Related papers: Optical chirality in high harmonic generation
Polarisation effects in the microcavity parametric oscillator are studied using a simple model in which two chi-three optical parametric oscillators are coupled together. It is found that there are, in general, a number of steady states of…
This thesis is mainly devoted to the study of the quantum properties of optical parametric oscillators (OPOs), which are nowadays the sources of the highest-quality quantum-correlated light, apart from fundamental tools in the…
Chirality describes the asymmetry between an object and its mirror image and manifests itself in diverse functionalities across all scales of matter - from molecules and aggregates to thin films and bulk chiral materials. A particularly…
We show how both the ellipticity $\eta$ and degree of polarization $\textit{P}$ influences the extraordinary optical chirality properties of non-paraxial vortex beams. We find that, in stark contrast to paraxial optics and non-vortex modes,…
We demonstrate that electric-dipole scatterers can mimic chiral light-matter interaction by generating far-field circular polarization upon scattering, even though the optical chirality of the incident field as well as that of the scattered…
The present work introduces a robust way to generate attosecond pulses with tunable ellipticity via high-order harmonic generation by co-rotating $\omega - 2\omega$ bicircular laser fields. The total electric field of the laser fields…
We employ a rotating frame of reference to elucidate high-harmonic generation of circularly polarized light by bicircular driving fields. In particular, we show how the experimentally observed circular components of the high-harmonic…
Chirality is a structural property of molecules lacking mirror symmetry that has strong implications in diverse fields, ranging from life to materials sciences. Established spectroscopic methods that are sensitive to chirality, such as…
Chiroptical effects, characterized by different optical responses for left- (LCP) and right- handed circularly polarized light (RCP), are powerful and valuable tools in optics with wide applications in polarization resolved imaging and…
Similariton-like pulses are found to be formed in synchronously pumped singly resonant optical parametric oscillators (OPO) by numerical simulation. The nonlinear coupled-wave equations can be reduced to inhomogeneous nonlinear…
Chirality, a fundamental property of asymmetric structures, plays a crucial role in pharmaceutical, biological and chemical systems, offering a powerful tool for screening organic compounds. While the conventional optical chirality…
We extend the concept of radially and azimuthally polarized optical beams to the polychromatic domain by introducing cylindrically polarized nondiffracting optical pulses. In particular, we discuss in detail the case of cylindrically…
Chirality is ubiquitous in nature and of fundamental importance in science. The present work focuses on understanding the conditions required to modify the chirality during ultrafast electronic motion by bringing enantiomers…
Molecular chirality is a key design property for many technologies including bioresponsive imaging, circularly polarized light detection and emission, molecular motors and switches. Imaging and manipulating the primary steps of transient…
We present a comprehensive theoretical investigation of high-order harmonic generation in H$_2^+$ molecular ions within a quantum optical framework. Our study focuses on characterizing various quantum optical and quantum information…
The rotation of polarization occurs for light interacting with chiral materials. It requires the light states with opposite chiralities interact differently with the materials. We demonstrate analogous rotation of polarization also exists…
Chiroptical techniques for detecting and characterizing the chirality of matter and artificial nanostructures are traditionally based on their interaction with chiral light, typically circularly-polarized fields propagating in free space.…
We calculate the quantum correlations existing among the three output fields (pump, signal, and idler) of a triply resonant non-degenerate Optical Parametric Oscillator operating above threshold. By applying the standard criteria [P. van…
When ultrafast noncritical cascaded second-harmonic generation of energetic femtosecond pulses occur in a bulk lithium niobate crystal optical Cherenkov waves are formed in the near- to mid-IR. Numerical simulations show that the few-cycle…
We analyze how chirality can generate pulling optical forces and left-handed torques by cross-coupling linear-to-angular momenta between the light field and the chiral object. In the dipolar regime, we reveal that such effects can emerge…