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Ensembles of nitrogen-vacancy (NV) centers in diamond are versatile quantum sensors with broad applications in the physical and life sciences. The concentration of neutral substitutional nitrogen ([N$_\text{s}^0$]) strongly influences…

Negatively-charged nitrogen-vacancy (NV$^-$) centers in diamond have generated much recent interest for their use in sensing. The sensitivity improves when the NV ground-state microwave transitions are narrow, but these transitions suffer…

We demonstrate a novel method for coherent optical manipulation of individual nuclear spins in the solid state, mediated by the electronic states of a proximal quantum emitter. Specifically, using the nitrogen-vacancy (NV) color center in…

Quantum Physics · Physics 2020-04-22 M. L. Goldman , T. L. Patti , D. Levonian , S. F. Yelin , M. D. Lukin

We present ab-initio calculations of photoionization thresholds and cross sections of the negatively charged nitrogen-vacancy (NV) center in diamond from the ground $^{3}\!A_2$ and the excited $^{3}\!E$ states. We show that after the…

The photoluminescence of nitrogen-vacancy (NV) centers in diamond nanoparticles exhibits specific properties as compared to NV centers in bulk diamond. For instance large fluctuations of lifetime and brightness from particle to particle…

Optics · Physics 2011-07-05 J. -J. Greffet , J. -P. Hugonin , M. Besbes , N. D. Lai , F. Treussart , J. -F. Roch

We use nominally forbidden electron-nuclear spin transitions in nitrogen-vacancy (NV) centers in diamond to demonstrate coherent manipulation of a nuclear spin ensemble using microwave fields at room temperature. We show that employing an…

Quantum Physics · Physics 2021-04-21 P. Huillery , J. Leibold , T. Delord , L. Nicolas , J. Achard , A. Tallaire , G. Hétet

We present systematic measurements of longitudinal relaxation rates ($1/T_1$) of spin polarization in the ground state of the nitrogen-vacancy (NV$^-$) color center in synthetic diamond as a function of NV$^-$ concentration and magnetic…

Quantum Physics · Physics 2015-12-17 A. Jarmola , A. Berzins , J. Smits , K. Smits , J. Prikulis , F. Gahbauer , R. Ferber , D. Erts , M. Auzinsh , D. Budker

Diamond-based quantum sensors have enabled high-resolution NMR spectroscopy at the microscale in scenarios where fast molecular motion averages out dipolar interactions among target nuclei. However, in samples with low-diffusion, ubiquitous…

Quantum Physics · Physics 2025-08-26 Carlos Munuera-Javaloy , Ander Tobalina , Jorge Casanova

In recent years, the field of quantum sensing has garnered increasing attention due to its potential to revolutionize various scientific and technological domains. Among the different quantum sensors, the nitrogen-vacancy (NV) color center…

Quantum Physics · Physics 2024-10-01 C. Munuera-Javaloy

The nitrogen vacancy (NV) center in diamond is a versatile color center used for magnetometry, quantum computing, and quantum communications. In this article, using a single laser beam as a pump and probe, we measure the spin states of the…

Applied Physics · Physics 2025-05-28 Reza Kashtiban , Gavin W. Morley , Mark E. Newton , A T M Anishur Rahman

The negatively charged nitrogen-vacancy (NV) center in diamond is a leading solid-state quantum emitter, offering spin-photon interfaces over a wide temperature range with applications from electromagnetic sensing to bioimaging. While NV…

Using a Hartman-Hahn protocol, we demonstrate spin polarization transfer from a single, optically-polarized nitrogen-vacancy (NV) center to the ensemble of paramagnetic defects hosted by an individual diamond nanocrystal. Owing to the…

Mesoscale and Nanoscale Physics · Physics 2017-03-14 Abdelghani Laraoui , Carlos A. Meriles

Here we propose and analyse in detail protocols that can achieve rapid hyperpolarization of 13C nuclear spins in randomly oriented ensembles of nanodiamonds at room temperature. Our protocols exploit a combination of optical polarization of…

Quantum Physics · Physics 2015-11-25 Q. Chen , I. Schwarz , F. Jelezko , A. Retzker , M. B. Plenio

Nuclear magnetic resonance (NMR) spectroscopy is widely used in fields ranging from chemistry, material science to neuroscience. Nanoscale NMR spectroscopy using Nitrogen-vacancy (NV) centers in diamond has emerged as a promising platform…

The ability to create time-dependent magnetic fields of controlled polarization is essential for many experiments with magnetic resonance. We describe a microstrip circuit that allows us to generate strong magnetic field at microwave…

Atomic Physics · Physics 2015-05-28 Mariusz Mrozek , Janusz Mlynarczyk , Daniel S. Rudnicki , Wojciech Gawlik

By using an ensemble of nitrogen-vacancy (NV) centers, the vector components of a time-varying (AC) magnetic field are measured in a phase sensitive manner. This allows for the determination of the magnetic field's polarization. This…

Quantum Physics · Physics 2025-07-01 M. S. J. Barson , T. J. Christie , J. P. Duff , K. Helmerson

We investigate nuclear spin hyperpolarization from nitrogen vacancy centers in isotopically enriched diamonds with $^{13}$C concentrations up to 100%. $^{13}$C enrichment leads to hyperfine structure of the nitrogen vacancy electron spin…

We perform sensitive nuclear magnetic resonance (NMR) with spin ensembles which are polarized by nitrogen vacancy centers (NV centers) in diamond at room-temperature. With a near shot-noise-limited photoluminescence detection and a highly…

New schemes that exploit the unique properties of Nitrogen-Vacancy (NV) centers in diamond are presently being explored as a platform for high-resolution magnetic sensing. Here we focus on the ability of a NV center to monitor an adjacent…

Mesoscale and Nanoscale Physics · Physics 2011-10-12 Abdelghani Laraoui , Jonathan S. Hodges , Colm Ryan , Carlos A. Meriles

Nitrogen-Vacancy (NV) color centers in diamond have emerged as promising quantum solid-state systems, with applications ranging from quantum information processing to magnetic sensing. One of the most useful properties of NVs is the ability…

Quantum Physics · Physics 2016-01-20 Sigal A. Wolf , Itamar Rosenberg , Ronen Rapaport , Nir Bar-Gill