Related papers: Single-photon absorption by single photosynthetic …
We develop a method to simulate the excitonic dynamics of realistic photosynthetic light harvesting systems including non-Markovian coupling to phonon degrees of freedom, under excitation by N-photon Fock state pulses. This method combines…
The technologies of heating, photovoltaics, water photocatalysis and artificial photosynthesis depend on the absorption of light and novel approaches such as coherent absorption from a standing wave promise total dissipation of energy.…
We study the dynamics of single-photon absorption by a single emitter coupled to a one-dimensional waveguide that simultaneously provides channels for spontaneous emission decay and a channel for the input photon. We have developed a…
We study the dynamics of single-photon absorption by a single emitter coupled to a one-dimensional waveguide that simultaneously provides channels for spontaneous emission decay and a channel for the input photon. We have developed a…
We theoretically investigate the dynamic interaction of a quantum dot in a nanocavity with timesymmetric single photon pulses. The simulations, based on a wavefunction approach, reveal that almost perfect single photon absorption occurs for…
The absorption of a single photon that excites a quantum system from a low to a high energy level is an elementary process of light-matter interaction, and a route towards realizing pure single-photon absorption has both fundamental and…
In this work we study the first step in photosynthesis for the limiting case of a single photon interacting with photosystem II (PSII). We model our system using quantum trajectory theory, which allows us to consider not only the average…
Decoherence is mostly detrimental in quantum information and quantum optics applications. However, the interplay between environment-induced incoherent dynamics and unitary evolution can give rise to novel quantum many-body phenomena that…
The emission and absorption of single photons by single atomic particles is a fundamental limit of matter-light interaction, manifesting its quantum mechanical nature. At the same time, as a controlled process it is a key enabling tool for…
Single atoms form a model system for understanding the limits of single photon detection. Here, we develop a non-Markov theory of single-photon absorption by a two-level atom to place limits on the absorption (transduction) time. We show…
The influence of the center of mass motion of a trapped two level system on efficient resonant single photon absorption is investigated. It is shown that this absorption process depends strongly on the ratio between the characteristic time…
The dynamics of pigment-pigment and pigment-protein interactions in light-harvesting complexes is studied with a novel approach which combines molecular dynamics (MD) simulations with quantum chemistry (QC) calculations. The MD simulations…
In natural light harvesting systems, the sequential quantum events of photon absorption by specialized biological antenna complexes, charge separation, exciton formation and energy transfer to localized reaction centers culminates in the…
We demonstrate a single-photon collection efficiency of $(44.3\pm2.1)\%$ from a quantum dot in a low-Q mode of a photonic-crystal cavity with a single-photon purity of $g^{(2)}(0)=(4\pm5)\%$ recorded above the saturation power. The high…
Biology offers a boundless source of adaptation, innovation, and inspiration. A wide range of photosynthetic organisms exist that are capable of harvesting solar light in an exceptionally efficient way, using abundant and low-cost…
Together with photon emission, the absorption of a single photon by a single atom is a fundamental process in matter-light interaction that manifests its quantum mechanical nature. As an experimentally controlled process, it is a key tool…
We consider the free carrier dispersion effect in a semiconductor nanocavity in the limit of discrete photoexcited electron-hole pairs. This analysis reveals the possibility of ultrafast, incoherent transduction and gain from a single…
The long spin coherence times in ambient conditions of color centers in solids, such as nitrogen-vacancy (NV$^{-}$) centers in diamond, make these systems attractive candidates for quantum sensing. Quantum sensing provides remarkable…
Photoinduced biological processes occur via one photon absorption in natural light, which is weak, CW and incoherent, but are often studied in the laboratory using pulsed coherent light. Here we compare the response of a molecule to these…
We show that a three-level lambda quantum emitter with equal spontaneous emission rates on both optically active transitions can absorb an incident light field with a probability approaching unity, provided that the focused light profile…