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We present quantum electron transport theory that incorporates dynamical effects of motion of atoms on electrode-molecule interfaces in the calculations of the electric current. The theory is based on non-equilibrium Green's functions. We…

Mesoscale and Nanoscale Physics · Physics 2018-08-14 Vincent F. Kershaw , Daniel S. Kosov

Non-equilibrium Green's function theory for non-adiabatic effects in quantum transport [Kershaw and Kosov, J.Chem. Phys. 2017, 147, 224109 and J. Chem. Phys. 2018, 149, 044121] is extended to the case of interacting electrons. We consider a…

Mesoscale and Nanoscale Physics · Physics 2019-02-20 Vincent F. Kershaw , Daniel S. Kosov

The molecular junction geometry is modelled in terms of nuclear degrees of freedom that are embedded in a stochastic quantum environment of non-equilibrium electrons. Time-evolution of the molecular geometry is governed via a mean force, a…

Mesoscale and Nanoscale Physics · Physics 2020-10-28 Vincent F. Kershaw , Daniel S. Kosov

Molecule-electrode interfaces in molecular electronic junctions are prone to chemical reactions, structural changes, and localized heating effects caused by electric current. These can be exploited for device functionality or may be…

Mesoscale and Nanoscale Physics · Physics 2020-04-22 Riley J. Preston , Vincent F. Kershaw , Daniel S. Kosov

We present a novel ab initio non-equilibrium approach to calculate the current across a molecular junction. The method rests on a wave function based description of the central region of the junction combined with a tight binding…

Materials Science · Physics 2009-11-11 Martin Albrecht , Bo Song , Alexander Schnurpfeil

The interaction with time-dependent external fields, especially the interplay between time-dependent driving and quantum correlations, changes the familiar picture of electron transport through nanoscale systems. Although the exact solution…

Mesoscale and Nanoscale Physics · Physics 2020-02-13 Thomas D. Honeychurch , Daniel S. Kosov

We investigate the effect of time-dependent cyclic-adiabatic driving on the charge transport in quantum junction. We propose a nonequilibrium Greens function formalism to study statistics of the charge pumped (at zero bias) through the…

Statistical Mechanics · Physics 2016-02-03 Hari Kumar Yadalam , Upendra Harbola

The electric conductance of a molecular junction is calculated by recasting the Keldysh formalism in Liouville space. Dyson equations for nonequilibrium many body Green's functions (NEGF) are derived directly in real (physical) time. The…

Quantum Physics · Physics 2007-05-23 U. Harbola , S. Mukamel

Based on the nonequilibrium Green's function (NEGF), we develop a quantum nonlinear theory to study time-dependent ac transport properties in the low frequency and nonlinear bias voltage regimes. By expanding NEGF in terms of time to the…

Mesoscale and Nanoscale Physics · Physics 2023-11-07 Lei Zhang , Fuming Xu , Jian Chen , Yanxia Xing , Jian Wan

This review deals with the nonequilibrium Green's function (NEGF) method applied to the problems of energy transport due to atomic vibrations (phonons), primarily for small junction systems. We present a pedagogical introduction to the…

Mesoscale and Nanoscale Physics · Physics 2013-05-28 Jian-Sheng Wang , Bijay Kumar Agarwalla , Huanan Li , Juzar Thingna

Electron transport through a diatomic molecular tunnel junction shows wave like interference phenomenon. By using Keldysh non-equilibrium Green's function (NEGF) theory, we have explicitly presented current and differential conductance…

Mesoscale and Nanoscale Physics · Physics 2012-12-18 Muhammad Imran

We review a recent theoretical development based on non-equilibrium Green's function formalism to study heat transport in nanomechanical devices modeled by phononic systems of coupled quantum oscillators driven by ac forces and connected to…

Mesoscale and Nanoscale Physics · Physics 2015-06-12 Liliana Arrachea , Bruno Rizzo

Due to technological needs, nanoscale heat management, energy conversion and quantum thermodynamics have become key areas of research, putting heat pumps and nanomotors center stage. The treatment of these particular systems often requires…

Mesoscale and Nanoscale Physics · Physics 2024-04-26 Sebastián E. Deghi , Raúl A. Bustos-Marún

We introduce diagrammatic technique for Hubbard nonequilibrium Green functions (NEGF). The formulation is an extension of equilibrium considerations for strongly correlated lattice models to description of current carrying molecular…

Mesoscale and Nanoscale Physics · Physics 2016-11-04 Feng Chen , Maicol A. Ochoa , Michael Galperin

The nonequilibrium Green's function formalism provides a versatile and powerful framework for numerical studies of nonequilibrium phenomena in correlated many-body systems. For calculations starting from an equilibrium initial state, a…

Strongly Correlated Electrons · Physics 2024-07-11 Matthias Murray , Hiroshi Shinaoka , Philipp Werner

The interaction between electronic and vibrational degrees of freedom in single-molecule junctions may result from the dependence of the electronic energies or the electronic states of the molecular bridge on the nuclear displacement. The…

Mesoscale and Nanoscale Physics · Physics 2015-06-09 A. Erpenbeck , R. Härtle , M. Thoss

We present a theory of molecular motors based on the Ehrenfest dynamics for the nuclear coordinates and the adiabatic limit of the Kadanoff-Baym equations for the current-induced forces. Electron-electron interactions can be systematically…

Mesoscale and Nanoscale Physics · Physics 2018-07-25 Miroslav Hopjan , Gianluca Stefanucci , Enrico Perfetto , Claudio Verdozzi

This research demonstrates analytical time-dependent non-equilibrium green function (TD-NEGF) algorithms to investigate dynamical functionalities of quantum devices, especially for photon-assisted transports. Together with the lumped…

Mesoscale and Nanoscale Physics · Physics 2021-06-08 I-Lin Ho

We present a novel ab initio non-equilibrium approach to calculate the current across a molecular junction. The method rests on a wave function based full ab initio description of the central region of the junction combined with a tight…

Materials Science · Physics 2007-05-23 Alexander Schnurpfeil , Bo Song , Martin Albrecht

Nonequilibrium Green's functions represent a promising tool for describing central nuclear reactions. Even at the single-particle level, though, the Green's functions contain more information that computers may handle in the foreseeable…

Nuclear Theory · Physics 2016-05-04 Pawel Danielewicz , Arnau Rios , Brent Barker
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