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We study third-harmonic generation (THG) in an excitonic insulator (EI) described in a two-band correlated electron model. Employing the perturbative expansion with respect to the external electric field, we derive the THG susceptibility…

Strongly Correlated Electrons · Physics 2021-12-28 Tetsuhiro Tanabe , Tatsuya Kaneko , Yukinori Ohta

Giant second-harmonic generation (SHG) in the terahertz (THz) frequency range is observed in a thin film of an s-wave superconductor NbN, where the time-reversal ($\mathcal{T}$-) and space-inversion ($\mathcal{P}$-) symmetries are…

Superconductivity · Physics 2020-08-31 Sachiko Nakamura , Kota Katsumi , Hirotaka Terai , Ryo Shimano

Third-harmonic generation (THG) is a key nonlinear optical process for ultrafast imaging, terahertz (THz) signal generation, and symmetry-sensitive probes, often dominating in centrosymmetric materials where lower-order responses vanish.…

Optics · Physics 2026-01-09 Sanjay Sarkar , Debottam Mandal , Amit Agarwal

Dynamical control of the nonlinear optical properties of solids -- with light itself -- will be essential for future ultrafast photonic technologies. Previously, methods to modulate nonlinear processes including second-harmonic generation…

We study the nonlinear optical response in a superconducting NbN thin film with strong terahertz (THz)wave. Besides the expected third harmonic generation, we observe a new transient oscillation which softensin frequency with temperature…

Superconductivity · Physics 2022-03-30 Z. X. Wang , J. R. Xue , H. K. Shi , X. Q. Jia , T. Lin , L. Y. Shi , T. Dong , F. Wang , N. L. Wang

We investigate the third-harmonic generation (THG) of s-wave superconductors under microwave pulse irradiation. We consider the effect of paramagnetic impurities on the THG intensity of dirty superconductors. The nonlinear response function…

Superconductivity · Physics 2018-01-08 Takanobu Jujo

We compute and analyze the dependence of excitonic second- and third-harmonic generation (SHG/THG) as a function of the optical excitation intensity in the presence of static electric fields by solving the semiconductor Bloch equations. Our…

Mesoscale and Nanoscale Physics · Physics 2025-11-10 Ruixin Zuo , Matthias Reichelt , Cong Ngo , Xiaohong Song , Weifeng Yang , Torsten Meier

Improving the conversion efficiency is critical for advancing nonlinear photonic devices, enabling applications in ultrafast optics, quantum light sources, and high-resolution imaging. Herein, we present a bilayer waveguide integrated with…

Optics · Physics 2025-08-21 Xin Huang , Qi Lin , Sheng-Xuan Xia , Xiang Zhai , Gui-Dong Liu

Multiband superconductors can host collective excitations with marked differences with respect to their single-band counterpart. We first study the spectrum of collective amplitude fluctuations in a clean two-bands superconductor, showing…

Superconductivity · Physics 2022-09-26 Jacopo Fiore , Mattia Udina , Marco Marciani , Goetz Seibold , Lara Benfatto

Metasurfaces have emerged as a promising platform for integrated nonlinear optics. Nonlocal metasurfaces enable high nonlinear conversion efficiency, while the local ones can offer versatile wavefront control, yet achieving both within a…

Optics · Physics 2026-02-03 Yu Tian , Nuo Wang , Qi Liu , Shuyuan Xiao , Tingting Liu , Olivier J. F. Martin , Ying Gu

Recent advancements in nonlinear nanophotonics are driven by the exploration of sharp resonances within high-index dielectric metasurfaces. In this work, we leverage doubly degenerate quasi-bound states in the continuum (quasi-BICs) to…

The study of interaction between different degrees of freedom in solids is of fundamental importance to understand the functionalities of materials. One striking example of such interaction is the intertwined coupling or competition between…

The interplay between superconductivity and charge density wave has often been studied from an equilibrium point of view. For example, using static tuning knobs such as doping, magnetic field and pressure, superconductivity can be enhanced…

We study high-order harmonic generation (HHG) resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneities of the local electric field and the confinement of the electron motion…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , Srdjan S. Acimovic , T. Shaaran , J. Biegert , R. Quidant , M. Lewenstein

Successful phase-matching methods for Third Harmonics Generation (THG) include phase-matching in birefringent crystal and quasi-phase-matching (QPM) in crystal with periodically poled domains. However, these methods are not feasible in some…

Optics · Physics 2013-07-25 Tan Yizhou , Yang Yisheng , Liao Jiali , Zhang Ming

We show both theoretically and experimentally that the magnetization density accompanying ultrafast excitation of a semiconductor with circular polarized light varies rapidly enough to produce a detectable THz field.

Materials Science · Physics 2007-05-23 F. Nastos , R. W. Newson , J. Hübner , J. E. Sipe , H. M. van Driel

Detection of the Higgs mode in superconductors using nonlinear terahertz spectroscopy is a key area of interest in condensed matter physics. We investigate the influence of disorder on the nonlinear terahertz response and the Higgs mode in…

Recent experiments with strong THz fields in unconventional cuprates superconductors have clearly evidenced an increase of the non-linear optical response below the superconducting critical temperature Tc. As in the case of conventional…

Superconductivity · Physics 2023-06-21 Mattia Udina , Jacopo Fiore , Tommaso Cea , Claudio Castellani , Goetz Seibold , Lara Benfatto

Nonlinear metasurfaces offer new paradigm for boosting optical effect beyond limitations of conventional materials. In this work, we present an alternative way to produce pronounced third-harmonic generation (THG) based on nonlinear field…

We present experimental and theoretical results for the angular dependence of third harmonic generation (THG) of water droplets in the micrometer range (size parameter $62<ka<248$). The THG signal in $p$- and $s$-polarization obtained with…