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Chirality is ubiquitous in nature and fundamental in science, from particle physics to metamaterials.The most established technique of chiral discrimination - photoabsorption circular dichroism - relies on the magnetic properties of a…

To date, optical orientation of free-carrier spins and spin currents have been achieved by circularly polarized light, while the linearly polarized light has been used for optical alignment of electron momenta. Here we show that, in…

Mesoscale and Nanoscale Physics · Physics 2009-11-11 S. A. Tarasenko , E. L. Ivchenko

Left and right circularly polarized transverse electromagnetic waves propagate at slightly different speeds in a magnetic material leading to a polarization rotation by an amount proportional to the projection of the magnetic field along…

Optics · Physics 2025-01-30 Koray Koksal , Fatma Tambag , Jamal Berakdar , Mohamed Babiker

Since its invention in 1999, optical centrifuge has become a powerful tool for controlling molecular rotation and studying molecular dynamics and molecular properties at extreme levels of rotational excitation. The technique has been…

Instrumentation and Detectors · Physics 2020-05-20 Ian MacPhail-Bartley , Walter W. Wasserman , Alexander A. Milner , V. Milner

We analyze the alignment of molecules generated by a pair of crossed ultra-short pump pulses of different polarizations by a technique based on the induced time-dependent gratings. Parallel polarizations yield an intensity grating, while…

Quantum Physics · Physics 2009-11-13 Arnaud Rouzee , Vincent Renard , Stephane Guerin , Olivier Faucher , Bruno Lavorel

We show how a medium, under the influece of a coherent control field which is resonant or close to resonance to an appropriate atomic transition, can lead to very strong asymmetries in the propagation of unpolarized light when the direction…

Quantum Physics · Physics 2009-11-07 G. S. Agarwal , Shubhrangshu Dasgupta

Coherent, optically dressed media composed of two-level molecular systems without inversion symmetry are considered as all-optically tunable sources of coherent radiation in the microwave domain. A theoretical model and a numerical toolbox…

Quantum Physics · Physics 2020-12-08 Piotr Gładysz , Piotr Wcisło , Karolina Słowik

An axisymmetric fully ionized plasma rotates around its axis when a charge separation between magnetic surfaces is produced from DC fields or RF waves. On each magnetic surface both electrons and ions obey the isorotation law and perform an…

Plasma Physics · Physics 2019-01-30 J. M. Rax , E. J. Kolmes , I. E. Ochs , N. J. Fisch , R. Gueroult

Asymmetric molecules look different when viewed from one side or the other. This difference influences the electronic structure of the valence electrons, thereby giving stereo sensitivity to chemistry and biology. We show that attosecond…

Intense single-cycle THz pulses resonantly interacting with molecular rotations are shown to induce significant field-free orientation under ambient conditions. We calculate and measure the angular distribution associated with THz-driven…

Chemical Physics · Physics 2015-05-28 Sharly Fleischer , Yan Zhou , Robert W. Field , Keith A. Nelson

It is demonstrated that strong laser pulses can introduce torsional motion in the axially chiral molecule 3,5-diflouro-3',5'-dibromo-biphenyl (DFDBrBPh). A nanosecond laser pulse spatially aligns the stereogenic carbon-carbon (C-C) bond…

We investigate the orientation dependence of high-order harmonic generation (HHG) from H$_2^+$ with different internuclear distances irradiated by intense laser fields both numerically and analytically. The calculated molecular HHG spectra…

Atomic Physics · Physics 2009-11-13 Yanjun Chen , Jie Liu , Bambi Hu

We solve the three-dimensional time-dependent Schr\"{o}dinger equation for a few-cycle circularly polarized femtosecond laser pulse interacting with an oriented target exemplified by an Argon atom, initially in a $3\text{p}_{x}$ or…

Atomic Physics · Physics 2015-05-18 C. P. J. Martiny , M. Abu-samha , L. B. Madsen

Precise magnetometry is vital in numerous scientific and technological applications. At the forefront of sensitivity, optical atomic magnetometry, particularly techniques utilizing nonlinear magneto-optical rotation (NMOR), enables…

Optics · Physics 2024-12-31 S. Pustelny , P. Włodarczyk

For a long time transverse and longitudinal optical forces are used for non-contact and noninvasive manipulation of small individual particles. The following question arises: What is the impact of these forces on the ensemble of thousand…

Optics · Physics 2021-05-26 Lubomir Kovachev

We introduce a new optical tool - a "two-dimensional optical centrifuge", capable of aligning molecules in extreme rotational states. Unlike the conventional centrifuge, which confines the molecules in the plane of their rotation, its…

Chemical Physics · Physics 2016-05-18 A. A. Milner , A. Korobenko , V. Milner

We show that the optical force exerted on a finite size chiral sphere by a surface plasmon mode has a component along a direction perpendicular to the plasmon linear momentum. We reveal how this chiral lateral force, pointing in opposite…

Optics · Physics 2016-01-20 Antoine Canaguier-Durand , Cyriaque Genet

The generation of ultrashort pulses hinges on the careful management of dispersion. Traditionally, this has exclusively involved second-order dispersion, while higher-order dispersion was treated as a nuisance to be minimized. Here we show…

The yield of strong-field ionization, by a linearly polarized probe pulse, is studied experimentally and theoretically, as a function of the relative orientation between the laser field and the molecule. Experimentally, carbonyl sulfide,…

We have investigated non-dipole effects in the interaction of a hydrogen atom with elliptically polarized laser pulses of intensity 10$^{14}$ W/cm$^2$ with about 8 fs duration. The study was performed within the framework of a hybrid…

Atomic Physics · Physics 2025-09-03 Vladimir S. Melezhik , Sara Shadmehri
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