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Using classical electrodynamics we determine the angular dependence of the light intensities radiated in second and third harmonic generation by spherical metal clusters. Forward and backward scattering is analyzed in detail. Also resonance…

Condensed Matter · Physics 2007-05-23 J. Dewitz , W. Hubner , K. H. Bennemann

Layered van der Waals (vdW) materials have emerged as a promising platform for nanophotonics due to large refractive indexes and giant optical anisotropy. Unlike conventional dielectrics and semiconductors, the absence of covalent bonds…

Nonlinear metasurfaces have become prominent tools for controlling and engineering light at the nanoscale. Usually, the polarization of the total generated third harmonic is studied. However, diffraction orders may present different…

We develop multipolar theory of nonlinear generation of entangled photons from subwavelength dielectric particles due to the spontaneous parametric downconversion. We demonstrate that optical excitation in resonance with the high-quality…

Optics · Physics 2018-08-15 Alexander N. Poddubny , Daria A. Smirnova

In the currently accepted models of the nonlinear optics, the nonlinear radiation was treated as the result of an infinitesimally thin polarization sheet layer, and a three layer model was generally employed. The direct consequence of this…

Chemical Physics · Physics 2016-08-29 De-sheng Zheng , Yuan Wang , An-an Liu , Hong-fei Wang

We examine the far-field optical response, under-plane wave excitation in the presence of a static magnetic field, of core-shell nanoparticles involving a gyroelectric component, either as the inner or the outer layer, through analytic…

Mesoscale and Nanoscale Physics · Physics 2020-11-13 P. Elli Stamatopoulou , Vassilios Yannopapas , N. Asger Mortensen , Christos Tserkezis

Plasmonic resonances in metallic nanostructures have been shown to drastically enhance local electromagnetic fields, and thereby increase the efficiency of nonlinear optical phenomena, such as second harmonic generation (SHG). While it has…

In this article, we analytically study second harmonic (SH) generation from thin metallic films with subwavelength, non-centrosymmetry patterns. Because the thickness of the film is much smaller than the SH wavelength, retardation effects…

Optics · Physics 2009-05-11 Yong Zeng , Jerome V. Moloney

It has been recently suggested that the nonlinear optical processes in plasmonic nanoantennas allow for a substantial boost in the sensitivity of plasmonic sensing platforms. Here we present a sensing device based on an array of…

We study optical harmonic generation on the 1S exciton-polariton in the semiconductor ZnSe. Intense and spectrally narrow exciton resonances are found in optical second (SHG), third (THG), and fourth (FHG) harmonic generation spectra. The…

Optics · Physics 2020-07-29 Johannes Mund , Dmitri R. Yakovlev , Marina A. Semina , Manfred Bayer

Recent techniques have allowed transition metal dichalcogenides (TMD) monolayers to be grown and adequately characterised. Of particular interest, their nonlinear optical response presents many promising opportunities for future…

Mesoscale and Nanoscale Physics · Physics 2020-03-06 David N. Carvalho , Fabio Biancalana

High-index spherical nanoparticles with low material losses support sharp high-Q electric and magnetic resonances and exhibit a number of interesting optical phenomena. Developments in fabrication techniques have enabled the further study…

Optics · Physics 2020-12-30 D. A. Pidgayko , Z. F. Sadrieva , K. S. Ladutenko , A. A. Bogdanov

Extended defects with one dimensionality smaller than that of the host, such as 2D grain boundaries in 3D materials or 1D grain boundaries in 2D materials, can be particularly damaging since they directly impede the transport of charge,…

Enhancement of optical response with high-index dielectric nanoparticles is attributed to the excitation of their Mie-type magnetic and electric resonances. Here we study Raman scattering from crystalline silicon nanoparticles and reveal…

Topological photonics enables robust light manipulation with third-order optical nonlinearity, yet integrating second-order optical nonlinearity into a topological system faces fundamental challenges: frequency-dependent topological…

Optics · Physics 2025-06-30 Ruoyu Wang , Yiming Pan , Xiaoqin Shen

We show that the lack of inversion symmetry in monolayer MoS2 allows strong optical second harmonic generation. Second harmonic of an 810-nm pulse is generated in a mechanically exfoliated monolayer, with a nonlinear susceptibility on the…

Materials Science · Physics 2015-06-15 Nardeep Kumar , Sina Najmaei , Qiannan Cui , Frank Ceballos , Pulickel M. Ajayan , Jun Lou , Hui Zhao

Scattering of electromagnetic waves by an arbitrary nanoscale object can be characterized by a multipole decomposition of the electromagnetic field that allows to describe the scattering intensity and radiation pattern through interferences…

Optics · Physics 2017-02-22 Wei Liu , Yuri S. Kivshar

Nonlinear disordered media uniquely combine multiple scattering and second-harmonic generation. Here, we investigate the statistical properties of the nonlinear light generated within such media. We report super-Rayleigh statistics of the…

Generation of second-harmonic waves is one of the universal nonlinear phenomena that have found numerous technical applications in many modern technologies, in particular, in photonics. This phenomenon also has great potential in the field…

Mesoscale and Nanoscale Physics · Physics 2024-03-01 K. O. Nikolaev , S. R. Lake , G. Schmidt , S. O. Demokritov , V. E. Demidov

We show that spatially structured radiation generates second harmonic in a two-dimensional system even if the system is homogeneous and isotropic. The effect originates from non-locality of electric response to structured electromagnetic…

Mesoscale and Nanoscale Physics · Physics 2025-04-23 A. A. Gunyaga , M. V. Durnev , S. A. Tarasenko