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We performed magnetic field and frequency tunable electron paramagnetic resonance spectroscopy of an Er$^{3+}$ doped Y$_2$SiO$_5$ crystal by observing the change in flux induced on a direct current-superconducting quantum interference…

Precise measurement of the electric dipole moments (EDM) of fundamental charged particles would provide a significant probe of physics beyond the standard model. Any measurably large EDM would imply violation of both time reversal and…

Accelerator Physics · Physics 2015-12-07 Richard Talman

We propose a method based on optically detected magnetic resonance (ODMR) to measure the decoherence time $T_{2}$ of a single electron spin in a semiconductor quantum dot. The electron spin resonance (ESR) of a single excess electron on a…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 Oliver Gywat , Hans-Andreas Engel , Daniel Loss , R. J. Epstein , F. M. Mendoza , D. D. Awschalom

Detection of a single nuclear spin constitutes an outstanding problem in different fields of physics such as quantum computing or magnetic imaging. Here we show that the energy levels of a single nuclear spin can be measured by means of…

Mesoscale and Nanoscale Physics · Physics 2011-12-16 F. Delgado , J. Fernández-Rossier

We demonstrate optically detected spin resonance of a single electron confined to a self-assembled quantum dot. The dot is rendered dark by resonant optical pumping of the spin with a coherent laser. Contrast is restored by applying a radio…

We consider fluctuations of the electronic spin due to coupling to nuclear spin. Noise spectroscopy of an electronic spin can be revealed in the Scanning Tunnelling Microscope (STM). We argue that the noise spectroscopy of electronic spin…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 A. V. Balatsky , J. Fransson , D. Mozyrsky , Yishay Manassen

Detection of electron paramagnetic resonance (EPR) using a microwave cavity resonating at a fixed frequency (between 9 and 10 GHz) remains the most popular method until now. Here, we report a cavity-less technique which makes use of only an…

Applied Physics · Physics 2020-02-06 Ushnish Chaudhuri , R. Mahendiran

Magnetic Resonance Force Microscopy (MRFM) describes a range of approaches to detect nuclear spins with mechanical sensors. MRFM has the potential to enable magnetic resonance imaging (MRI) with near-atomic spatial resolution, opening up…

Historically, electron spin resonance (ESR) has provided excellent insight into the electronic, magnetic, and chemical structure of samples hosting spin centers. In particular, the hyperfine interaction between the electron and the nuclear…

Mesoscale and Nanoscale Physics · Physics 2022-11-23 Laëtitia Farinacci , Lukas M. Veldman , Philip Willke , Sander Otte

Sensing, localising and identifying individual nuclear spins or frequency components of a signal in the presence of a noisy environments requires the development of robust and selective methods of dynamical decoupling. An important…

Random motion of spins is usually detrimental in magnetic resonance experiments. The spin diffusion in non-uniform magnetic fields causes broadening of the resonance and limits the sensitivity and the spectral resolution in applications…

Quantum Physics · Physics 2023-01-18 Xiangdong Zhang , Jinbo Hu , Nan Zhao

In dynamic nuclear polarization (DNP) experiments, the compound is driven out-of-equilibrium by microwave (MW) irradiation of the radical electron spins. Their stationary state has been recently probed via electron double resonance (ELDOR)…

Strongly Correlated Electrons · Physics 2017-02-28 Filippo Caracciolo , Marta Filibian , Pietro Carretta , Alberto Rosso , Andrea De Luca

Nonlinear spectroscopy is widely used for studying physical systems. Conventional nonlinear optical spectroscopy and magnetic resonance spectroscopy, which use classical probes such as electromagnetic waves, can only access certain types of…

We demonstrate an all-optical Raman spin echo technique, using Electromagnetically Induced Transparency (EIT) to create the different pulses of the spin echo sequence: initialization, pi-rotation, and readout. The first pulse of the…

Quantum Physics · Physics 2016-09-21 Andreas Walther , Adam N. Nilsson , Qian Li , Lars Rippe , Stefan Kröll

We describe a simple experimental method to detect electron paramagnetic resonance (EPR) in polycrystalline 2,2-diphenyl-1-picrylhydrazyl (DPPH) sample, the standard g-marker for EPR spectroscopy, without using a cavity resonator or a…

Materials Science · Physics 2021-04-23 Lee Yong Heng , Ushnish Chaudhuri , Ramanathan Mahendiran

Quantum emitters respond to resonant illumination by radiating electromagnetic fields. A component of these fields is phase-coherent with the driving tone, while another one is incoherent, consisting of spontaneously emitted photons and…

Raman heterodyne spectroscopy is a powerful tool for characterizing the energy and dynamics of spins. The technique uses an optical pump to transfer coherence from a spin transition to an optical transition where the coherent emission is…

Sensors play a crucial role in advanced apparatuses and it is persistently pursued to improve their sensitivities. Recently, the singularity of a non-Hermitian system, known as the exceptional point (EP), has drawn much attention for this…

Quantum Physics · Physics 2024-01-04 Yao-Dong Hu , Yi-Pu Wang , Rui-Chang Shen , Zi-Qi Wang , Wei-Jiang Wu , J. Q. You

We experimentally isolate, characterize and coherently control up to six individual nuclear spins that are weakly coupled to an electron spin in diamond. Our method employs multi-pulse sequences on the electron spin that resonantly amplify…

Mesoscale and Nanoscale Physics · Physics 2012-10-23 T. H. Taminiau , J. J. T. Wagenaar , T. van der Sar , F. Jelezko , V. V. Dobrovitski , R. Hanson

We compute the electron spin resonance (ESR) intensity for one-dimensional quantum wires in semiconductor heterostructures, taking into account electron-electron interactions and spin-orbit coupling. The ESR spectrum is shown to be very…

Strongly Correlated Electrons · Physics 2012-09-27 A. De Martino , R. Egger