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The recently developed technique of Cyclotron Radiation Emission Spectroscopy (CRES) uses frequency information from the cyclotron motion of an electron in a magnetic bottle to infer its kinetic energy. Here we derive the expected radio…

High-spatial-resolution vibrational spectroscopy is one of the principal techniques for nanoscale compositional analysis in biological materials. Here, we present a new method for the analysis of whole-cell biological specimens through…

Laser-plasma technology promises a drastic reduction of the size of high energy electron accelerators. It could make free electron lasers available to a broad scientific community, and push further the limits of electron accelerators for…

Time-resolved femtosecond stimulated Raman spectroscopy (FSRS) is a powerful tool for investigating ultrafast structural and vibrational dynamics in light absorbing systems. However, the technique generally requires exposing a sample to…

Instrumentation and Detectors · Physics 2018-07-10 Matthew N. Ashner , William A. Tisdale

We theoretically propose a multidimensional high-harmonic echo spectroscopy technique which utilizes strong optical fields to resolve coherent electron dynamics spanning an energy range of multiple electron Volts. Using our recently…

The operation of photoemission electron sources with wavelengths near the photoemission threshold has been shown to dramatically decrease the minimum achievable photocathode emittance, but at the cost of significantly reduced quantum…

Accelerator Physics · Physics 2018-08-22 Jai Kwan Bae , Ivan Bazarov , Pietro Musumeci , Siddharth Karkare , Howard Padmore , Jared Maxson

Electron beam accelerators are essential in many scientific and technological fields. Their operation relies heavily on the stability and precision of the electron beam. Traditional diagnostic techniques encounter difficulties in addressing…

Machine Learning · Computer Science 2024-11-18 Till Korten , Vladimir Rybnikov , Mathias Vogt , Juliane Roensch-Schulenburg , Peter Steinbach , Najmeh Mirian

Performing time and angle resolved photoemission spectroscopy (tr-ARPES) at high momenta necessitates extreme ultraviolet laser pulses, which are typically produced via high harmonic generation (HHG). Despite recent advances, HHG-based…

The Scanning electron microscope (SEM) and Electron-Dispersive Spectroscope (EDS) are two highly effective instruments in the field of nanoscience and nanotechnology. The quality of these instruments is determined by various factors, with…

Applied Physics · Physics 2023-10-24 Hamidreza Moradi , Fatemeh Mehradnia

One of the frontiers in electron scattering is to couple ultrafast temporal resolution with highly localized probes to investigate the role of microstructure on material properties. Here, taking advantage of the unprecedented average…

Applied Physics · Physics 2019-06-07 Fu-Hao Ji , Daniel Durham , Andrew Minor , Pietro Musumeci , Jorge Navarro , Daniele Filippetto

We report the design and performance of a time-resolved electron diffraction apparatus capable of producing intense bunches with simultaneously single digit micron probe size, long coherence length, and $200$ fs rms time resolution. We…

Modern particle accelerators and their applications increasingly rely on precisely coordinated interactions of intense charged particle and laser beams. Femtosecond-scale synchronization alongside micrometre-scale spatial precision are…

Imaging changes in molecular geometries on their natural femtosecond timescale with sub-Angstrom spatial precision is one of the critical challenges in the chemical sciences, since the nuclear geometry changes determine the molecular…

We report on the first detailed beam test attesting the fundamental principle behind the development of high-current-efficiency ultrafast electron microscope systems where a radio-frequency cavity is incorporated as a condenser lens in the…

Materials Science · Physics 2024-01-03 Xiaoyi Sun , Joseph William , Sachin Sharma , Shriraj Kunjir , Dan Morris , Shen Zhao , Chong-Yu Ruan

Resonant radiofrequency cavities enable exquisite time-energy control of electron beams when synchronized with laser driven photoemission. We present a lossless monochromator design that exploits this fine control in the…

Accelerator Physics · Physics 2021-01-07 Cameron J. R. Duncan , David A. Muller , Jared M. Maxson

We report on the development of an ultrafast Transmission Electron Microscope based on a laser-driven cold-field emission source. We first describe the instrument before reporting on numerical simulations of the laser-driven electron…

Optics · Physics 2019-11-27 G. M. Caruso , F. Houdellier , S. Weber , M. Kociak , A. Arbouet

The advent of isolated and intense sub-femtosecond X-ray pulses enables tracking of quantummechanical motion of electrons in molecules and solids. The combination of X-ray spectroscopy and diffraction imaging is a powerful approach to…

Phase-shaped electron energy-loss spectroscopy (PSEELS) measures the scattering probability of structured free electron beams by a target. Over the last decade, it was shown that this scheme can be employed to emulate polarized optical…

Optics · Physics 2024-11-19 Simon Garrigou , Hugo Lourenço-Martins

Electron energy-loss spectroscopy (EELS) coupled with scanning transmission electron microscopy (STEM) is a powerful technique to determine materials composition and bonding with high spatial resolution. Noise is often a limitation…

Instrumentation and Detectors · Physics 2025-05-21 Yifan Wang , Mai Tan , Carlos Fernandez-Granda , Peter A. Crozier

Many experiments in biological and medical sciences currently use multiphoton microscopy as a core imaging technique. To date, solid-state lasers are most commonly used as excitation beam sources. However, the most demanding applications…