Related papers: Extracting spectroscopic molecular parameters from…
Proposals to determine biomolecular structures from diffraction experiments using femtosecond X-ray free-electron laser (XFEL) pulses involve a conflict between the incident brightness required to achieve diffraction-limited atomic…
Based on the work done by an electromagnetic field on an atomic or molecular electronic system, a general gauge invariant formulation of transient absorption spectroscopy is presented within the semi-classical approximation. Avoiding…
As demonstrated in our previous work [J. Chem. Phys. 149, 174109 (2018)], the kinetic energy imparted to a quantum rotor by a non-resonant electromagnetic pulse with a Gaussian temporal profile exhibits quasi-periodic drops as a function of…
Photoelectron angular distributions of the two-photon ionization of neutral atoms are theoretically investigated. Numerical calculations of two-photon ionization cross sections and asymmetry parameters are carried out within the…
The operation of photoemission electron sources with wavelengths near the photoemission threshold has been shown to dramatically decrease the minimum achievable photocathode emittance, but at the cost of significantly reduced quantum…
The build-up dynamics of a continuous spectrum under the action of a weak laser field on a Fano resonance with the use of the pulses with the Lorentz spectrum and ultrashort pulses in the wavelet form is investigated. A dispersion-time…
The time-dependent Schr\"{o}dinger equation for the hydrogen atom and its interaction with coherent intense high-frequency short laser pulses is solved numerically exactly by propagating the single-electron wave packets. Thereby, the…
Quantum emitters promise to emit exactly one photon with high probability when pumped by a laser pulse. However, even in ideal systems, re-excitation during a laser pulse causes the consecutive emission of two photons, thus limiting the…
We theoretically investigate the scattering of an attosecond electron wave packet launched by an attosecond pulse under the influence of an infrared laser field. As the electron scatters inside a spatially extended system, the dressing…
We predict a significant delay of two-electron photoemission from the helium atom after absorption of an attosecond XUV pulse. We establish this delay by solving the time dependent Schr\"odinger equation and by subsequent tracing the…
In this work, we study the electromagnetic energy and energy rate spectra produced by a point particle in the presence of plane wave fields. Our approach is based on a semiclassical formulation, in which the current distribution that…
The electron-cyclotron maser instability is widespread in the Universe, producing, e.g., radio emission of the magnetized planets and cool substellar objects. Diagnosing the parameters of astrophysical radio sources requires comprehensive…
The electron localization in the dissociation of the asymmetric charged molecular ion HeH$^{2+}$ exposed to an intense few-cycle laser pulse is studied by solving numerically the 3D time-dependent Schr\"odinger equation. By varying the…
The temporal dynamics of double ionization of H2 has been investigated both experimentally and theoretically with few-cycle laser pulses. The main observables are the proton spectra associated to the H^+ + H^+ fragmentation channel. The…
Focused laser fields with textured polarization on a sub-wavelength scale allow extracting information on electronic processes which are not directly accessible by homogeneous fields. Here, we consider photoionization in radially and…
A dc electron gun, generating picosecond pulses with up to $8\times10^{6}$ electrons per pulse, was developed. Its applicability for future time-resolved-diffraction experiments on state- and conformer-selected laser-aligned or oriented…
We calculated third order non-linear polarization to estimate the two-photon absorption of non-interacting two-level molecules in the transmission-type degenerate pump-probe geometry. The spectral intensity and the phase changes of the…
We have implemented a new approach for measuring the time-dependent intensity and phase of ultrashort optical pulses. It is based on the interaction between shaped pulses and atoms, leading to coherent transients.
Using time dependent density functional theory (TDDFT) we examine the energy, angular and time-resolved photoelectron spectra (TRPES) of ethylene in a pump-probe setup. To simulate TRPES we expose ethylene to an ultraviolet (UV) femtosecond…
Based on new obtained analytical results, the main properties of photon echo quantum memory protocols are analysed and discussed together with recently achieved experimental results. The main attention is paid to studying the influence of…