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The absorption of large bipolarons is investigated using the path-integral method. The response of a bipolaron to an external electromagnetic field is derived in the framework of the memory-function approach. The bipolaron optical…

Strongly Correlated Electrons · Physics 2009-10-31 J. T. Devreese , S. N. Klimin , V. M. Fomin

A novel approach to obtain the excitation spectrum of nuclei is presented as well as its proof-of-principle. The Monte Carlo Shell Model is extended so that the excitation spectrum can be calculated from its ground state with full of…

Nuclear Theory · Physics 2018-07-02 Takaharu Otsuka , Tomoaki Togashi , Noritaka Shimizu , Yutaka Utsuno , Toshio Suzuki

X-ray absorption spectroscopy (XAS) is a powerful experimental technique to probe the local order in materials with core electron excitations. Experimental interpretation requires supporting theoretical calculations. For water, these…

Computational Physics · Physics 2022-05-17 Fujie Tang , Zhenglu Li , Chunyi Zhang , Steven G. Louie , Roberto Car , Diana Y. Qiu , Xifan Wu

We present a unified theory of luminescence spectra for highly excited semiconductors, which is applicable both to the electron-hole BCS state and to the exciton Bose-Einstein condensate. The crossover behavior between electron-hole BCS…

Strongly Correlated Electrons · Physics 2009-10-31 T. J. Inagaki , M. Aihara , A. Takahashi

Doppler-broadened $\gamma$-ray spectra for positron annihilation on molecules are calculated using many-body theory. By employing Gaussian bases for the electron and positron wavefunctions, a computable expression that involves a…

Atomic Physics · Physics 2025-02-19 S. K. Gregg , J. P. Cassidy , A. R. Swann , J. Hofierka , B. Cunningham , D. G. Green

We present a first-principles-based multiscale simulation framework for quantitative predictions of the high-energy part of the Ultraviolet Photoelectron Spectroscopy (UPS) spectra of amorphous molecular solids. The approach combines a…

This chapter introduces the use of X-ray absorption spectroscopy (XAS) in studying the local electronic and atomic structure of high-entropy materials. The element selectivity of XAS makes it particularly suitable to address the challenges…

Materials Science · Physics 2024-11-12 Alexei Kuzmin

We present a formalism for the resonant inelastic x-ray scattering (RIXS) cross section. The resulting compact expression in terms of polarizability matrix elements, particularly lends itself to the implementation in an all-electron…

Materials Science · Physics 2022-08-17 Christian Vorwerk , Francesco Sottile , Claudia Draxl

We present a comprehensive study of the optical transitions and selection rules of variably charged single self-assembled InAs/GaAs quantum dots. We apply high resolution polarization sensitive photoluminescence excitation spectroscopy to…

Mesoscale and Nanoscale Physics · Physics 2012-08-28 Y. Benny , Y. Kodriano , E. Poem , T. A. Truong , P. M. Petroff , D. Gershoni

We demonstrate tunneling spectroscopy of synthetic quantum matter in superconducting circuit lattices. We measure site-resolved excitation spectra by coupling the lattice to engineered driven-dissipative particle baths that serve as local…

Quantum Gases · Physics 2025-05-20 Botao Du , Qihao Guo , Santiago López , Ruichao Ma

We present initial results from observations of the low-mass X-ray binary EXO 0748-67 with the Reflection Grating Spectrometer on board the XMM-Newton Observatory. The spectra exhibit discrete structure due to absorption and emission from…

Astrophysics · Physics 2011-05-23 J. Cottam , S. M. Kahn , A. C. Brinkman , J. W. den Herder , C. Erd

The component of photoexcited states with large spatial extent is investigated for poly(para-phenylenevinylene) using the intermediate exciton theory. We find a peak due to long-range excitons at the higher-energy side of the lowest main…

Condensed Matter · Physics 2008-02-03 Kikuo Harigaya

Measurements of x-ray emission and absorption spectra of the constituents of MgB$_2$ are presented. The results obtained are in good agreement with calculated x-ray spectra, with dipole matrix elements taken into account. The comparison of…

We study Fermi edge singularities in photo-absorption spectra of generic mesoscopic systems such as quantum dots or nanoparticles. We predict deviations from macroscopic-metallic behavior and propose experimental setups for the observation…

Mesoscale and Nanoscale Physics · Physics 2009-08-12 M. Hentschel , D. Ullmo , H. U. Baranger

We present an \textit{ab initio} method to calculate phonon-assisted absorption and emission spectra in the presence of strong excitonic effects. We apply the method to bulk hexagonal BN which has an indirect band gap and is known for its…

Materials Science · Physics 2019-05-15 Fulvio Paleari , Henrique P. C. Miranda , Alejandro Molina-Sánchez , Ludger Wirtz

The lowest electronic excitations of benzene and a set of donor-acceptor molecular complexes are calculated for the gas phase and on the Al(111) surface using the many-body Bethe-Salpeter equation (BSE). The energy of the charge-transfer…

Mesoscale and Nanoscale Physics · Physics 2015-05-27 J. M. Garcia-Lastra , K. S. Thygesen

Cyclotron Radiation Emission Spectroscopy (CRES) is an approach to measuring the energy of an electron trapped in an externally applied magnetic field. The bare electron can come from different interactions, including photoelectric…

Atomic Physics · Physics 2020-08-12 Kareem Kazkaz , Nathan Woollett

In this paper, we propose a Bayesian spectral deconvolution considering the properties of peaks in different energy domains. Bayesian spectral deconvolution regresses spectral data into the sum of multiple basis functions. Conventional…

Coherent two-dimensional spectroscopy in IR or visible region is very effective for studying correlations, energy relaxation/transfer pathways in complex multi-chromophore or multi-mode systems. However it is usually restricted up to…

Chemical Physics · Physics 2020-09-15 Darius Abramavicius

We report on a new general relativistic computational model enhancing, in various respects, the capability of presently available tools for fitting spectra of X-ray sources. The new model is intended for spectral analysis of black-hole…

Astrophysics · Physics 2011-02-22 M. Dovciak , V. Karas , A. Martocchia , G. Matt , T. Yaqoob