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Polarization-dependent photon spectroscopy (dichroism) of the second-harmonic generation (SHG) response is shown to reveal chiral and magnetic properties of a sample. Two dichroic signals are allowed with electric-dipole (E1) and…

Strongly Correlated Electrons · Physics 2019-12-11 S. W. Lovesey , G. van der Laan

Second-harmonic generation (SHG) is a quintessential probe of inversion symmetry breaking in condensed matter. While perturbative $\chi^{(2)}$ processes are well-documented, the nonperturbative regime under intense driving remains largely…

Strongly Correlated Electrons · Physics 2026-04-08 Keisuke Kitayama , Masao Ogata

We present theoretical studies of high-order harmonic generation (HHG) produced by non-homogeneous fields as resulting from the illumination of plasmonic nanostructures with a short laser pulse. We show that both the inhomogeneity of the…

Atomic Physics · Physics 2012-04-27 M. F. Ciappina , J. Biegert , R. Quidant , M. Lewenstein

Two-dimensional (2D) materials serve as exceptional platforms for controlled second harmonic generation (SHG), an important nonlinear optical phenomenon with diverse applications. Current approaches to SHG control often depend on…

Mesoscale and Nanoscale Physics · Physics 2024-07-03 Soonyoung Cha , Tianyi Ouyang , Takashi Taniguchi , Kenji Watanabe , Nathaniel M. Gabor , Chun Hung Lui

The outstanding optical properties for plasmon resonances in noble metal nanoparticles enable the observation of non-linear optical processes such as second-harmonic generation (SHG) at the nanoscale. Here, we investigate the SHG process in…

The second-order nonlinear optical susceptibility $\Pi^{(2)}$ for second harmonic generation is calculated for gapped graphene. The linear and second-order nonlinear plasmon excitations are investigated in context of second harmonic…

Mesoscale and Nanoscale Physics · Physics 2015-06-17 Godfrey Gumbs , Yonatan Abranyos , Upali Aparajita , Oleksiy Roslyak

Here we employ the quasi-bound state in the continuum (quasi-BIC) resonance in all-dielectric metasurfaces for efficient nonlinear processes in consideration of the backward frequency conversion. We theoretically study the second-harmonic…

Optics · Physics 2024-06-28 Xu Tu , Siqi Feng , Jiajun Li , Yangguang Xing , Feng Wu , Tingting Liu , Shuyuan Xiao

Mid-infrared nanophotonics can be realized using sub-diffractional light localization and field enhancement with surface phonon polaritons in polar dielectric materials. We experimentally demonstrate second harmonic generation due to the…

Optical resonances in nanostructures enable strong enhancement of nonlinear processes at the nanoscale, such as second-harmonic generation (SHG), with high-$Q$ modes providing intensified light--matter interactions and sharp spectral…

High-harmonic generation (HHG) in solids has been touted as a way to probe ultrafast dynamics and crystal symmetries in condensed matter systems. Here, we investigate the polarization properties of high-order harmonics generated in…

We predict frequency multiplication of surface acoustic waves in dielectric substrates via the ferromagnetic resonance of adjacent magnetic transducers when driven by microwaves. We find pure second harmonic generation (SHG) without any…

Mesoscale and Nanoscale Physics · Physics 2023-03-29 Chengyuan Cai , Xi-Han Zhou , Weichao Yu , Tao Yu

The second harmonic generation is one of the most important applications of nonlinear effect, which has attracted great interests in nonlinear optics and microwave in the past decades. To the best of our knowledge, however, generating the…

Optical harmonic generation on excitons is found in ZnSe/BeTe quantum wells with type-II band alignment. Two experimental approaches with spectrally-broad femtosecond laser pulses and spectrally-narrow picosecond pulses are used for…

We present a combined experimental and theoretical study of enhanced third-harmonic generation (THG) in silicon nitride metasurfaces. These structures exhibit strong resonant nonlinear responses, enabling up to two orders of magnitude…

Strong second harmonic generation (SHG) in silicon nitride has been extensively studied-among others, in terms of laser-induced SHG enhancement in Si3N4 waveguides. This enhancement has been ascribed to the all-optical poling induced by the…

Broken symmetries and electronic topology are nicely manifested together in the second order nonlinear optical responses from topologically nontrivial materials. While second order nonlinear optical effects from the electric dipole (ED)…

Materials Science · Physics 2023-10-25 Youngjun Ahn , Xiaoyu Guo , Rui Xue , Kejian Qu , Kai Sun , David Mandrus , Liuyan Zhao

Second-harmonic (SH) generation is tremendously important for nonlinear sensing, microscopy and communication system. One of the great challenges of current designs is to enhance the SH signal and simultaneously tune its radiation direction…

We theoretically study high-order harmonic generation (HHG) from solid-phase systems in spatially inhomogeneous strong laser fields originated by resonant plasmons within a metallic nanostructure. The intensity of the second plateau in HHG…

Optics · Physics 2016-09-12 Tao-Yuan Du , Zhong Guan , Xiao-Xin Zhou , Xue-Bin Bian

The nonlinear magneto-plasmonics aims to utilize plasmonic excitations to control the mechanisms and taylor the efficiencies of the non-linear light frequency conversion at the nanoscale. We investigate the mechanisms of magnetic second…

We show that the second harmonic generation (SHG) is enhanced in the chiral one-dimensional electron currents in a broad frequency range. The origin of the enhancement is two-fold: first, the linear dispersion of the current and the…

Mesoscale and Nanoscale Physics · Physics 2020-04-17 Ivan Iorsh , Gulnaz Rakhmanova
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