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Exciton-phonon coupling (ExPC) is crucial for energy relaxation in semiconductors, yet the first-principles calculation of such coupling remains challenging, especially for low-dimensional systems. Here, an accurate algorithm for…

Materials Science · Physics 2024-07-22 Xiao-Wei Zhang , Kaichen Xie , En-Ge Wang , Ting Cao , Xin-Zheng Li

Two-dimensional (2D) semiconducting materials are promising building blocks for optoelectronic applications, many of which require efficient dissociation of excitons into free electrons and holes. However, the strongly bound excitons…

Exciton condensation, the Bose-Einstein-like condensation of quasibosonic particle-hole pairs, has been the subject of much theoretical and experimental interest and holds promise for ultra-energy-efficient technologies. Recent advances in…

We report the observation of band gaps for low loss exciton-polaritons propagating outside the light cone in GaAs-based planar waveguides patterned into two-dimensional photonic crystals. By etching square lattice arrays of shallow holes…

Multiple exciton generation (MEG) is a widely studied phenomenon in semiconductor nanocrystals and quantum dots, aimed at improving the energy conversion efficiency of solar cells. MEG is the process wherein incident photon energy is…

Strongly Correlated Electrons · Physics 2023-10-24 S. R. Sahu , S. Khan , A. Tripathy , K. Dey , N. Bano , S. Raj Mohan , M. P. Joshi , S. Verma , B. T. Rao , V. G. Sathe , D. K. Shukla

Two-dimensional stacking fault defects embedded in a bulk crystal can provide a homogeneous trapping potential for carriers and excitons. Here we utilize state-of-the-art structural imaging coupled with density functional and effective-mass…

We studied theoretically the behavior of an injected electron-hole pair in crystalline polyethylene. Time-dependent adiabatic evolution by ab-initio molecular dynamics simulations show that the pair will become self-trapped in the perfect…

Materials Science · Physics 2015-06-25 D. Ceresoli , M. C. Righi , E. Tosatti , S. Scandolo , G. Santoro , S. Serra

Electric dipole radiation can be controlled by coherent optical feedback, as has previously been studied by modulating the photonic environment for point dipoles placed both in optical cavities and near metal mirrors. In experiments…

Mesoscale and Nanoscale Physics · Physics 2020-02-05 Christopher Rogers , Dodd Gray , Nathan Bogdanowicz , Takashi Taniguchi , Kenji Watanabe , Hideo Mabuchi

Wave functions and electron potentials of laterally-confined surface states are determined experimentally by means of photoemission from stepped Au(111) surfaces. Using an iterative formalism borrowed from x-ray diffraction, we retrieve the…

Materials Science · Physics 2012-11-13 A. Mugarza , J. E. Ortega , F. J. Himpsel , F. J. Garcia de Abajo

Excitons, electron-hole pairs bound by the Coulomb potential, are fundamental quasiparticles of coherent light-matter interaction energizing processes from photosynthesis to optoelectronics. Excitons are observed in semiconductors, and…

Mesoscale and Nanoscale Physics · Physics 2015-06-19 Xuefeng Cui , Cong Wang , Adam Argondizzo , Sean Garrett-Roe , Branko Gumhalter , Hrvoje Petek

Simultaneous photoluminescence and photocurrent measurements on individual single-walled carbon nanotubes reveal spontaneous dissociation of excitons into free electron-hole pairs. Correlation of luminescence intensity and photocurrent…

Mesoscale and Nanoscale Physics · Physics 2014-03-19 Y. Kumamoto , M. Yoshida , A. Ishii , A. Yokoyama , T. Shimada , Y. K. Kato

Bound electron-hole excitonic states are generally not expected to form with charges of negative effective mass. We identify such excitons in a single layer of the semiconductor WSe2, where they give rise to narrow-band upconverted…

Here we report on the reflectivity and transmissivity of a TE-polarized wave incident on a microcavity containing strongly coupled, in-plane oriented one dimensional (1D) excitons. We first discuss the propagation of the electric field…

Optics · Physics 2019-12-02 F. Le Roux , R. A. Taylor , D. D. C. Bradley

We simulate the time-dependent coherent dynamics of a spatially indirect exciton (an electron-hole pair with the two particles confined in different layers) in a GaAs coupled quantum well system. We use a unitary wave-packet propagation…

Mesoscale and Nanoscale Physics · Physics 2016-05-25 Federico Grasselli , Andrea Bertoni , Guido Goldoni

Angle-resolved photoemission spectroscopy (ARPES) is a powerful probe of electron correlations in two-dimensional layered materials. In this Letter we demonstrate that ARPES can be used to probe the onset of exciton condensation in…

Strongly Correlated Electrons · Physics 2013-02-25 Stefan Rist , A. A. Varlamov , A. H. MacDonald , Rosario Fazio , Marco Polini

We investigate the microscopic description of exciton-polaritons that involves electrons, holes and photons within a two-dimensional microcavity. We show that in order to recover the simplified exciton-photon model that is typically used to…

Quantum Gases · Physics 2021-09-06 Jesper Levinsen , Guangyao Li , Meera M. Parish

Control of the band-edge offsets at heterojunctions between organic semiconductors allows efficient operation of either photovoltaic or light-emitting diodes. We investigate systems where the exciton is marginally stable against charge…

Soft Condensed Matter · Physics 2013-09-27 Arne C. Morteani , Paiboon Sreearunothai , Laura M. Herz , Richard H. Friend , Carlos Silva

The quantum states of an electron-hole pair in one-dimensional semiconductors under a static electric field are theoretically analyzed using a two-band model with on-site Coulomb interaction. In the absence of static field, the electron and…

Mesoscale and Nanoscale Physics · Physics 2026-01-09 Adriana García , Alexander López , Jorge Quereda , Francisco Domínguez-Adame

Spontaneous emission (SE) from a two-level atom in a photonic crystal (PC) with anisotropic one-band model is investigated using the fractional calculus. Analytically solving the kinetic equation in terms of the fractional exponential…

Other Condensed Matter · Physics 2015-05-13 Jing-Nuo Wu , Chih-Hsien Huang , Szu-Cheng Cheng , Wen-Feng Hsieh

We combine electron energy-loss spectroscopy (EELS) and density functional theory (DFT) calculations to study the dispersion and effective mass of excitons in the bulk of WSe$_2$. Our EELS data suggest substantial deviations from the…

Mesoscale and Nanoscale Physics · Physics 2016-08-10 R. Schuster , Y. Wan , M. Knupfer , B. Büchner