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We use confocal microscopy to directly visualize the dynamics of aging colloidal glasses. We prepare a colloidal suspension at high density, a simple model system which shares many properties with other glasses, and initiate experiments by…

Disordered Systems and Neural Networks · Physics 2009-11-07 Rachel E. Courtland , Eric R. Weeks

We study aging in a colloidal suspension consisting of micron-sized particles in a liquid. This system is made glassy by increasing the particle concentration. We observe samples composed of particles of two sizes, with a size ratio of…

Soft Condensed Matter · Physics 2008-10-02 Jennifer M. Lynch , Gianguido C. Cianci , Eric R. Weeks

We study bidisperse colloidal suspensions confined within glass microcapillary tubes to model the glass transition in confined cylindrical geometries. We use high speed three-dimensional confocal microscopy to observe particle motions for a…

Soft Condensed Matter · Physics 2013-02-28 Nabiha Saklayen , Gary L. Hunter , Kazem V. Edmond , Eric R. Weeks

In this paper we analyze the changes in the microscopic dynamics of a colloidal glass submitted to an oscillatory shear. We use Multispeckle diffusing Wave Spectroscopy to monitor the transient dynamical regimes following a shear…

Soft Condensed Matter · Physics 2007-05-23 Virgile Viasnoff , Francois Lequeux

We study concentrated colloidal suspensions, a model system which has a glass transition. Samples in the glassy state show aging, in that the motion of the colloidal particles slows as the sample ages from an initial state. We study the…

Soft Condensed Matter · Physics 2007-05-23 Gianguido C. Cianci , Rachel E. Courtland , Eric R. Weeks

We study confined colloidal suspensions as a model system which approximates the behavior of confined small molecule glass-formers. Dense colloidal suspensions become glassier when confined between parallel glass plates. We use confocal…

Soft Condensed Matter · Physics 2015-03-13 Kazem V. Edmond , Carolyn R. Nugent , Eric R. Weeks

The dynamics of a glass-forming material slow greatly near the glass transition, and molecular motion becomes inhibited. We use confocal microscopy to investigate the motion of colloidal particles near the colloidal glass transition. As the…

Disordered Systems and Neural Networks · Physics 2009-11-07 Eric R. Weeks , D. A. Weitz

Aging in an attraction-driven colloidal glass is studied by computer simulations. The system is equilibrated without attraction and instantaneously ``quenched'', at constant colloid volume fraction, to one of two states beyond the glass…

Soft Condensed Matter · Physics 2015-06-25 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

We study the aging dynamics in a model for dense simple liquids, in which particles interact through a hard-core repulsion complemented by a short-ranged attractive potential, of the kind found in colloidal suspensions. In this system, at…

Statistical Mechanics · Physics 2007-05-23 G. Foffi , E. Zaccarelli , S. Buldyrev , F. Sciortino , P. Tartaglia

We study concentrated colloidal suspensions, a model system which has a glass transition. The non-equilibrium nature of the glassy state is most clearly highlighted by aging -- the dependence of the system's properties on the time elapsed…

Soft Condensed Matter · Physics 2007-05-23 Gianguido C. Cianci , Rachel E. Courtland , Eric R. Weeks

We use confocal microscopy and time-resolved light scattering to investigate plasticity in a col- loidal polycrystal, following the evolution of the network of grain boundaries as the sample is submitted to thousands of shear deformation…

Soft Condensed Matter · Physics 2014-08-28 Elisa Tamborini , Luca Cipelletti , Laurence Ramos

We investigate experimentally and theoretically thin layers of colloid particles held adjacent to a solid substrate by gravity. Epifluorescence, confocal, and holographic microscopy, combined with Monte Carlo and hydrodynamic simulations,…

Vapour deposition can directly produce ultrastable glasses, which are similar to conventional glasses aged over thousands of years. The highly mobile surface layer is believed to accelerate the ageing process of vapour-deposited glasses,…

Soft Condensed Matter · Physics 2016-10-20 Xin Cao , Huijun Zhang , Yilong Han

It is well established that physical aging of amorphous solids is governed by a marked change in dynamical properties as the material becomes older. Conversely, structural properties such as the radial distribution function exhibit only a…

Despite their technological relevance, a full microscopic understanding of glasses is still lacking. This applies even more to their surfaces whose properties largely differ from that of the bulk material. Here, we experimentally…

Soft Condensed Matter · Physics 2022-11-23 Li Tian , Clemens Bechinger

We use colloidal suspensions encapsulated in emulsion droplets to model confined glass-forming liquids with tunable boundary mobility. We show dynamics in these idealized systems are governed by physical interactions with the boundary.…

Soft Condensed Matter · Physics 2014-05-29 Gary L. Hunter , Kazem V. Edmond , Eric R. Weeks

We study colloidal particle dynamics of a model glass system using confocal and fluorescence microscopy as the sample evolves from a hard-sphere glass to a liquid with attractive interparticle interactions. The transition from hard-sphere…

Soft Condensed Matter · Physics 2015-05-13 Andrzej Latka , Yilong Han , Ahmed M. Alsayed , Andrew B. Schofield , A. G. Yodh , Piotr Habdas

Using fast confocal microscopy we image the three-dimensional dynamics of particles in a yielded hard-sphere colloidal glass under steady shear. The structural relaxation, observed in regions with uniform shear, is nearly isotropic but is…

Soft Condensed Matter · Physics 2009-11-11 R. Besseling , Eric R. Weeks , A. B. Schofield , W. C. K. Poon

The coupling of active, self-motile particles to topological constraints can give rise to novel non-equilibrium dynamical patterns that lack any passive counterpart. Here we study the behavior of self-propelled rods confined to a compact…

Statistical Mechanics · Physics 2018-08-21 Liesbeth M. C. Janssen , Andreas Kaiser , Hartmut Löwen

We present here a microscopic study of the effect of shear on a dense purely repulsive colloidal suspension. We use Multispeckle Diffusing Wave Spectroscopy to monitor the transient motions of colloidal particles after being submitted to an…

Soft Condensed Matter · Physics 2007-05-23 V. Viasnoff , S. Jurine , F. Lequeux
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