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Sr2IrO4 exhibits a novel insulating state driven by spin-orbit interactions. We report two novel phenomena, namely a large magnetoresistivity in Sr2IrO4 that is extremely sensitive to the orientation of magnetic field but exhibits no…

Strongly Correlated Electrons · Physics 2015-05-28 M. Ge , T. F. Qi , O. B. Korneta , D. E. De Long , P. Schlottmann , W. P. Crummett , G. Cao

Iridates are of considerable current interest because of the strong spin-orbit coupling that leads to a variety of new phenomena. Using density-functional studies, we predict the formation of a spin-orbital entangled two-dimensional…

Materials Science · Physics 2019-09-04 Churna Bhandari , S. Satpathy

Based on the microscopic model including strong spin-orbit coupling, on-site Coulomb and Hund's interactions, as well as crystal field effects, we have investigated magnetic and optical properties of Sr2IrO4. Taking into account all…

Strongly Correlated Electrons · Physics 2012-12-11 Beom Hyun Kim , G. Khaliullin , B. I. Min

Sr2IrO4 is a prototype of the class of Mott insulators in the strong spin-orbit interaction (SOI) limit described by a $J_{\mathrm{eff}}=1/2$ ground state. In Sr2IrO4, the strong SOI is predicted to manifest itself in the slaving of the…

Strongly Correlated Electrons · Physics 2013-09-30 S. Boseggia , H. C. Walker , J. Vale , R. Springell , Z. Feng , M. Moretti Sala , H. M. Rønnow , S. P. Collins , D. F. McMorrow

We used resonant inelastic x-ray scattering to reveal the nature of magnetic interactions in Sr2IrO4, a 5d transition-metal oxide with a spin-orbit entangled ground state and Jeff=1/2 magnetic momemts, referred to as 'isospins'. The magnon…

High temperature superconductivity in cuprates arises from an electronic state that remains poorly understood. We report the observation of a related electronic state in a non-cuprate material Sr2IrO4 in which the unique cuprate Fermiology…

Strongly Correlated Electrons · Physics 2014-06-18 Y. K. Kim , O. Krupin , J. D. Denlinger , A. Bostwick , E. Rotenberg , Q. Zhao , J. F. Mitchell , J. W. Allen , B. J. Kim

Iridium-based 5d transition-metal oxides are attractive candidates for the study of correlated electronic states due to the interplay of enhanced crystal-field, Coulomb and spin-orbit interaction energies. At ambient pressure, these…

Strongly Correlated Electrons · Physics 2014-06-05 D. A. Zocco , J. J. Hamlin , B. D. White , B. J. Kim , J. R. Jeffries , S. T. Weir , Y. K. Vohra , J. W. Allen , M. B. Maple

Superconductivity in underdoped cuprates emerges from an unusual electronic state characterised by nodal quasiparticles and an antinodal pseudogap. The relation between this state and superconductivity is intensely studied but remains…

We explore possible superconducting states in $t_{2g}$ multi-orbital correlated electron systems with strong spin-orbit coupling (SOC). In order to study such systems in a controlled manner, we employ large-scale dynamical mean-field theory…

Strongly Correlated Electrons · Physics 2014-10-24 Zi Yang Meng , Yong Baek Kim , Hae-Young Kee

We use neutron scattering to demonstrate that electron-doped superconducting Pr0.88LaCe0.12CuO4 in the underdoped regime is electronically phase separated in the ground state, showing the coexistence of a superconducting phase with a…

Superconductivity · Physics 2009-11-11 Pengcheng Dai , H. J. Kang , H. A. Mook , M. Matsuura , J. W. Lynn , Y. Kurita , Seiki Komiya , Yoichi Ando

High-temperature superconductivity in cuprates emerges upon doping the parent Mott insulator. Robust signatures of the low-doped electronic state include a Hall carrier density that initially tracks the number of doped holes and the…

Strongly Correlated Electrons · Physics 2025-05-27 Yu-Te Hsu , Andreas Rydh , Maarten Berben , Caitlin Duffy , Alberto de la Torre , Robin S Perry , Nigel E Hussey

By combining 5d transition-metal oxides showing pronounced spin-orbit interactions and oxide-based heterostructures, we propose rutile-based IrO2/TiO2 superlattices as promising candidates for unconventional electronic properties. By means…

Strongly Correlated Electrons · Physics 2017-02-16 Xing Ming , Kunihiko Yamauchi , Tamio Oguchi , Silvia Picozzi

The Jeff=1/2 state is manifested in systems with large cubic crystal field splitting and spin-orbit coupling that are comparable to the on-site Coulomb interaction, U. 5d transition metal oxides host parameters in this regime and strong…

Strongly Correlated Electrons · Physics 2014-02-18 S. Calder , G. -X Cao , S. Okamoto , J. W. Kim , V. R. Cooper , Z. Gai , B. C. Sales , M. D. Lumsden , D. Mandrus , A. D. Christianson

We sought the origin of the metal-insulator transition in Sr2-xLaxCoO4, using electron-correlation corrected density functional calculations. Our results show that Sr2CoO4 is in an intermediate-spin (IS) state and a strong Co4+ 3d-O 2p…

Strongly Correlated Electrons · Physics 2015-06-11 Hua Wu

It has recently been proposed that Na4Ir3O8 is a weak Mott insulator at ambient pressure, supporting a three-dimensional spin liquid phase with a spinon Fermi surface. This proposal is consistent with recent experimental findings that the…

Strongly Correlated Electrons · Physics 2013-05-29 Daniel Podolsky , Yong Baek Kim

We report neutron scattering measurements of spin density wave order within the superconducting state of a single crystal of predominately stage-4 La2CuO4+y with a Tc(onset) of 42 K. The low temperature elastic magnetic scattering is…

Superconductivity · Physics 2009-10-31 Y. S. Lee , R. J. Birgeneau , M. A. Kastner , Y. Endoh , S. Wakimoto , K. Yamada , R. W. Erwin , S. H. Lee , G. Shirane

We performed resonant x-ray diffraction experiments at the $L$ absorption edges for the post-perovskite-type compound CaIrO$_{3}$ with $(t_{2g})^5$ electronic configuration. By observing the magnetic signals, we could clearly see that the…

The Mott insulator Ca2RuO4 is a paradigmatic example among transition metal oxides, where the interplay of charge, spin, orbital, and lattice degrees of freedom leads to competing quantum phases. In this paper, we focus on and review some…

Strongly Correlated Electrons · Physics 2024-11-26 Giuseppe Cuono , Filomena Forte , Alfonso Romano , Canio Noce

The path from a Mott insulating phase to high temperature superconductivity encounters a rich set of unconventional phenomena involving the insulator-to-metal transition (IMT) such as emergent electronic orders and pseudogaps that…

Strongly Correlated Electrons · Physics 2019-05-17 Zhenyu Wang , Daniel Walkup , Yulia Maximenko , Wenwen Zhou , Tom Hogan , Ziqiang Wang , Stephen D. Wilson , Vidya Madhavan

Recent quasi-2D systems with judicious exploitation of the atomic monolayer or few-layer architecture exhibit unprecedented physical properties that challenge the conventional wisdom on the condensed matter physics. Here we show that the…