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An intriguing idea of spin-orbit Mott insulator has been proposed to explain magnetic insulating behavior in various iridates. This scenario relies on the strength of the spin-orbit coupling being comparable to electronic correlations, and…

Strongly Correlated Electrons · Physics 2013-05-30 Jean-Michel Carter , Hae-Young Kee

Ir-based materials have drawn much attention due to the observation of insulating phase believed to be driven by spin-orbit coupling while Ir 5$d$ states are expected to be weakly correlated due to their large orbital extensions. IrO$_2$, a…

It is commonly anticipated that an insulating state collapses in favor of an emergent metallic state at high pressures as the unit cell shrinks and the electronic bandwidth broadens to fill the insulating energy band gap. Here we report a…

Strong spin-orbit coupling fosters exotic electronic states such as topological insulators and superconductors, but the combination of strong spin-orbit and strong electron-electron interactions is just beginning to be understood. Central…

We investigate the double layered Sr$_{3}$(Ru$_{1-x}$Mn$_{x}$)$_{2}$O$_{7}$ and its doping-induced quantum phase transition (QPT) from a metal to an antiferromagnetic (AFM) Mott insulator. Using spectroscopic imaging with the scanning…

Strongly Correlated Electrons · Physics 2019-07-09 Justin Leshen , Mariam Kavai , Ioannis Giannakis , Yoshio Kaneko , Yoshi Tokura , Shantanu Mukherjee , Wei-Cheng Lee , Pegor Aynajian

We present a theoretical investigation of the effects of correlations on the electronic structure of the Mott insulator Sr$_2$IrO$_4$ upon electron doping. A rapid collapse of the Mott gap upon doping is found, and the electronic structure…

Strongly Correlated Electrons · Physics 2018-04-11 Alice Moutenet , Antoine Georges , Michel Ferrero

The electron-doping-driven collapse of the charge gap and staggered magnetization of the spin-orbit-assisted Mott insulator Sr$_{3}$Ir$_{2}$O$_{7}$ is explored via first-principles computational methods. In the antiferromagnetic phase, the…

Strongly Correlated Electrons · Physics 2018-08-15 Michael W. Swift , Zach Porter , Stephen D. Wilson , Chris G. Van de Walle

We report the study of metal-STO-metal memristors where the doping concentration in STO can be fine-tuned through electric field migration of oxygen vacancies. In this tunnel junction device, the evolution of the Density Of States (DoS) can…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Alireza Mottaghizadeh , Qian Yu , Pei Lin Lang , Alexandre Zimmers , Herve Aubin

The electronic phase diagram of the weak spin-orbit Mott insulator (Sr(1-x)Lax)3Ir2O7 is determined via an exhaustive experimental study. Upon doping electrons via La substitution, an immediate collapse in resistivity occurs along with a…

Strongly Correlated Electrons · Physics 2015-07-07 Tom Hogan , Z. Yamani , D. Walkup , Xiang Chen , Rebecca Dally , Thomas Z. Ward , John Hill , Z. Islam , Vidya Madhavan , Stephen D. Wilson

We investigate the metal-insulator transition (MIT) and phase diagram of the half-filled Fermi Hubbard model with Rashba-type spin-orbit coupling (SOC) on a square optical lattice. The interplay between the atomic interactions and SOC…

Strongly Correlated Electrons · Physics 2015-03-13 Xin Zhang , Wei Wu , Gang Li , Lin Wen , Qing Sun , An-Chun Ji

We investigate how the antiferromagnetic Mott insulator evolves into the d-wave BCS superconductor through hole doping. Allowing spin fluctuations in the strong coupling approach, we find a spin-gapped incoherent metal with preformed…

Strongly Correlated Electrons · Physics 2009-11-13 Ki-Seok Kim , Mun Dae Kim

Sr$_{2}$IrO$_{4}$ with strong spin-orbit coupling (SOC) and Hubbard repulsion (U) hosts Mott insulating states. The similar crystal structure, magnetic and electronic properties, particularly the $d$-wave gap observed in Sr$_{2}$IrO$_{4}$…

Strongly Correlated Electrons · Physics 2023-12-04 Haozhe Wang , Madalynn Marshall , Zhen Wang , Kemp W. Plumb , Martha Greenblatt , Yimei Zhu , David Walker , Weiwei Xie

Multilayer (TiO$_2$)$_m$/(VO$_2$)$_n$ nanostructures ($d^1$ - $d^0$ interfaces with no polar discontinuity) show a metal-insulator transition with respect to the VO$_2$ layer thickness in first principles calculations. For $n$ $\geq$ 5…

Strongly Correlated Electrons · Physics 2015-05-14 Victor Pardo , Warren E. Pickett

Many emergent phenomena appear in doped Mott insulators near the insulator-to-metal transition. In high-temperature cuprate superconductors, superconductivity arises when antiferromagnetic (AFM) order is gradually suppressed by carrier…

In strongly correlated electron systems, the emergence of states in the Mott gap in the single-particle spectrum following the doping of the Mott insulator is a remarkable feature that cannot be explained in a conventional rigid-band…

Strongly Correlated Electrons · Physics 2015-08-20 Masanori Kohno

The phenomenon of Mott insulation involves the localization of itinerant electrons due to strong local repulsion. Upon doping, a pseudogap (PG) phase emerges - marked by selective gapping of the Fermi surface without conventional symmetry…

Strongly Correlated Electrons · Physics 2026-02-25 Abhirup Mukherjee , S. R. Hassan , Anamitra Mukherjee , N. S. Vidhyadhiraja , A. Taraphder , Siddhartha Lal

We report a systematic study of electron doping of Sr2RuO4 by non-isovalent substitution of La^(3+) for Sr^(2+). Using a combination of de Haas-van Alphen oscillations, specific heat, and resistivity measurements, we show that electron…

Strongly Correlated Electrons · Physics 2009-11-10 N. Kikugawa , A. P. Mackenzie , C. Bergemann , R. A. Borzi , S. A. Grigera , Y. Maeno

A series of polycrystalline samples of Sr2-xIrO4 have been synthesized by a solid-state reaction method. The crystal structure of this doped system can be explained on the basis of the extended nature of 5d electrons and strontium vacancies…

Strongly Correlated Electrons · Physics 2016-11-09 Jimei Kong , S. L. Liu , Jie Cheng , Haiyun Wang , Xing ao Li , Z. H. Wang

The collective magnetic excitations in the spin-orbit Mott insulator (Sr$_{1-x}$La$_x$)$_2$IrO$_4$ ($x=0,\,0.01,\,0.04,\, 0.1$) were investigated by means of resonant inelastic x-ray scattering. We report significant magnon energy gaps at…

We report a study of magnetic, thermal, and transport properties of La(3+) substituted Sr2RuO4, performed in order to investigate the effects of additional electron doping in this correlated metal. A gradual enhancement of the electronic…

Strongly Correlated Electrons · Physics 2007-05-23 N. Kikugawa , C. Bergemann , A. P. Mackenzie , Y. Maeno