Iridates are of considerable current interest because of the strong spin-orbit coupling that leads to a variety of new phenomena. Using density-functional studies, we predict the formation of a spin-orbital entangled two-dimensional electron gas (2DEG) in the δ-doped iridate LaδSr2IrO4, where a single SrO layer is replaced by a LaO layer. The extra La electron resides close to the δ-doped layer, partially occupying the Jeff=1/2 upper Hubbard band and thereby making the interface metallic. The magnetic structure of the bulk is destroyed near the interface, with the Ir0 layer closest to the interface becoming non-magnetic, while the next layer (Ir1) continues to maintain the AFM structure of the bulk, but with a reduced magnetic moment. The Fermi surface consists of a hole pocket and an electron pocket, located in two different Ir layers (Ir0 and Ir1), with both carriers derived from the Jeff=1/2 upper Hubbard band. The presence of both electrons and holes at the δ-doped interface suggests unusual transport properties, leading to possible device applications.
@article{arxiv.1902.00578,
title = {Two dimensional electron gas in the $\delta$-doped iridates with strong spin-orbit coupling: La$_\delta$Sr$_2$IrO$_4$},
author = {Churna Bhandari and S. Satpathy},
journal= {arXiv preprint arXiv:1902.00578},
year = {2019}
}