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We report the development of a continuous-wave and pulsed X-band electron spin resonance (ESR) spectrometer for the study of spins on ordered surfaces down to cryogenic temperatures. The spectrometer operates in ultra-high vacuum and…

We establish a testbed system for the development of high-sensitivity Electron Spin Resonance (ESR) techniques for small samples at cryogenic temperatures. Our system consists of a Niobium Nitride thin-film planar superconducting…

Electron spin resonance (ESR) is a powerful tool for characterizing and manipulating spin systems, but commercial ESR spectrometers can be expensive and designed to work in narrow frequency bands. This work presents an inexpensive…

Instrumentation and Detectors · Physics 2024-08-01 Charles A. Collett , Sofia M. Davvetas , Abdulelah Alsuhaymi , Grigore A. Timco

Counting the microwave photons emitted by an ensemble of electron spins when they relax radiatively has recently been proposed as a sensitive method for electron paramagnetic resonance (EPR) spectroscopy, enabled by the development of…

We performed magnetic field and frequency tunable electron paramagnetic resonance spectroscopy of an Er$^{3+}$ doped Y$_2$SiO$_5$ crystal by observing the change in flux induced on a direct current-superconducting quantum interference…

Electron paramagnetic resonance (EPR) spectroscopy is an important technology in physics, chemistry, materials science, and biology. Sensitive detection with a small sample volume is a key objective in these areas, because it is crucial,…

High-Field Electron Spin Resonance measurements were made on powder samples of Cu_{1-x}Zn_{x}GeO_{3} (x=0.00, 0.01, 0.02, 0.03 and 0.05) at different frequencies (95, 110, 190, 220, 330 and 440 GHz) at low temperatures. The spectra of the…

Strongly Correlated Electrons · Physics 2015-06-25 A. K. Hassan , L. A. Pardi , G. B. Martins , G. Cao , L-C. Brunel

Coherence times of electron spins bound to phosphorus donors have been measured, using a standard Hahn echo technique, to be up to 20 ms in isotopically pure silicon with [P]$ = 10^{14}$ cm$^{-3}$ and at temperatures $\leq 4 $K. Although…

Mesoscale and Nanoscale Physics · Physics 2020-12-29 Philipp Ross , Brendon C. Rose , Cheuk C. Lo , Mike L. W. Thewalt , Alexei M. Tyryshkin , Stephen A. Lyon , John J. L. Morton

We present a novel method that combines spin resonance spectroscopy with transmission electron microscopy (TEM), enabling localized in-situ detection of microwave (MW)-driven spin excitations. Our approach utilizes continuous wave MW…

Multi-frequency electron spin resonance (ESR) transmission spectra have been measured as function of temperature and magnetic field on single crystals of the quasi-one-dimensional spin-1 chain compound SrNi2V2O8 in the GHz frequency range.…

Strongly Correlated Electrons · Physics 2013-03-18 Zhe Wang , M. Schmidt , A. K. Bera , A. T. M. N. Islam , B. Lake , A. Loidl , J. Deisenhofer

The development of a new era of quantum devices requires an understanding of how paramagnetic dopants or impurity spins behave in crystal hosts. Here, we describe a new spectroscopic technique which uses traditional Electron Spin Resonance…

We report electron spin resonance (ESR) measurements on a large-area silicon MOSFET. An ESR signal at g-factor 1.9999(1), and with a linewidth of 0.6 G, is observed and found to arise from two-dimensional (2D) electrons at the Si/SiO2…

Materials Science · Physics 2009-12-20 S. Shankar , A. M. Tyryshkin , S. Avasthi , S. A. Lyon

Presented are magnetization measurements on a crystal of Fe8 single-molecule magnets using a Hall probe magnetometer. Irradiation with microwaves at frequencies of 92 and 110-120 GHz leads to the observation of electron paramagnetic…

Mesoscale and Nanoscale Physics · Physics 2007-05-23 K. Petukhov , W. Wernsdorfer , A. -L. Barra

Coherent spin resonance methods, such as nuclear magnetic resonance and electron spin resonance spectroscopy, have led to spectrally highly sensitive, non-invasive quantum imaging techniques. Here, we propose a pump-probe spin resonance…

Quantum Physics · Physics 2024-12-02 Philipp Haslinger , Stefan Nimmrichter , Dennis Rätzel

In this work, we demonstrate the use of frequency-tunable superconducting NbTiN coplanar waveguide microresonators for multi-frequency pulsed electron spin resonance (ESR) experiments. By applying a bias current to the center pin, the…

Quantum Physics · Physics 2017-07-19 A. T. Asfaw , A. J. Sigillito , A. M. Tyryshkin , T. Schenkel , S. A. Lyon

We demonstrate electron spin polarization detection and electron paramagnetic resonance (EPR) spectroscopy using a direct current superconducting quantum interference device (dc-SQUID) magnetometer. Our target electron spin ensemble is…

Mesoscale and Nanoscale Physics · Physics 2024-06-24 Hiraku Toida , Yuichiro Matsuzaki , Kosuke Kakuyanagi , Xiaobo Zhu , William J. Munro , Kae Nemoto , Hiroshi Yamaguchi , Shiro Saito

We combine top-down and bottom-up nanolithography to optimize the coupling of small molecular spin ensembles to $1.4$ GHz on-chip superconducting resonators. Nanoscopic constrictions, fabricated with a focused ion beam at the central…

We present the fabrication and measurement of a radio frequency single electron transistor (rf-SET), that displays a very high charge sensitivity of 1.9 microlectrons/sqrt(Hz) at 4.2 K. At 40 mK, the charge sensitivity is 0.9 and 1.0…

Mesoscale and Nanoscale Physics · Physics 2011-03-11 Henrik Brenning , Sergey Kafanov , Tim Duty , Sergey Kubatkin , Per Delsing

Magnetic resonance with ensembles of electron spins is nowadays performed in frequency ranges up to 240 GHz and in corresponding magnetic fields of up to 10 T. However, experiments with single electron and nuclear spins so far only reach…

Electron spin resonance with a scanning tunneling microscope (ESR-STM) combines the high energy resolution of spin resonance spectroscopy with the atomic scale control and spatial resolution of STM. Here we describe the upgrade of a…

Instrumentation and Detectors · Physics 2019-01-30 Fabian D. Natterer , François Patthey , Tobias Bilgeri , Patrick R. Forrester , Nicolas Weiss , Harald Brune