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Linear sp carbon nanostructures are gathering interest for the physical properties of one-dimensional (1D) systems. At present, the main obstacle to the synthesis and study of these systems is their instability. Here we present a simple…

Surface chemistry is important across diverse fields such as corrosion and nanostructure synthesis. Unfortunately, many as-synthesized nanomaterials, including partially dealloyed nanoparticle catalysts for fuel cells, with highly active…

Structural stability and electronic properties of alkaline-earth metals (Ca, Sr, Ba) induced Si(111)-3x2 surfaces have been comprehensively studied by means of ab initio calculations. Adsorption energy and charge density difference…

Materials Science · Physics 2018-11-20 Jun-Shuai Chai , Zhen-Zhen Li , Lifang Xu , Jian-Tao Wang

The adsorption of oxygen on the Ag(001) is investigated by means of density functional techniques. Starting from a characterization of the clean silver surfaces oxygen adsorption in several modifications (molecularly, on-surface,…

Materials Science · Physics 2009-11-10 M. Gajdos , A. Eichler , J. Hafner

We study the optical and electrical properties of silver films with a graded thickness obtained through metallic evaporation in vacuum on a tilted substrate to evaluate their use as semitransparent electrical contacts. We measure their…

Understanding elemental corrosion currents and visualizing corroding topographies provide a detailed insight into corrosion mechanisms at the nano-scale. Here, we develop a strategy to understand the elemental composition, corrosion…

Applied Physics · Physics 2021-04-16 Dominik Dworschak , Marina Bishara , Hsiu-Wei Cheng , Markus Valtiner

The data experimental synthesis and studies of layered organic-inorganic nanocomposites [Cu2(OH)3 + DS], resulting from ablation of copper in aqueous solutions of surfactant - dodecyl sodium sulfate (SDS) are presented. By the methods of…

Mesoscale and Nanoscale Physics · Physics 2012-03-15 Vyacheslav T. Karpukhin , Mikhail M. Malikov , Tatyana I. Borodina , Evgeniy G. Valyano , Olesya A. Gololobova

Systematic studies of the gradual fabrication by means of carbon ion-implantation of high-quality 6H-SiC layers on silicon surfaces have been carried out. The fluence of carbon ions varied from 5*10^15 cm-2 to 10^17 cm-2. Results of…

The electronic structure of carbon shells of carbon encapsulated iron nanoparticles carbon encapsulated Fe@C has been studied by X-ray resonant emission and X-ray absorption spectroscopy. The recorded spectra have been compared to the…

Materials Science · Physics 2013-03-20 V. R. Galakhov , S. N. Shamin , E. M. Mironova , M. A. Uimin , A. Ye. Yermakov , D. W. Boukhvalov

We present a first-principles study of the electronic properties of silicon clathrate nanowires intercalated with various types of alkali or alkaline-earth atoms. We find that the band structure of the nanowires can be tuned by varying the…

Materials Science · Physics 2009-11-11 S. Sirichantaropass , V. M. García-Suárez , C. J. Lambert

The electronic excitation occurring on adsorbates at ultrafast time scales from optical lasers that initiate surface chemical reactions is still an open question. Here, we report the ultrafast temporal evolution of X-ray absorption…

The structure of AgCl formed in the course of chlorine adsorption on Ag(111) surface was studied by STM. For the first time atomic resolution STM images of silver chloride were obtained. The silver chloride was detected as small (30-60 A in…

Materials Science · Physics 2009-10-31 B. V. Andryushechkin , K. N. Eltsov , V. M. Shevlyuga

The forces of electrical imaging strongly polarize the surface of colloidal silica. I used X-ray scattering to study the adsorbed 2-nm-thick compact layer of alkali ions at the surface of concentrated solutions of 5-nm, 7-nm, and 22-nm…

Soft Condensed Matter · Physics 2007-05-23 Aleksey M. Tikhonov

We consider the factors that affect the photoactivity of silicon electrodes for the water-splitting reaction using a self-consistent continuum solvation (SCCS) model of the solid-liquid interface. This model allows us to calculate the…

Mesoscale and Nanoscale Physics · Physics 2019-09-10 Quinn Campbell , Ismaila Dabo

X-ray photoemission and x-ray absorption spectroscopy are important techniques to characterize chemical bonding at surfaces and are often used to identify the strength and nature of adsorbate-substrate interactions. In this study, we judge…

Materials Science · Physics 2023-02-09 Samuel J. Hall , Benedikt P. Klein , Reinhard J. Maurer

The self-assembled monolayers of alkane thiolates on Ag (111) surfaces and nanoparticles are studied using molecular dynamics. Reactive force fields allow simulations of very large systems such as nanoparticles of 10 nm. Stable (sqrt(7) X…

Chemical Physics · Physics 2024-01-11 Adam Lahouari , Jean-Philip Piquemal , Johannes Richardi

We report hard x-ray photoemission spectroscopy measurements of the electronic structure of the prototypical correlated oxide SrxCa1-xVO3. By comparing spectra recorded at different excitation energies, we show that 2.2 keV photoelectrons…

Strongly Correlated Electrons · Physics 2015-04-22 J. Laverock , J. Kuyyalil , B. Chen , R. P. Singh , G. Balakrishnan , B. Karlin , J. C Woicik , K. E. Smith

With the advancement of nanoscience, silver/silver chloride (Ag/AgCl) electrodes have become widely utilised in microscale and nanoscale fluidic experiments, because of their stability. However, our findings reveal that the dissolution of…

Electronic structure and cohesive properties of metastable hexagonal AgB_{2} and silver-deficient borides Ag_{0.875}B_{2} and Ag_{0.750}B_{2} were investigated by means of the projected augmented wave method in the framework of the density…

Materials Science · Physics 2007-05-23 I. R. Shein , N. I. Medvedeva , A. L. Ivanovskii

The structural evolution and dynamics of silver nanodrops Ag${}_{2896}$ (4.4 nm in diameter) during rapid cooling conditions has been studied by means of molecular dynamics simulations and electronic density of state calculations. The…

Materials Science · Physics 2009-01-22 I. Lobato , J. Rojas , C. V. Landauro , J. Torres
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