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Femtosecond coherent multidimensional spectroscopy is demonstrated for an ultracold gas. For this, a setup for phase modulation spectroscopy is used to probe the $3^2\mathrm{S}_{1/2} - 2^2\mathrm{P}_{1/2, 3/2}$ transition in an 800…

Atomic Physics · Physics 2023-01-16 Friedemann Landmesser , Tobias Sixt , Katrin Dulitz , Lukas Bruder , Frank Stienkemeier

High-brightness femtosecond-to-attosecond pulses are indispensable for probing electron dynamics on their fundamental temporal scales. X-ray free-electron lasers (XFELs) at high repetition rates will facilitate high-statistics measurements…

Accelerator Physics · Physics 2026-05-01 Junhao Liu , Zhen Wang , Lanpeng Ni , Yujie Lu , Chao Feng , Zhentang Zhao

High-harmonic spectroscopy (HHS) is a nonlinear all-optical technique with inherent attosecond temporal resolution, which has been applied successfully to a broad variety of systems in the gas phase and solid state. Here, we extend HHS to…

The temporal resolution of ultrafast electron diffraction (UED) at weakly relativistic beam energies ($\lesssim$ 100 keV) suffers from space-charge induced electron pulse broadening. We describe the implementation of a radio frequency (RF)…

Accelerator Physics · Physics 2024-05-08 Thomas Sutter , Joshua Lee , Atharva Kulkarni , Pietro Musumeci , Anshul Kogar

Current advances in ultrafast electron microscopy make it possible to combine optical pumping of a nanostructure and electron beam probing with sub{\aa}ngstrom and femtosecond spatiotemporal resolution. We present a theory predicting that…

Recent advancements in ultrafast laser systems and high harmonic generation (HHG) techniques have enabled time-resolved photoemission spectroscopy on femtosecond timescales, opening up unprecedented opportunities to explore quantum…

Strongly Correlated Electrons · Physics 2025-11-03 Takeshi Suzuki , Kozo Okazaki

Superconducting transition-edge sensors (TES) are extremely sensitive microcalorimeters used as photon detectors with unparalleled energy resolution. They have found application from measuring astronomical spectra through to determining the…

Photons, electrons, and their interplay are at the heart of photonic devices and modern instruments for ultrafast science [1-10]. Nowadays, electron beams of the highest intensity and brightness are created by photoemission with short laser…

Watching the motion of electrons on their natural nanometre length- and femtosecond time scales is a fundamental goal and an open challenge of contemporary ultrafast science. Optical techniques and electron microscopy currently mostly…

Optics · Physics 2018-01-23 Jan Vogelsang , Germann Hergert , Dong Wang , Petra Groß , Christoph Lienau

Electron beam energies in Transmission Electron Microscopes (TEMs) reach the relativistic realm constituting Quantum Electrodynamics (QED) the appropriate framework for the study of electron matter interaction in TEMs. We focus on the…

Atomic Physics · Physics 2026-01-12 Ioannis Iatrakis , Valerii Brudanin

A high-current electron source for inverse photoemission spectroscopy (IPES) is described. The source comprises a thermal cathode electron emission system, an electrostatic deflector-monochromator, and a lens system for variable kinetic…

Materials Science · Physics 2024-01-30 H. Ibach , H. Sato , M. Kubo , F. S. Tautz , H. Yoshida , F. C. Bocquet

Ultrafast transmission electron microscopy (UTEM) has emerged as a versatile technique for the time-resolved imaging of nanoscale dynamics on timescales down to few-hundred attoseconds but the temporal and spatial resolutions are still…

Instrumentation and Detectors · Physics 2024-11-01 Alexander Schröder , Andreas Wendeln , Jonathan T. Weber , Masaki Mukai , Yuji Kohno , Sascha Schäfer

The femtosecond evolution of the electronic temperature of laser-excited gold nanoparticles is measured, by means of ultrafast time-resolved photoemission spectroscopy induced by extreme-ultraviolet radiation pulses. The temperature of the…

Scanning Electron Microscopy (SEM) is pivotal in revealing intricate micro- and nanoscale features across various research fields. However, obtaining high-resolution SEM images presents challenges, including prolonged scanning durations and…

Image and Video Processing · Electrical Eng. & Systems 2024-10-08 Tom Reclik , Setareh Medghalchi , Philipp Schumacher , Maximilian Wollenweber , Talal Al-Samman , Sandra Korte-Kerzel , Ulrich Kerzel

We present a review on the developments in the photoemission spectrometer with a vacuum ultraviolet laser at Institute for Solid State Physics at the University of Tokyo. The advantages of high energy resolution, high cooling ability, and…

Superconductivity · Physics 2016-03-02 Takahiro Shimojima , Kozo Okazaki , Shik Shin

Electron energy loss spectroscopy (EELS) has been established as a powerful analytical technique for investigating the oxidation state, band structure, and dielectric properties of materials with exceptional spatial resolution. Inspired by…

Aberration-corrected optics have made electron microscopy at atomic-resolution a widespread and often essential tool for nanocharacterization. Image resolution is dominated by beam energy and the numerical aperture of the lens ({\alpha}),…

Van der Waals (vdW) materials exhibit intriguing structural, electronic and photonic properties. Electron Energy Loss Spectroscopy (EELS) within Scanning Transmission Electron Microscope (STEM) allows for nanoscale mapping of such…

An environmental cell high resolution electron microscope (EHREM) has been developed for in situ studies of dynamic chemical reactions on the atomic scale. It allows access to metastable intermediate phases of catalysts and to sequences of…

Chemical Physics · Physics 2017-05-17 Edward Boyes , Pratibha Gai

Scanning transmission electron microscopy (STEM) has advanced rapidly in the last decade thanks to the ability to correct the major aberrations of the probe forming lens. Now atomic-sized beams are routine, even at accelerating voltages as…