English
Related papers

Related papers: Orienting Asymmetric Molecules by Laser Fields wit…

200 papers

Twisted atomic bilayers are emerging platforms for manipulating chiral light-matter interaction at the extreme nanoscale, due to their inherent magnetoelectric responses induced by the finite twist angle and quantum interlayer coupling…

Optics · Physics 2021-05-19 Xinyan Zhang , Yuhan Zhong , Tony Low , Hongsheng Chen , Xiao Lin

The measurements of the linear polarisation of visible light from quasars give strong evidence for large-scale coherent orientations of their polarisation vectors in some regions of the sky. We show that these observations can be explained…

Cosmology and Nongalactic Astrophysics · Physics 2009-11-04 A. Payez , J. R. Cudell , D. Hutsemékers

Chiral circularly polarized (CP) light is central to many photonic technologies, from optical communication of spin information to novel display and imaging technologies. As such, there has been significant effort in the development of…

Materials Science · Physics 2023-07-25 Li Wan , Yizhou Liu , Matthew J. Fuchter , Binghai Yan

A relativistic electron-positron beam propagating through a magnetized electron-ion plasma is shown to generate both circularly and linearly polarized synchrotron radiation. The degrees of circular and linear polarizations depend both on…

Plasma Physics · Physics 2019-05-29 Ujjwal Sinha , Christoph H. Keitel , Naveen Kumar

Light-induced rotation of absorbing microscopic particles by transfer of angular momentum from light to the material raises the possibility of optically driven micromachines. The phenomenon has been observed using elliptically polarized…

The strong coupling between intense laser fields and valence electrons in molecules causes a distortion of the potential energy hypersurfaces which determine the motion of nuclei in a molecule and influences possible reaction pathways. The…

Laser pulses are known to induce symmetric demagnetization: equal loss of magnetic moments in the identical sublattices of antiferromagnets and ferromagnets at ultrashort timescales. Using time-dependent density functional theory, we show…

Materials Science · Physics 2026-02-19 Zhaobo Zhou , Sangeeta Sharma , John Kay Dewhurst , Junjie He

We present a novel approach to model ultrafast time-dependent nonlinear optical polarization sensitive signals emitted from randomly-oriented molecules. By projecting the laboratory-frame analyzer polarization axis into the molecular frame…

Chemical Physics · Physics 2025-07-17 R. L. Thurston , N. Shivaram , Th. Weber , L. Z. Tan , D. S. Slaughter

We consider laser alignment of ortho and para spin isomers of water molecules by using strong and short off-resonance laser pulses. A single pulse is found to create a distinct transient alignment and antialignment of the isomeric species.…

Quantum Physics · Physics 2009-11-13 E. Gershnabel , I. Sh. Averbukh

We present a theoretical study of recent laser-alignment and mixed-field-orientation experiments of asymmetric top molecules. In these experiments, pendular states were created using linearly polarized strong ac electric fields from pulsed…

We report the observation of macroscopic field-free orientation, i.e. more than 73 % of CO molecules pointing in the same direction. This is achieved through an all-optical scheme operating at high particle densities ($>10^{17}$cm$^{-3}$)…

Chemical Physics · Physics 2014-07-09 P. M. Kraus , D. Baykusheva , H. J. Wörner

Study on a rectified current induced by active particles has received a great attention due to its possible application to a microscopic motor in biological environments. Insertion of an {\em asymmetric} passive object amid many active…

Soft Condensed Matter · Physics 2021-11-19 Jae Sung Lee , Jong-Min Park , Jae Dong Noh , Hyunggyu Park

Circularly polarized colliding laser pulses can create abundant electron-positron pair plasma [A. R. Bell and J. G. Kirk, Phys. Rev. Lett. 101, 200403 (2008)], which scattering the incoming electromagnetic waves can prevent them from…

Precision searches for time-reversal symmetry violating interactions in polar molecules are extremely sensitive probes of high energy physics beyond the Standard Model. To extend the reach of these probes into the PeV regime, long coherence…

Atomic Physics · Physics 2017-10-03 Ivan Kozyryev , Nicholas R. Hutzler

Achiral molecules can be made temporarily chiral by excitation with electric fields, in the sense that an average over molecular orientations displays a net chiral signal [Tikhonov et al., Sci. Adv. 8, eade0311 (2022)]. Here, we go beyond…

We consider injection and subsequent acceleration of electrons in narrow plasma channels irradiated by linearly and radially polarized ultraintense laser pulses. Using three-dimensional particle-in-cell simulations, we show that radially…

Structured x-rays carrying an orbital angular momentum break spatial inversion symmetry and have been proposed as a means to probe chirality. We theoretically investigate twisted non-resonant x-ray diffraction from chiral molecules and…

Optics · Physics 2026-03-02 Akilesh Venkatesh , Phay J. Ho , Jérémy R. Rouxel

We show that it is possible to generate continuous-wave fields and pulses of polarization squeezed light by sending classical, linearly polarized laser light twice through an atomic sample which causes an optical Faraday rotation of the…

Quantum Physics · Physics 2011-10-13 Jacob F. Sherson , Klaus Molmer

Ionization and excitation of water molecules in intense laser pulses is studied theoretically by solving the three-dimensional time-dependent electronic Schr\"odinger equation within the single-active-electron approximation. The possibility…

Atomic Physics · Physics 2011-12-13 Simon Petretti , Alejandro Saenz , Alberto Castro , Piero Decleva

The alignment of permanent dipole moments and the resulting spontaneous orientation polarization (SOP) is commonly observed in evaporated neat films of polar organic molecules and leads to a so-called giant surface potential. In case of…

Materials Science · Physics 2025-05-01 Alexander Hofmann , Albin Cakaj , Lea Kolb , Yutaka Noguchi , Wolfgang Brütting