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Lightweight 2D materials due to its large surface area are being studied for its hydrogen storage applications. The characteristics of hydrogen adsorption on the electric field-induced h-BN bilayer were investigated. The overall storage…

Chemical Physics · Physics 2021-06-01 B. Bhettri , P. K. Patra , D. P. Rai

Hydrogen adsorption on delta-Pu (100) and (111) surfaces using the generalized gradient approximation of the density functional theory with Perdew and Wang functionals have been studied at both the spin-polarized level and the…

Strongly Correlated Electrons · Physics 2009-11-10 M. N. Huda , A. K. Ray

Van Hove singularities (VHS's) in the density of states play an outstanding and diverse role for the electronic and thermodynamic properties of crystalline solids. At the critical point the Fermi surface connectivity changes and topological…

Mesoscale and Nanoscale Physics · Physics 2016-12-06 Youngwook Kim , Patrick Herlinger , Pilkyung Moon , Mikito Koshino , Takashi Taniguchi , Kenji Watanabe , Jurgen. H Smet

The absorption sites and the low-lying rotational and vibrational (RV) energy states for H$_2$ adsorbed within a metal-organic framework are calculated via van der Waals density functional theory. The induced dipole due to bond stretching…

Other Condensed Matter · Physics 2015-05-20 Lingzhu Kong , Yves J. Chabal , David C. Langreth

We investigate and discuss how hydrogen behaves at the edges of a graphite sheet, in particular the armchair edge. Our density functional theory-based calculations results show that, in contrast to the zigzag edge [cf., e-J. Surf. Sci.…

We have investigated the adsorption of Li on graphene oxide using density functional theory. We show a novel and simple approach to achieve a positive lithiation potential on epoxy and hydroxyl functionalized graphene, compared to the…

Materials Science · Physics 2015-10-28 Rajiv K. Chouhan , Pushpa Raghani

As mechanical structures enter the nanoscale regime, the influence of van der Waals forces increases. Graphene is attractive for nanomechanical systems because its Young's modulus and strength are both intrinsically high, but the mechanical…

Mesoscale and Nanoscale Physics · Physics 2015-05-28 Steven P. Koenig , Narasimha G. Boddeti , Martin L. Dunn , J. Scott Bunch

Halogenated aromatic molecules assemble on surfaces forming both hydrogen and halogen bonds. Even though these systems have been intensively studied on flat metal surfaces, high-index vicinal surfaces remain challenging, as they may induce…

Materials Science · Physics 2018-01-17 Rengin Peköz , Davide Donadio

Nitrogen-doped graphene was recently synthesized and was reported to be a catalyst for hydrogen dissociative adsorption under a perpendicular applied electric field (F). In this work, the diffusion of H atoms on N-doped graphene, in the…

Materials Science · Physics 2012-02-15 Z. M. Ao , A. D. Hernández-Nieves , F. M. Peeters , S. Li

We study the low temperature properties of a single layer of parahydrogen adsorbed on graphene, by means of Quantum Monte Carlo simulations. The computed phase diagram is very similar to that of helium on the same substrate, featuring…

Mesoscale and Nanoscale Physics · Physics 2018-05-02 Marisa Dusseault , Massimo Boninsegni

We have theoretically investigated the electronic and magnetic properties of graphene whose zigzag edges are oxidized. The alteration of these properties by adsorption of $\mathrm{H_{2}O}$ and $\mathrm{NH_3}$ molecules have been considered.…

Chemical Physics · Physics 2015-05-14 Julia Berashevich , Tapash Chakraborty

Recent measurements of the conductivity of nanoperforated graphene are interpreted in terms of edges states existing near the edge of each nanohole. The perimetric quantization of edge states should result in the formation of a…

Mesoscale and Nanoscale Physics · Physics 2017-03-14 V. V. Enaldiev , V. A. Volkov

We have performed first-principles studies on adsorption patterns of hydrogen adatoms on uniaxially strained graphene. Our simulation reveals that the adsorption energy of adatoms are sensitive to the strain. Hydrogen adatoms on zigzag…

Mesoscale and Nanoscale Physics · Physics 2011-12-13 Daniel Cole , Li Yang

The geometric and electronic properties of Bi-adsorbed monolayer graphene, enriched by the strong effect of substrate, are investigated by first-principles calculations. The six-layered substrate, corrugated buffer layer, and slightly…

Materials Science · Physics 2016-08-24 S. Y. Lin , S. L. Chang , H. H. Chen , S. H. Su , J. C. A. Huang , M. -F. Lin

Crystallographic alignment between two-dimensional crystals in van der Waals heterostructures brought a number of profound physical phenomena, including observation of Hofstadter butterfly and topological currents, and promising novel…

Using first-principles calculations within density functional theory we demonstrate that the adsorption of single oxygen atom results in significant electron transfer from graphene to oxygen. This strongly disturbs the charge landscape of…

Materials Science · Physics 2015-06-11 M. Topsakal , S. Ciraci

Optical properties of graphene are explored by using the generalized tight-binding model. The main features of spectral structures, the form, frequency, number and intensity, are greatly enriched by the complex relationship among the…

Computational Physics · Physics 2016-07-20 Chiun-Yan Lin , Thi-Nga Do , Yao-Kung Huang , Ming-Fa Lin

Pillared Graphene Frameworks are a novel class of microporous materials made by graphene sheets separated by organic spacers. One of their main features is that the pillar type and density can be chosen to tune the material properties. In…

Materials Science · Physics 2017-07-04 Andrea Pedrielli , Simone Taioli , Giovanni Garberoglio , Nicola Maria Pugno

Theoretical calculations based on density functional theory have made significant contributions to our understanding of metal oxides, their surfaces, and the binding of molecules at these surfaces. In this paper we investigate the binding…

Materials Science · Physics 2007-05-23 Oyvind Borck , Elsebeth Schroder

The low-frequency magneto-optical absorption spectra of bilayer Bernal graphene are studied within the tight-binding model and gradient approximation. The interlayer interactions strongly affect the electronic properties of the Landau…

Mesoscale and Nanoscale Physics · Physics 2009-08-07 Yen-Hung Ho , Yu-Huang Chiu , De-Hone Lin , Chen-Peng Chang , Ming-Fa Lin
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