Related papers: Upper limit on nonlinear optical processes: shift …
Transition metal dichalcogenides (TMDCs) have demonstrated significant potential as versatile quantum materials for light absorption and emission. Their unique properties are primarily governed by exciton-photon interactions, which can be…
The scaling of the fundamental limits of the second hyperpolarizability is used to define the intrinsic second hyperpolarizability, which aids in identifying material classes with ultralarge nonlinear-optical response per unit of molecular…
We present a detailed theoretical investigation of the linear and non-linear optical response in a model system for a disordered d-wave superconductor, showing that for both quantities the gap symmetry considerably changes the paradigm of…
Terahertz high harmonic generation (THz HHG) is a common property of nonlinear systems. Recently it has been used to investigate fundamental principles that govern transport and nonlinear dynamics in novel quantum materials like graphene,…
Optical modulation of high-harmonics generation in solids enables the detection of material properties such as the band structure and promising new applications such as super-resolution imaging in semiconductors. Various recent studies have…
The existence of large nonlinear optical coefficients is one of the preconditions for using nonlinear optical materials in nonlinear optical devices. For a crystal, such large coefficients can be achieved by matching photon energies with…
Experimental insight into the elementary processes underlying charge transfer across interfaces has blossomed with the wide-spread availability of ultra-high vacuum set-ups that allow the preparation and characterization of solid surfaces…
We derive an expression for the effective second-harmonic coefficient of a dilute suspension of coated spherical particles. It is assumed that the coating material, but not the core or the host, has a nonlinear susceptibility for…
We conduct a theoretical and numerical study on the second-harmonic (SH) optical response of a nano-structured metamaterial composed of a periodic array of inclusions. Both the inclusions and their surrounding matrix are made of…
We experimentally demonstrate coherent control of the nonlinear response of optical second harmonic generation in resonant nanostructures beyond the weak-field regime. Contrary to common perception, we show that maximizing the intensity of…
The static second hyperpolarizability is derived from the space-fractional Schr\"{o}dinger equation in the particle-centric view. The Thomas-Reiche-Kuhn sum rule matrix elements and the three-level ansatz determines the maximum second…
We present a modeling of the nonlinear optical response of a metal surface in order to account for recent experimental results from two-color Sum-Frequency Generation experiments on gold. The model allows calculating the surface and bulk…
The Eulerian cosmological fluid equations are used to study the nonlinear mode coupling of density fluctuations. We evaluate the second-order power spectrum including all four-point contributions. In the weakly nonlinear regime we find that…
Second harmonic generation (SHG) is a coherent nonlinear phenomenon that plays an important role in laser color conversion. Lithium niobate (LN), which features both a large band gap and outstanding second-order nonlinearities, acts as an…
We develop a general theory of high-harmonic generation (HHG) in solid-state systems, based on a weak-correlation expansion of photonic and matter degrees of freedom. Unlike standard HHG theories, which treat light-matter dynamics through…
We develop an analytical framework to derive upper bounds to light--matter interactions in the optical near field, where applications ranging from spontaneous-emission amplification to greater-than-blackbody heat transfer show…
The generation of second and third harmonics by an acoustic wave propagating along one dimension in a weakly nonlinear elastic medium that is loaded harmonically in time with frequency $\omega_0$ at a single point in space, is analyzed by…
Monolayer transition-metal dichalcogenides (TMDCs) present high second-order optical nonlinearity, which is extremely desirable for, e.g., frequency conversion in nonlinear photonic devices. On the other hand, the atomic thickness of 2D…
High-harmonic generation (HHG), an extreme nonlinear effect, introduces an unprecedented paradigm to detect emergent quantum phases and electron dynamics inconceivable in the framework of linear and low-order nonlinear processes. As an…
The strong-field process of high-harmonic generation (HHG) has, in recent years, been treated from a quantum optical perspective in the emerging research area of strong-field quantum optics. These investigations show that HHG radiation is,…