Related papers: Extracting spectroscopic molecular parameters from…
Controlling the wave function of free electrons is important to improve the spatial resolution of electron microscopes, the efficiency of electron interaction with sample modes of interest, and our ability to probe ultrafast materials…
For the first time, a global model of electromagnetic pulse (EMP) emission connects charge separation in the laser target to quantitative measurements of the electromagnetic field. We present a frequency-domain dipole antenna model which…
We study the fundamental limits of the precision of estimating parameters of a quantum matter system when it is probed by a travelling pulse of quantum light. In particular, we focus on the estimation of the interaction strength between the…
We investigate attosecond time delays in the emission of photoelectrons using a hierarchy of models of the $CO_2$ molecule including the strong field approximation, Coulomb-scattering, short-range parts of the molecular potential, Hartree…
In this work we present a hypothesis that spectral response of atoms or molecules to a pulse of electromagnetic radiation with fast rising or falling fronts would contain a unique emission line that is located approximately near the…
The toolbox for time-resolved direct measurements of electron dynamics covers a variety of methods. Since the experimental effort is increasing rapidly with achievable time resolution, there is an urge for simple and robust measurement…
Sub-angstrom spatial resolution of electron density coupled with sub-femtosecond temporal resolution is required to directly observe the dynamics of the electronic structure of a molecule after photoinitiation or some other ultrafast…
The dynamics of atomic levels resonantly coupled by a coherent and intense short high-frequency laser pulse is discussed and it is advocated that this dynamics is sensitively probed by measuring the spectra of the particles emitted. It is…
In attosecond streaking, an electron is released by a short xuv pulse into a strong near infrared laser field. When the laser coupling between two states in the target is weak relative to the detuning, the streaking technique, which allows…
We consider the theory of the non-linear spectroscopy for a single molecule undergoing stochastic dynamics and interacting with a sequence of two laser pulses. General expressions for photon counting statistics are obtained, and an exact…
The correlated behavior of electrons determines the structure and optical properties of molecules, semiconductor and other systems. Valuable information on these correlations is provided by measuring the response to femtosecond laser…
A two level model of a single molecule undergoing spectral diffusion dynamics and interacting with a sequence of two short laser pulses is investigated. Analytical solution for the probability of n=0,1,2 photon emission events for the…
We propose the scheme of temporal double-slit interferometer to precisely measure the electric field of shaped intense femtosecond laser pulse directly, and apply it to control the electron tunneling wave packets in attosecond precision. By…
Imaging the quantum motion of electrons not only in real-time, but also in real-space is essential to understand for example bond breaking and formation in molecules, and charge migration in peptides and biological systems. Time-resolved…
Quantum theory of self-phase and cross-phase modulation of ultrashort light pulses in the Kerr medium is developed with taking into account the response time of an electronic nonlinearity. The correspondent algebra of time-dependent…
An all non-optical method for accurately determining the pulse parameters of individual few-cycle laser shots is presented. By analyzing the "left" and "right" asymmetry of high-energy photoelectrons along the polarization axis using the…
We present a time dependent quantum calculation of the scattering of a few-photon pulse on a single atom. The photon wave packet is assumed to propagate in a transversely strongly confined geometry, which ensures strong atom-light coupling…
Images of electron flow through a two-dimensional electron gas from a quantum point contact (QPC) can be obtained at liquid He temperatures using scanning probe microscopy (SPM). A negatively charged SPM tip depletes the electron gas…
A stochastic cumulant GW method is presented, allowing us to map the evolution of photoemission spectra, quasiparticle energies, lifetimes and emergence of collective excitations from molecules to bulk-like systems with up to thousands of…
Modelling the emission properties of compact high energy sources such as X-ray binaries, AGN or gamma-ray bursts represents a complex problem. Contributions of numerous processes participate non linearly to produce the observed spectra:…