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Quantum interference is shown to deliver a means of regulating the diffraction pattern of a thermal atomic beam interacting with two standing wave electric fields. Parameters have been identified to enhance the diffraction probability of…

Atomic Physics · Physics 2009-11-10 Bijoy K. Dey

Computer-driven molecular design combines the principles of chemistry, physics, and artificial intelligence to identify novel chemical compounds and materials with desired properties for a specific application. In particular,…

Chemical Physics · Physics 2023-09-04 Alessio Fallani , Leonardo Medrano Sandonas , Alexandre Tkatchenko

Fermi's Golden Rule (FGR) is one of the most impactful formulas in quantum mechanics, providing a link between easy-to-measure observables - such as transition rates - and fundamental microscopic properties - such as density of states or…

Detailed quantum chemistry calculations within the multireference configuration interaction approximation with the Davidson correction (MRCI+Q) are presented using an aug-cc-pV6Z basis set, for the potential energy curves and transition…

Atomic Physics · Physics 2016-09-08 Robert C. Forrey , James F. Babb , Phillip C. Stancil , Brendan M. McLaughlin

The study and prediction of chemical reactivity is one of the most important application areas of molecular quantum chemistry. Large-scale, fully error-tolerant quantum computers could provide exact or near-exact solutions to the underlying…

Quantum Physics · Physics 2019-09-12 Michael Kühn , Sebastian Zanker , Peter Deglmann , Michael Marthaler , Horst Weiß

The extraordinary success in laser cooling, trapping, and coherent manipulation of atoms has energized the efforts in extending this exquisite control to molecules. Not only are molecules ubiquitous in nature, but the control of their…

Atomic Physics · Physics 2022-04-27 D. Mitra , K. H. Leung , T. Zelevinsky

Simulating molecular systems on quantum processors has the potential to surpass classical methods in computational resource efficiency. The limited qubit connectivity, small processor size, and short coherence times of near-term quantum…

Quantum Physics · Physics 2025-04-08 Abhishek Sadhu , Aritra Sarkar , Akash Kundu

The inaugural edition of the MIT Quantum Index Report (QIR). Quantum technologies are evolving from theoretical concepts into tangible technologies with commercial promise. Their rapid progress is capturing global attention and suggests we…

Physics and Society · Physics 2025-06-06 Jonathan Ruane , Elif Kiesow , Johannes Galatsanos , Carl Dukatz , Edward Blomquist , Prashant Shukla

Explicitly correlated quantum chemical calculations require calculations of five types of molecular integrals beyond the standard electron repulsion integrals. We present a novel scheme, which utilises general ideas of the…

Chemical Physics · Physics 2015-04-14 Michał Silkowski , Michał Lesiuk , Robert Moszynski

QTRAJ is a computer code that simulates the propagation of quarkonium in the quark-gluon plasma (QGP) based on the quantum-trajectory algorithm. This algorithm solves a master equation in which the quarkonium is treated as an open quantum…

High Energy Physics - Phenomenology · Physics 2024-10-25 Jorge M. Mtz-Vera , Andrea Beraudo , Miguel Ángel Escobedo , Paolo Parotto , Michael Strickland

The uncertainty principle sets limit on our ability to predict the values of two incompatible observables measured on a quantum particle simultaneously. This principle can be stated in various forms. In quantum information theory, it is…

Quantum Physics · Physics 2018-09-27 H. Dolatkhah , S. Haseli , S. Salimi , S. A. Khorashad

Machine learning (ML) can be used to construct surrogate models for the fast prediction of a property of interest. ML can thus be applied to chemical projects, where the usual experimentation or calculation techniques can take hours or days…

Accurate quantum chemical calculations are critical for understanding molecular properties, yet their computational cost remains a major challenge. Full Configuration Interaction (FCI) provides exact solutions but is prohibitively expensive…

Quantum Physics · Physics 2026-03-09 Fumihiko Aiga , Hayato Goto

Quasiparticle interference (QPI) in spectroscopic imaging scanning tunneling microscopy provides a powerful method to detect orbital band structures and orbital ordering patterns in transition metal oxides. We use the $T$-matrix formalism…

Strongly Correlated Electrons · Physics 2010-05-05 Wei-Cheng Lee , D. P. Arovas , Congjun Wu

Electron transport is theoretically investigated in a molecular device made of anthracene molecule attached to the electrodes by thiol end groups in two different configurations (para and meta, respectively). Molecular system is described…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Kamil Walczak

We study numerically the influence of non-resonant effects on the dynamics of a single $\pi$-pulse quantum CONTROL-NOT (CN) gate in a macroscopic ensemble of fo ur-spin molecules at room temperature. The four nuclear spins in each molecule…

Quantum Physics · Physics 2007-05-23 G. P. Berman , A. R. Bishop , G. D. Doolen , G. V. Lopez , V. I. Tsifrinovich

In molecular communications, the direct detection of signaling molecules may be challenging due to a lack of suitable sensors and interference in the environment. Motivated by research in molecular biology, we investigate an indirect…

Information Theory · Computer Science 2022-04-25 Trang Ngoc Cao , Vahid Jamali , Wayan Wicke , Phee Lep Yeoh , Nikola Zlatanov , Jamie S Evans , Robert Schober

Unimolecular gas phase chemical reactions could be activated by both infrared (IR) radiation and inter-molecular collision in the interstellar environment. Understanding the interplay and competition between the radiation and collision…

Astrophysics of Galaxies · Physics 2024-10-29 Xiaorui Zhao , Rui Ming Zhang , Xuefei Xu , Haitao Xu

Hardware-efficient empirical variational ans\"atze for Variational Quantum Eigensolver simulations of Quantum Chemistry suffer from the lack of a direct connection to classical Quantum Chemistry methods. In the present work, we propose a…

Quantum Physics · Physics 2025-09-03 Davide Materia , Leonardo Ratini , Celestino Angeli , Leonardo Guidoni

Quantum theory implies, and empirical evidence confirms, that while particles $\textit{can}$ exhibit wave-like behavior in interferometric experiments, this behavior is so limited as $\textit{not}$ to allow for third- and higher-order…

Quantum Physics · Physics 2025-10-27 Sebastian Horvat