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Frequency references based on solid state spins promise simplicity, compactness, robustness, multifunctionality, ease of integration, and high densities of emitters. Nitrogen-vacancy (NV) centers in diamond are a natural candidate, but the…

Dynamic polarization protocols aim to hyperpolarize a spin bath by transferring spin polarization from a well-controlled qubit such as a quantum dot or a color defect. Building on techniques from shortcuts to adiabaticity, we design fast…

Quantum Physics · Physics 2021-02-17 Tamiro Villazon , Pieter W. Claeys , Anatoli Polkovnikov , Anushya Chandran

Polarization transfers from an electron spin to a nuclear spin are essential for various physical tasks, such as dynamic nuclear polarization in nuclear magnetic resonance and quantum state transformations on hybrid electron-nuclear spin…

Quantum Physics · Physics 2015-11-11 Haidong Yuan , Robert Zeier , Nikolas Pomplun , Steffen J. Glaser , Navin Khaneja

We discuss the polarization dynamics during solid effect dynamic nuclear polarization (DNP) in a central spin model that consists of an electron surrounded by many nuclei. To this end we use a recently developed formalism and validate first…

Other Condensed Matter · Physics 2016-03-23 Daniel Wiśniewski , Alexander Karabanov , Igor Lesanovsky , Walter Köckenberger

Bulk 13C polarization can be strongly enhanced in diamond at room-temperature based on the optical pumping of nitrogen-vacancy color centers. This effect was confirmed by irradiating suitably aligned single-crystals at a ~50 mT field…

An obstacle for spin-based quantum sensors is magnetic noise due to proximal spins. However, such a spin cluster surrounding the sensor can become an asset, if it can be controlled. Here, we polarize and readout a cluster of three nitrogen…

Quantum Physics · Physics 2016-09-07 Helena S. Knowles , Dhiren M. Kara , Mete Atatüre

The nitrogen vacancy (NV) color center in diamond is an enormously important platform for the development of quantum sensors, including for single spin and single molecule NMR. Detection of weak single-spin signals is greatly enhanced by…

Quantum Physics · Physics 2017-05-29 J. E. Lang , J. Casanova , Z. -Y. Wang , M. B. Plenio , T. S. Monteiro

Several efforts have been made to polarize the nearby nuclear environment of nitrogen vacancy (NV) centers for quantum metrology and quantum information applications. Different methods showed different nuclear spin polarization efficiencies…

Quantum Physics · Physics 2021-06-01 H. Duarte , H. T. Dinani , V. Jacques , J. R. Maze

We present dynamic nuclear polarization (DNP) in the simplest pseudospin quantum Hall ferromagnet (QHF) of an InSb two-dimensional electron gas with a large g factor using tilted magnetic fields. The DNP-induced amplitude change of a…

Mesoscale and Nanoscale Physics · Physics 2015-05-18 H. W. Liu , K. F. Yang , T. D. Mishima , M. B. Santos , Y. Hirayama

Understanding the origins of spin lifetimes in hybrid quantum systems is a matter of current importance in several areas of quantum information and sensing. Methods that spectrally map spin relaxation processes provide insight into their…

Precise coherent control of the individual electronic spins associated with atom-like impurities in the solid state is essential for applications in quantum information processing and quantum metrology. We demonstrate all-optical…

Quantum Physics · Physics 2015-03-05 Yiwen Chu , Matthew Markham , Daniel J. Twitchen , Mikhail D. Lukin

We propose a method for the estimation of the initial polarization of spinful nuclei of the 13 C isotope in diamond via a measurement of the evolution of the coherence of an NV center spin qubit. Existing polarization measurement methods…

Quantum Physics · Physics 2025-04-01 Mateusz Kuniej , Katarzyna Roszak

We demonstrate significant improvements of the spin coherence time of a dense ensemble of nitrogen-vacancy (NV) centers in diamond through optimized dynamical decoupling (DD). Cooling the sample down to $77$ K suppresses longitudinal spin…

The application of magnetic resonance (MR) spectroscopy at progressively smaller length scales may eventually permit "chemical imaging" of spins at the surfaces of materials and biological complexes. In particular, the negatively charged…

Mesoscale and Nanoscale Physics · Physics 2015-06-18 Hai-Jing Wang , Chang S. Shin , Scott J. Seltzer , Claudia E. Avalos , Alexander Pines , Vikram S. Bajaj

Nitrogen vacancy (NV) centers in diamond are promising elemental blocks for quantum optics [1, 2], spin-based quantum information processing [3, 4], and high-resolution sensing [5-13]. Yet, fully exploiting these capabilities of single NV…

Spin defects in solids, such as the nitrogen-vacancy (NV) center in diamond, have emerged as a key tool for detecting nuclear spins at the nanoscale. While active nuclear spin control via radio-frequency (RF) irradiation is often…

Recently, rotation sensors utilizing the nuclear spins of nitrogen-vacancy color centers in diamond have been demonstrated. However, these devices are power-intensive and challenging to integrate into small chip-based radiofrequency…

In recent years, nitrogen-vacancy (NV) color centers in diamond have become excellent solid-state quantum sensors due to their electronic spin properties. Especially for their easy optical initialization and detection, together with their…

Ensembles of nitrogen-vacancy (NV) centers in diamond are versatile quantum sensors with broad applications in the physical and life sciences. The concentration of neutral substitutional nitrogen ([N$_\text{s}^0$]) strongly influences…

Sensitive nanoscale magnetic resonance imaging (MRI) of target spins using nitrogen-vacancy (NV) centers in diamond will require a quantitative understanding of dominant noise at the surface. We probe this noise by applying dynamical…

Mesoscale and Nanoscale Physics · Physics 2014-07-11 Bryan A. Myers , Matthieu C. Dartiailh , Kenichi Ohno , Ananda Das , David D. Awschalom , Ania C. Bleszynski Jayich