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We introduce a general Monte Carlo scheme for achieving atomistic simulations with monoelectronic Hamiltonians including the thermalization of both nuclear and electronic degrees of freedom. The kinetic Monte Carlo algorithm is used to…

Materials Science · Physics 2009-11-07 F. Calvo , F. Spiegelman

The configurational and melting properties of large two-dimensional clusters of charged classical particles interacting with each other via the Coulomb potential are investigated through the Monte Carlo simulation technique. The particles…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 Minghui Kong , B. Partoens , F. M. Peeters

We have studied molecular hydrogen in a pure 1D geometry and inside a narrow carbon nanotube by means of the diffusion Monte Carlo method. The one-dimensionality of H2 in the nanotube is well maintained in a large density range, this system…

Condensed Matter · Physics 2009-10-31 M. C. Gordillo , J. Boronat , J. Casulleras

In this study, the interaction between the gas molecules, including H2O, N2, CO, NO, NO2 and N2O, with the WSe2 monolayer containing a Se vacancy (denoted as VSe) is theoretically studied. It is found that H2O and N2 molecules are highly…

Materials Science · Physics 2017-06-15 Ma Dongwei , He Chaozheng , Ma Benyuan , Lu Zhiwen , Tang Yanan , Lu Zhansheng , Yang Zongxian

We employ the Delta-variance analysis and study the turbulent gas dynamics of simulated molecular clouds (MCs). Our models account for a simplified treatment of time-dependent chemistry and the non-isothermal nature of the gas. We…

Solar and Stellar Astrophysics · Physics 2015-08-06 Erik Bertram , Ralf S. Klessen , Simon C. O. Glover

Geometric configuration and energy of a hydrogen molecule centered between two point-shaped tips of equal charge are calculated with the variational quantum Monte-Carlo (QMC) method without the restriction of the Born-Oppenheimer (BO)…

Mesoscale and Nanoscale Physics · Physics 2020-05-29 W. Schattke , T. Frederiksen , M. A. Van Hove , R. Díez Muiño

We present a multiple time step algorithm for hybrid path integral Monte Carlo simulations involving rigid linear rotors. We show how to calculate the quantum torques needed in the simulation from the rotational density matrix, for which we…

Statistical Mechanics · Physics 2007-05-23 G. Garberoglio , J. K. Johnson

Generally displacement fields in the vicinity of voids were determined by the equations of theory of elasticity. Such a description has its disadvantages as it does not take into account the discrete atomic structure of materials and it…

Materials Science · Physics 2017-04-18 A. V. Nazarov , I. V. Ershova , Y. S. Volodin

We describe a Monte Carlo scheme which, in a single simulation, yields a measurement of the chemical potential of a crystalline solid. Within the isobaric ensemble, this immediately provides an estimate of the system free energy, with…

Statistical Mechanics · Physics 2015-06-11 Nigel B. Wilding , Peter Sollich

Quantum Monte Carlo methods find fruitful application in large shell model problems. These methods reduce the imaginary-time many-body evolution operator to a coherent superposition of one-body evolutions in a fluctuating one-body field;…

Nuclear Theory · Physics 2008-02-03 S. E. Koonin

We propose a simple microscopic model of molecular dynamics simulation to study orientational glass in three dimensions. We present simulation results for mixtures of mildly anisotropic particles and spherical impurities. We realize fcc…

Soft Condensed Matter · Physics 2012-10-29 Kyohei Takae , Akira Onuki

We present Shell Model Monte Carlo calculations for nuclei within the full major shell 50-82 for both protons and neutrons. The interaction is determined solely by self-consistency and odd-even mass differences. The methods are illustrated…

Nuclear Theory · Physics 2009-01-23 Y. Alhassid , G. F. Bertsch , D. J. Dean , S. E. Koonin

I did off-lattice 3D Monte Carlo simulations for polymer translocation through a narrow pore at low external field, trying to be as close to a direct approach as possible. The process was found non equilibrium globally, but dynamics of the…

Soft Condensed Matter · Physics 2008-06-18 Stanislav Kotsev

We investigate the defect structures forming around two nanoparticles in a Gay-Berne nematic liquid crystal using molecular simulations. For small separations, disclinations entangle both particles forming the figure of eight, the figure of…

Soft Condensed Matter · Physics 2017-02-10 Anja Humpert , Samuel F. Brown , Michael P. Allen

We propose a novel computational strategy to study the glass transition of molecular fluids. Our approach combines the construction of simple yet realistic models with the development of Monte Carlo algorithms to accelerate equilibration…

Statistical Mechanics · Physics 2026-03-31 Romain Simon , Jean-Louis Barrat , Ludovic Berthier

The feasibility of shell-model calculations is radically extended by the Quantum Monte Carlo Diagonalization method with various essential improvements. The major improvements are made in the sampling for the generation of shell-model basis…

Nuclear Theory · Physics 2008-11-26 Michio Honma , Takahiro Mizusaki , Takaharu Otsuka

The STM induced rotation and dissociation dynamics of a single oxygen molecule on the Pt(111) surface have been finally determined by first principles calculations together with a newly developed statistical model for inelastic electron…

Other Condensed Matter · Physics 2010-10-28 Qiang Fu , Jinlong Yang , Yi Luo

We report new elastic and inelastic cross sections for O($^3P$)+CO$_2$ scattering at collision energies from 0.03 to 5 eV, of major importance to O escape from Mars, Venus, and CO$_2$-rich atmospheres. The cross sections were calculated…

Earth and Planetary Astrophysics · Physics 2021-01-19 Marko Gacesa , Robert J. Lillis , Kevin J. Zahnle

A mean field rate theory description of the homo- and co-polymerization of $f$-functional molecules is developed, which contains the formation of short cyclic structures inside the network. The predictions of this model are compared with…

Soft Condensed Matter · Physics 2021-03-31 Michael Lang , Konrad Schwenke , Jens-Uwe Sommer

In event-chain Monte Carlo simulations we model colloidal particles in two dimensions that interact according to an isotropic short-ranged pair potential which supports the two typical length scales present in decagonal quasicrystals. We…

Soft Condensed Matter · Physics 2020-05-14 M. Martinsons , J. Hielscher , S. C. Kapfer , M. Schmiedeberg