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Related papers: Pulsed polarisation for robust DNP

200 papers

We use nominally forbidden electron-nuclear spin transitions in nitrogen-vacancy (NV) centers in diamond to demonstrate coherent manipulation of a nuclear spin ensemble using microwave fields at room temperature. We show that employing an…

Quantum Physics · Physics 2021-04-21 P. Huillery , J. Leibold , T. Delord , L. Nicolas , J. Achard , A. Tallaire , G. Hétet

Systems of spins with strong dipolar interactions and controlled dimensionality enable new explorations in quantum sensing and simulation. In this work, we investigate the creation of strong dipolar interactions in a two-dimensional…

Dynamic nuclear polarization is widely used to enhance the sensitivity of nuclear magnetic resonance. It is presently the method of choice for enhancing the sensitivity of high-field solid state NMR experiments performed under cryogenic…

Chemical Physics · Physics 2022-02-02 Maria Grazia Concilio , Ilya Kuprov , Lucio Frydman

Nitrogen-Vacancy (NV) centers in diamonds provide a room-temperature platform for various emerging quantum technologies, e.g. the long nuclear spin coherence times as potential quantum memory registers. We demonstrate a freezing protocol…

Quantum Physics · Physics 2023-08-14 Abhishek Kejriwal , Dasika Shishir , Sumiran Pujari , Kasturi Saha

We demonstrate operation of a rotation sensor based on the $^{14}$N nuclear spins intrinsic to nitrogen-vacancy (NV) color centers in diamond. The sensor employs optical polarization and readout of the nuclei and a radio-frequency…

We introduce a method for the measurement of the lower bound on the initial polarization of spinful nuclei in a diamond by following the coherence evolution of an NV center spin qubit after a simple scheme is operated on the qubit to…

Quantum Physics · Physics 2026-02-24 Mateusz Kuniej , Katarzyna Roszak

Direct dynamic nuclear polarization of 1H nuclei in frozen water and water-ethanol mixtures is demonstrated using silicon nanoparticles as the polarizing agent. Electron spins at dangling-bond sites near the silicon surface are identified…

Mesoscale and Nanoscale Physics · Physics 2014-01-14 M. C. Cassidy , C. Ramanathan , D. G. Cory , J. W. Ager , C. M. Marcus

The control of nuclear spins in quantum dots is essential to explore their many-body dynamics and exploit their prospects for quantum information processing. We present a unique combination of dynamic nuclear spin polarization and…

Mesoscale and Nanoscale Physics · Physics 2015-12-16 Florian Forster , Max Mühlbacher , Dieter Schuh , Werner Wegscheider , Geza Giedke , Stefan Ludwig

The electronic spins of the nitrogen-vacancy centers (NV centers) in Chemical-Vapor-Deposition (CVD) grown diamonds form ideal probes of magnetic fields and temperature, as well as promising qu-bits for quantum information processing.…

Quantum Physics · Physics 2021-03-31 C. Pellet-Mary , P. Huillery , M. Perdriat , A. Tallaire , G. Hétet

High fidelity quantum control over qubits is of crucial importance for realistic quantum computing, and it turns to be more challenging when there are inevitable interactions among qubits. By employing a bandselective shaped pulse, we…

We present an experimental study of the Dynamic Nuclear Polarization (DNP) of \si{} nuclei in silicon crystals of natural abundance doped with As in the temperature range 0.1-1 K and in strong magnetic field of 4.6 T. This ensures very high…

Mesoscale and Nanoscale Physics · Physics 2020-06-24 J. Jarvinen , D. Zvezdov , J. Ahokas , S. Sheludyakov , L. Lehtonen , S. Vasiliev , L. Vlasenko , Y. Ishikawa , Y. Fujii

In dynamic nuclear polarization (DNP) experiments, the compound is driven out-of-equilibrium by microwave (MW) irradiation of the radical electron spins. Their stationary state has been recently probed via electron double resonance (ELDOR)…

Strongly Correlated Electrons · Physics 2017-02-28 Filippo Caracciolo , Marta Filibian , Pietro Carretta , Alberto Rosso , Andrea De Luca

Initializing quantum registers with high fidelity is a fundamental precondition for many applications like quantum information processing and sensing. The electronic and nuclear spins of a Nitrogen-Vacancy (NV) center in diamond form an…

Quantum Physics · Physics 2020-04-06 K. Rama Koteswara Rao , Yihua Wang , Zingfu Zhang , Dieter Suter

Spin engineering of advanced pulse sequences has had a transformative impact on the development of nuclear magnetic resonance (NMR) spectroscopy, to an extending degree also electron paramagnetic resonance (EPR), and the hybrid between the…

Chemical Physics · Physics 2025-01-31 Jose P. Carvalho , Anders Bodholt Nielsen , Eniko Baligacs , Nino Wili , Niels Chr. Nielsen

We address a problem of generating a robust entangling gate between electronic and nuclear spins in the system of a single nitrogen-vacany centre coupled to a nearest Carbon-13 atom in diamond against certain types of systematic errors such…

Quantum Physics · Physics 2010-07-14 R. S. Said , J. Twamley

The novel aspect of the centre (NV-) in diamond is the high degree of spin polarisation achieved through optical illumination. In this paper it is shown that the spin polarisation occurs as a consequence of an electron-vibration interaction…

Materials Science · Physics 2010-11-15 Neil Manson , Lachlan Rogers , Marcus Doherty , Lloyd Hollenberg

Nitrogen vacancy (NV) centers in diamond have been used as ultrasensitive magnetometers to perform nuclear magnetic resonance (NMR) spectroscopy of statistically polarized samples at 1 - 100 nm length scales. However, the spectral linewidth…

In this work we investigated the time behavior of the polarization of bulk 13C nuclei in diamond above the thermal equilibrium. This nonthermal nuclear hyperpolarization is achieved by cross relaxation between two nitrogen related…

Mesoscale and Nanoscale Physics · Physics 2018-08-01 Ralf Wunderlich , Jonas Kohlrautz , Bernd Abel , Jürgen Haase , Jan Meijer

Magnetic Resonance Imaging (MRI) can characterize and discriminate among tissues using their diverse physical and biochemical properties. Unfortunately, submicrometer screening of biological specimens is presently not possible, mainly due…

Mesoscale and Nanoscale Physics · Physics 2010-11-03 C. A. Meriles , L. Jiang , G. Goldstein , J. S. Hodges , J. R. Maze , M. D. Lukin , P. Cappellaro

Nitrogen-vacancy (NV) centers in diamond have emerged as valuable tools for sensing and polarizing spins. Motivated by potential applications in chemistry, biology, and medicine, we show that NV-based sensors are capable of detecting single…

Quantum Physics · Physics 2016-03-10 M. Bruderer , P. Fernández-Acebal , R. Aurich , M. B. Plenio