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We report the synthesis, structure, and magnetic and transport properties of a new ternary intermetallic compound PrRhSn3 which crystallizes in LaRuSn3-type cubic structure (space group Pm-3n). At low applied fields the dc magnetic…

Strongly Correlated Electrons · Physics 2014-07-22 V. K. Anand , D. T. Adroja , A. D. Hillier

We report the results of dc and ac magnetization measurements as a function of temperature (1.8 - 300 K) for the spin chain compound, Ca$_3$CoRhO$_6$, which has been recently reported to exhibit a partially disordered antiferromagnetic…

Strongly Correlated Electrons · Physics 2009-11-07 E. V. Sampathkumaran , Asad Niazi

We present high-resolution single crystal time-of-flight neutron scattering measurements on the candidate quantum spin liquid pyrochlore Tb2Ti2O7 at low temperature and in a magnetic field. At ~70 mK and in zero field, Tb2Ti2O7 reveals…

Strongly Correlated Electrons · Physics 2013-04-16 K. Fritsch , K. A. Ross , Y. Qiu , J. R. D. Copley , T. Guidi , R. I. Bewley , H. A. Dabkowska , B. D. Gaulin

We report on the muon spin rotation/relaxation study of a pyrochlore oxide, Cd2Os2O7, which exhibits a metal-insulator (MI) transition at T_{MI}~225 K without structural phase transition. It reveals strong spin fluctuation (>10^8/s) below…

Strongly Correlated Electrons · Physics 2009-11-13 A. Koda , R. Kadono , K. Ohishi , S. R. Saha , W. Higemoto , S. Yonezawa , Y. Muraoka , Z. Hiroi

Paramagnetic ions in solid state crystals form the basis for many advanced technologies such as lasers, masers, frequency standards, and quantum-enhanced sensors. One of the most-studied examples is the Cr3+ ion in sapphire (Al2O3), also…

Mesoscale and Nanoscale Physics · Physics 2020-10-07 Vikas K. Sewani , Rainer J. Stöhr , Roman Kolesov , Hyma H. Vallabhapurapu , Tobias Simmet , Andrea Morello , Arne Laucht

Intensity distribution of the neutron magnetic scattering has been taken in the reciprocal space of a single crystal of the "spin ice" system Ho2Ti2O7 at the elastic energy position in the temperature (T) region between 0.4 K and 50 K. The…

Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of…

Strongly Correlated Electrons · Physics 2012-09-28 P. Dalmas de Reotier , A. Yaouanc , Y. Chapuis , S. H. Curnoe , B. Grenier , E. Ressouche , C. Marin , J. Lago , C. Baines , S. R. Giblin

X-ray absorption spectroscopy (XAS) as well as x-ray magnetic circular dichroism (XMCD) and magnetization of hybrid pyrochlore Eu2-xFexTi2O7 were investigated, where the rare earth Eu (4f) was replaced with transition metal Fe (3d) to…

We report high resolution single crystal x-ray diffraction measurements of the frustrated pyrochlore magnet Tb2Ti2O7, collected using a novel low temperature pulsed magnet system. This instrument allows characterization of structural…

Strongly Correlated Electrons · Physics 2012-07-16 J. P. C. Ruff , Z. Islam , J. P. Clancy , K. A. Ross , H. Nojiri , Y. H. Matsuda , H. A. Dabkowska , A. D. Dabkowski , B. D. Gaulin

The low-temperature thermodynamic properties of the frustrated pyrochlore Tb$_{2+x}$Ti$_{2-x}$O$_{7+y}$ have been studied using the single crystal of $x=0.005$ sitting in a long range ordered phase in the $x$-$T$ phase diagram. We observed…

Strongly Correlated Electrons · Physics 2017-04-25 H. Takatsu , T. Taniguchi , S. Kittaka , T. Sakakibara , H. Kadowaki

Crystal structure, thermal and magnetic properties were systematically studied in the Y$_{1-x}$Pr$_x$CrO$_3$ with $0 \leq x \leq 0.3$ compositions. Magnetic susceptibility and specific heat measurements show an increase of the…

Materials Science · Physics 2018-02-08 A. Durán , R. Escamilla , R. Escudero , F. Morales , E. Verdín

EuTiO_3 is shown to exhibit novel strong spin-charge-lattice coupling deep in the paramagnetic phase. Its existence is evidenced by an, until now, unknown response of the paramagnetic susceptibility at temperatures exceeding the structural…

Materials Science · Physics 2013-09-18 K. Caslin , R. K. Kremer , Z. Guguchia , H. Keller , J. Köhler , A. Bussmann-Holder

The magnetic properties of polycrystaline La0.5Ba0.5CoO2.5+d (d = 0.44 and 0.485) where investigated using muon spin relaxation and bulk magnetization experiments. Below a Curie temperature of T_C = 160 K and 180 K, respectively, a magnetic…

Strongly Correlated Electrons · Physics 2011-11-23 M. Stingaciu , H. Luetkens , Y. G. Pashkevich , E. Pomjakushina , K. Conder , H. -H. Klauss

Spin ices, frustrated magnetic materials analogous to common water ice, are exemplars of high frustration in three dimensions. Recent experimental studies of the low-temperature properties of the paradigmatic Dy$_2$Ti$_2$O$_7$ spin ice…

Statistical Mechanics · Physics 2016-01-19 P. Henelius , T. Lin , M. Enjalran , Z. Hao , J. G. Rau , J. Altosaar , F. Flicker , T. Yavors'kii , M. J. P. Gingras

Neutron scattering has been used to study the magnetic order and spin dynamics of the colossal magnetoresistive pyrochlore Tl_2Mn_2O_7. On cooling from the paramagnetic state, magnetic correlations develop and appear to diverge at T_C (123…

Strongly Correlated Electrons · Physics 2009-10-31 J. W. Lynn , L. Vasiliu-Doloc , M. A. Subramanian

Cobalt pyrochlore fluoride NaCaCo$_2$F$_7$ is a disordered frustrated magnet composed of Co$^{2+}$ ions with an effective spin-$\frac{1}{2}$ magnetic moment and exhibits spin freezing below $T_f \sim$2.4 K. We perform ultrasound velocity…

Strongly Correlated Electrons · Physics 2020-06-17 T. Watanabe , H. Kato , Y. Hara , J. W. Krizan , R. J. Cava

The insulating pyrochlore compound Nd2Sn2O7 has been shown to undergo a second order magnetic phase transition at Tc ~ 0.91 K to a noncoplanar all-in--all-out magnetic structure of the Nd3+ magnetic moments. An anomalously slow paramagnetic…

Strongly Correlated Electrons · Physics 2017-05-04 P. Dalmas de Reotier , A. Yaouanc , A. Maisuradze , A. Bertin , P. J. Baker , A. D. Hillier , A. Forget

The "spin ice" state found in the rare earth pyrochlore magnets Ho2Ti2O7 and Dy2Ti2O7 offers a beautiful realisation of classical magnetostatics, complete with magnetic monopole excitations. It has been suggested that in "quantum spin ice"…

Strongly Correlated Electrons · Physics 2015-06-04 Owen Benton , Olga Sikora , Nic Shannon

The spin-glass behavior in the ferromagnetic phase of $\mathrm{Tm_2Cu_2In}$ was investigated by dc-, ac-magnetization, and non-equilibrium dynamics characterizations. Arc-melted polycrystalline compound of $\mathrm{Tm_2Cu_2In}$ crystallizes…

Materials Science · Physics 2021-11-10 Baidyanath Sahu , R. Djoumessi Fobasso , Andre M. Strydom

We report the properties of a triangular lattice iron-chalcogenide antiferromagnet FeAl$_{2}$Se$_{4}$. The spin susceptibility reveals a significant antiferromagnetic interaction with a Curie-Weiss temperature {\Theta}$_{CW}$ ~ -200K and a…

Strongly Correlated Electrons · Physics 2019-02-27 Kunkun Li , Shifeng Jin , Jiangang Guo , Yanping Xu , Yixi Su , Erxi Feng , Yu Liu , Shengqiang Zhou , Tianping Ying , Shiyan Li , Ziqiang Wang , Gang Chen , Xiaolong Chen
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