mechanical treatment, we derive a general formula, which enables to asses effects of different light…

Biological Physics · Physics 2012-01-30 Tomas Mancal , Leonas Valkunas