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The current (voltage) responsivity of the superlattice-based diode detectors in the terahertz frequency band which includes the region of the polar optical phonon frequencies has been analyzed theoretically. Within the framework of the…

Mesoscale and Nanoscale Physics · Physics 2014-05-30 Anatoly A. Ignatov

We demonstrate the self-phase modulation (SPM) of a single-cycle THz pulse in a semiconductor, using bulk n-GaAs as a model system. The SPM arises from the heating of free electrons in the electric field of the THz pulse, leading to an…

Materials Science · Physics 2012-08-13 Dmitry Turchinovich , Jørn M. Hvam , Matthias C. Hoffmann

Third-harmonic generation (THG) experiments on superconductors can be used to investigate collective excitations like the amplitude mode of the order parameter known as Higgs mode. These modes are visible due to resonances in the THG signal…

Superconductivity · Physics 2021-11-16 Lukas Schwarz , Rafael Haenel , Dirk Manske

A manifestation of electron-hole pairing in nonlinear electromagnetic response of a double layer graphene system is studied. It is shown that the pairing causes the appearance of a number of peaks in the frequency dependence of the…

Strongly Correlated Electrons · Physics 2017-10-20 K. V. Germash , D. V. Fil

A laser pulse composed of a fundamental and an appropriately phased second harmonic can drive a time-dependent current of photoionized electrons that generates broadband THz radiation. Over the propagation distances relevant to many…

High harmonic generation (HHG) in solid and gaseous targets has been proven to be a powerful avenue for the generation of attosecond pulses, whereas the influence of electron-phonon scattering on HHG is a critical outstanding problem. Here…

Optics · Physics 2022-06-02 Tao-Yuan Du , Chao Ma

We study the influence of the polarization states of femtosecond two-color pulses ionizing gases on the emitted terahertz radiation. A local-current model and plane-wave evaluations justify the previously-reported impact on the THz energy…

High-order harmonic generation in the presence of a chirped THz pulse is investigated numerically with a complete 3D non-adiabatic model. The assisting THz pulse illuminates the HHG gas cell laterally inducing quasi-phase-matching. We…

Strong light-matter coupling within electromagnetic environments provides a promising path to modify and control chemical and physical processes. The origin of the enhancement of nonlinear optical processes such as second-harmonic and…

Optics · Physics 2022-03-03 Davis M. Welakuh , Prineha Narang

The nonlinear process of second harmonic generation (SHG) in monolayer (1L) transition metal dichalcogenides (TMD), like $WS_2$, strongly depends on the polarization state of the excitation light. Combining plasmonic nanostructures with…

Optics · Physics 2021-10-08 Florian Spreyer , Claudia Ruppert , Philip Georgi , Thomas Zentgraf

The strong ellipticity dependence of high-harmonic generation in gases enables numerous experimental techniques that are nowadays routinely used, for instance, to create isolated attosecond pulses. Extending such techniques to high-harmonic…

We have investigated the terahertz (THz) nonlinear response of the multigap superconductor MgB$_2$, using THz two-dimensional coherent spectroscopy (THz 2DCS). With broadband THz drive fields, we identified a nonlinear response at twice the…

Superconductivity · Physics 2025-07-18 Kota Katsumi , Jiahao Liang , Ralph Romero , Ke Chen , Xiaoxing Xi , N. P. Armitage

Higgs spectroscopy is a new field in which Higgs modes in nonequilibrium superconductors are analyzed to gain information about the ground state. One experimental setup in which the Higgs mode in s-wave superconductors was observed is…

Superconductivity · Physics 2020-05-26 Lukas Schwarz , Dirk Manske

We experimentally investigate second harmonic generation from strongly coupled localized and propagative phonon polariton modes in arrays of silicon carbide nanopillars. Our results clearly demonstrate the hybrid nature of the system's…

In this study, we investigate second- and third-harmonic generation processes in Au nanorod systems using the real-time time-dependent density functional tight binding method. Our study focuses on the computation of nonlinear signals based…

Optics · Physics 2024-09-18 Sajal Kumar Giri , George C. Schatz

High input intensities are usually required to efficiently excite optical nonlinear effects in ultrathin structures. This problem is particularly critical at terahertz (THz) frequencies because high input power THz sources are not…

Optics · Physics 2019-02-27 Tianjing Guo , Boyuan Jin , Christos Argyropoulos

We investigate the high-order harmonic generation (HHG) in doped semiconductors. The HHG is simulated with the single-electron time-dependent Schr\"{o}dinger equation (TDSE). The results show that the high-order harmonics in the second…

Optics · Physics 2017-11-22 Tengfei Huang , Xiaosong Zhu , Liang Li , Xi Liu , Pengfei Lan , Peixiang Lu

State-of-the-art experiments employ strong ultrafast optical fields to study the nonlinear response of electrons in solids on an attosecond time-scale. Notably, a recent experiment retrieved a 3rd order nonlinear susceptibility by comparing…

We theoretically investigate the effects of the excitation frequency on the plateau of high-order terahertz sideband generation (HSG) in semiconductors driven by intense terahertz (THz) fields. We find that the plateau of the sideband…

Mesoscale and Nanoscale Physics · Physics 2014-01-17 Xiao-Tao Xie , Bang-Fen Zhu , Ren-Bao Liu

We present a detailed theoretical investigation of the linear and non-linear optical response in a model system for a disordered d-wave superconductor, showing that for both quantities the gap symmetry considerably changes the paradigm of…

Superconductivity · Physics 2023-07-17 L. Benfatto , C. Castellani , G. Seibold