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Catalytically active Janus particles suspended in solution create gradients in the chemical composition of the solution along their surfaces, as well as along any nearby container walls. The former leads to self-phoresis, while the latter…

Soft Condensed Matter · Physics 2016-09-22 W. E. Uspal , M. N. Popescu , S. Dietrich , M. Tasinkevych

Chemically active colloids move by creating gradients in the composition of the surrounding solution and by exploiting the differences in their interactions with the various molecular species in solution. If such particles move near…

Soft Condensed Matter · Physics 2017-02-24 M. N. Popescu , W. E. Uspal , S. Dietrich

Micron-sized particles moving through solution in response to self-generated chemical gradients serve as model systems for studying active matter. Their far-reaching potential applications will require the particles to sense and respond to…

Soft Condensed Matter · Physics 2016-03-09 W. E. Uspal , M. N. Popescu , S. Dietrich , M. Tasinkevych

Janus particles self-propel by generating local tangential concentration gradients along their surface. These gradients are present in a thin layer whose thickness is small compared to the particle size. Chemical asymmetry along the surface…

Soft Condensed Matter · Physics 2021-03-31 Prathmesh M. Vinze , Akash Choudhary , S. Pushpavanam

Surface bound catalytic chemical reactions self-propel chemically active Janus particles. In the vicinity of boundaries, these particles exhibit rich behavior, such as the occurrence of wall-bound steady states of "sliding". Most active…

Many biological microswimmers are capable of chemotaxis, i.e., they can sense an ambient chemical gradient and adjust their mechanism of motility to move towards or away from the source of the gradient. Synthetic active colloids endowed…

Soft Condensed Matter · Physics 2024-06-18 Viviana Mancuso , Mihail N. Popescu , William E. Uspal

Chemically active Janus particles generate tangential concentration gradients along their surface for self-propulsion. Although this is well studied in unbounded domains, the analysis in biologically relevant environments such as…

Soft Condensed Matter · Physics 2021-11-29 Akash Choudhary , K. V. S. Chaithanya , Sébastien Michelin , S. Pushpavanam

The dynamics of self-propelled colloidal particles are strongly influenced by their environment through hydrodynamic and, in many cases, chemical interactions. We develop a theoretical framework to describe the motion of confined active…

Fluid Dynamics · Physics 2025-08-29 Günther Turk , Rajesh Singh , Howard A. Stone

We study the self-diffusiophoresis of a spherical chemically active particle near a planar, impermeable wall, with a focus on the influence of particle orientation on propulsion. We analyze a Janus particle with asymmetric surface chemical…

Soft Condensed Matter · Physics 2026-03-03 Tachin Ruangkriengsin , Günther Turk , Howard A. Stone

A longstanding goal in colloidal active matter is to understand how gradients in fuel concentration influence the motion of phoretic Janus particles. Here, we present a theoretical description of the motion of a spherical phoretic Janus…

Soft Condensed Matter · Physics 2025-05-28 Parvin Bayati , Stewart A. Mallory

We study the effect of a nearby planar wall on the propulsion of a phoretic Janus micro-swimmer driven by asymmetric reactions on its surface which absorb reactants and generate products. We show that the behaviour of these swimmers near a…

Soft Condensed Matter · Physics 2017-06-01 Yahaya Ibrahim , Tanniemola B. Liverpool

We study the diffusiophoretic self-propulsion of a colloidal catalytic particle due to a surface chemical reaction in a vicinity of a solid wall. Diffusiophoresis is a chemico-mechanical transduction mechanism in which a concentration…

Soft Condensed Matter · Physics 2016-06-22 Ali Mozaffari , Nima Sharifi-Mood , Joel Koplik , Charles Maldarelli

Suspended colloidal particles interacting chemically with a solute are able to self-propel by autophoretic motion when they are asymmetrically patterned (Janus colloids). Here we demonstrate that the chemical anisotropy is not a necessary…

Soft Condensed Matter · Physics 2013-06-28 Sebastien Michelin , Eric Lauga , Denis Bartolo

We study the dynamics of active Janus particles that self-propel in solution by light-activated catalytic decomposition of chemical "fuel." We develop an analytical model of a photo-active self-phoretic particle that accounts for…

Soft Condensed Matter · Physics 2019-05-23 W. E. Uspal

Gold-capped Janus particles immersed in a near-critical binary mixture can be propelled using illumination. We employ a non-isothermal diffuse interface approach to investigate the self-propulsion mechanism of a single colloid. We attribute…

Soft Condensed Matter · Physics 2015-11-04 Sela Samin , René van Roij

We theoretically study the active motion of self-diffusiophoretic Janus particles (JPs) using the Onsager-Casimir reciprocal relations. The linear and angular velocity of a single JP are shown to respectively result from a coupling of…

Soft Condensed Matter · Physics 2019-10-30 Jérôme Burelbach , Holger Stark

We experimentally investigate active motion of spherical Janus colloidal particles in a viscoelastic fluid. Self-propulsion is achieved by a local concentration gradient of a critical polymer mixture which is imposed by laser illumination.…

Soft Condensed Matter · Physics 2016-03-31 Juan Ruben Gomez-Solano , Alex Blokhuis , Clemens Bechinger

Self-propulsion of particles is typically explained by phoretic mechanisms driven by externally imposed chemical, electric, or thermal gradients. In contrast, chemical reactions can enhance particle diffusion even in the absence of such…

Soft Condensed Matter · Physics 2025-10-08 A. Arango-Restrepo , J. M. Rubi

We propose a highly efficient mechanism to rectify the motion of active particles by exploiting particle-wall alignment interactions. Through numerical simulations of active particles' dynamics in a narrow channel, we demonstrate that a…

Soft Condensed Matter · Physics 2025-11-07 Poulami Bag , Tanwi Debnath , Shubhadip Nayak , Pulak K. Ghosh

Janus phoretic colloids (JPs) self-propel as a result of self-generated chemical gradients and exhibit spontaneous nontrivial dynamics within phoretic suspensions, on length scales much larger than the microscopic swimmer size. Such…

Fluid Dynamics · Physics 2021-11-29 Tullio Traverso , Sebastien Michelin
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