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Metal-insulator transitions involve a mix of charge, spin, and structural degrees of freedom, and when strongly-correlated, can underlay the emergence of exotic quantum states. Mott insulators induced by the opening of a Coulomb gap are an…

Strongly Correlated Electrons · Physics 2021-05-14 Yejun Feng , Yishu Wang , D. M. Silevitch , S. E. Cooper , D. Mandrus , Patrick A. Lee , T. F. Rosenbaum

Spin excitations are explored in the electron-doped spin-orbit Mott insulator (Sr$_{1-x}$La$_{x}$)$_3$Ir$_2$O$_7$. As this bilayer square lattice system is doped into the metallic regime, long-range antiferromagnetism vanishes, yet a…

Strongly Correlated Electrons · Physics 2016-09-14 Tom Hogan , Rebecca Dally , Mary Upton , J. P. Clancy , Kenneth Finkelstein , Young-June Kim , M. J. Graf , Stephen D. Wilson

The electronic structure of the topmost layer in Sr2RuO4 in the close vicinity of the Fermi level is investigated by angle-resolved photoemission spectroscopy (ARPES) with a 7-eV laser. We find that the spin-orbit coupling (SOC) predicted…

Strongly Correlated Electrons · Physics 2024-06-21 Takeshi Kondo , Masayuki Ochi , Shuntaro Akebi , Yuyang Dong , Haruka Taniguchi , Yoshiteru Maeno , Shik Shin

The path from a Mott insulating phase to high temperature superconductivity encounters a rich set of unconventional phenomena involving the insulator-to-metal transition (IMT) such as emergent electronic orders and pseudogaps that…

Strongly Correlated Electrons · Physics 2019-05-17 Zhenyu Wang , Daniel Walkup , Yulia Maximenko , Wenwen Zhou , Tom Hogan , Ziqiang Wang , Stephen D. Wilson , Vidya Madhavan

The effect of isoelectronic substitution within single crystals of (Sr1-xCax)2-yIrO4+z is explored. The nominal n=1 Ruddlesden-Popper phase with y=0, z=0 remains stable from x=0 until x=0.11, where the antiferromagnet spin-orbit Mott…

Materials Science · Physics 2016-11-23 Xiang Chen , Stephen D. Wilson

We investigated electronic structure of 5d transition-metal oxide Sr2IrO4 using angle-resolved photoemission, optical conductivity, and x-ray absorption measurements and first-principles band calculations. The system was found to be well…

Strongly Correlated Electrons · Physics 2009-11-13 B. J. Kim , Hosub Jin , S. J. Moon , J. -Y. Kim , B. -G. Park , C. S. Leem , Jaeju Yu , T. W. Noh , C. Kim , S. -J. Oh , J. -H. Park , V. Durairaj , G. Cao , E. Rotenberg

We report the evolution of the $k$-space electronic structure of lightly doped bulk Ca$_{2}$RuO$_{4}$ with uniaxial strain. Using ultrathin plate-like crystals, we achieve strain levels up to $-4.1\%$, sufficient to suppress the Mott phase…

In the paper, PRB {\bf 77}, 085118 (2008), the authors conclude that the observation of Ti-doping induced half-metallicity in SrRu$_{1-x}$TI$_x$O$_3$ within the limit of local density approximations is not valid as the experimental results…

Strongly Correlated Electrons · Physics 2008-07-21 Kalobaran Maiti

Electrostatic doping into an $n$-type Mott insulator Sm$_{2}$CuO$_{4}$ has been successfully achieved with use of the heterojunction with an $n$-type band semiconductor Nb-doped SrTiO$_{3}$. The junction exhibits rectifying current-voltage…

Strongly Correlated Electrons · Physics 2007-05-23 M. Nakamura , A. Sawa , H. Sato , H. Akoh , M. Kawasaki , Y. Tokura

We have studied in detail the electronic structure of IrO$_2$ including spin-orbit coupling (SOC) and electron-electron interaction, both within the GGA+U and GGA+DMFT approximations. Our calculations reveal that the Ir t$_{2g}$ states at…

Strongly Correlated Electrons · Physics 2014-04-25 S. K. Panda , S. Bhowal , A. Delin , O. Eriksson , I. Dasgupta

In solids, strong repulsion between electrons can inhibit their movement and result in a "Mott" metal-to-insulator transition (MIT), a fundamental phenomenon whose understanding has remained a challenge for over 50 years. A key issue is how…

The motion of doped electrons or holes in an antiferromagnetic lattice with strong on-site Coulomb interactions touches one of the most fundamental open problems in contemporary condensed matter physics. The doped charge may strongly couple…

Sr$_2$RuO$_4$ is an unconventional superconductor with a tetragonal structure, whereas Ca$_2$RuO$_4$ is a Mott insulator with orthorhombic symmetry. The substituted Ca$_{2-x}$Sr$_x$RuO$_4$ has yielded a rich phase diagram that is just…

Strongly Correlated Electrons · Physics 2012-08-27 R. Jin , J. R. Thompson , J. He , J. M. Farmer , N. Lowhorn , G. A. Lamberton, , T. M. Tritt , D. Mandrus

In the context of correlated insulators, where electron-electron interactions (U) drive the localization of charge carriers, the metal-insulator transition (MIT) is described as either bandwidth (BC) or filling (FC) controlled. Motivated by…

We report a high-field electron spin resonance study in the sub-THz frequency domain of a single crystal of Sr$_2$IrO$_4$ that has been recently proposed as a prototypical spin-orbital Mott insulator. In the antiferromagnetically (AFM)…

Strongly Correlated Electrons · Physics 2015-06-18 S. Bahr , A. Alfonsov , G. Jackeli , G. Khaliullin , A. Matsumoto , T. Takayama , H. Takagi , B. Büchner , V. Kataev

The doping induced insulator-metal transition in $La_{1-x}Sr_{x}TiO_{3}$ is studied using the ab-initio LDA+DMFT method. Combining the LDA bandstructure for the actual, distorted structure found recently with multi-orbital DMFT to treat…

Strongly Correlated Electrons · Physics 2016-08-31 L. Craco , M. S. Laad , S. Leoni , E. Müller-Hartmann

We investigate the magnetic properties of the series Sr2Ir1-xRuxO4 with neutron, resonant x-ray and magnetization measurements. The results indicate an evolution and coexistence of magnetic structures via a spin flop transition from…

The Mott insulator Ca$_2$RuO$_4$ exhibits a rare insulator-to-metal transition (IMT) induced by DC current. While structural changes associated with this transition have been tracked by neutron diffraction, Raman scattering, and x-ray…

The nature of insulating phase in 5$d$ based Sr$_2$IrO$_4$ is quite debated as the theoretical as well as experimental investigations have put forward evidences in favor of both magnetically driven Slater-type and interaction driven…

Strongly Correlated Electrons · Physics 2017-02-08 Imtiaz Noor Bhatti , A. K. Pramanik

Novel phases of two dimensional electron systems resulting from new surface or interface modified electronic structures have generated significant interest in material science. We utilize photoemission spectroscopy to show that the…

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