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Laser-assisted photoemission from a solid is considered within a numerically exactly solvable one-dimensional model of a crystal. The effect of the inelastic scattering and of the finite duration of the pump pulse on the photoelectron…

Materials Science · Physics 2015-06-10 E. E. Krasovskii , C. Friedrich , W. Schattke , P. M. Echenique

We present the extension of the time-dependent configuration interaction singles (TDCIS) method to the computation of the electron kinetic-energy spectrum in photoionization processes. Especially for strong and long ionizing light pulses…

Atomic Physics · Physics 2014-04-17 Antonia Karamatskou , Stefan Pabst , Yi-Jen Chen , Robin Santra

We introduce and experimentally demonstrate a method, where the two intrinsic time scales of a molecule, the slow nuclear motion and the fast electronic motion, are simultaneously measured in a photo-electron photo-ion coincidence…

Through examining the product of the mathematical variance of intensity with respect to time and frequency, we arrive at a temporal characterization of laser pulses through parameters for pulse duration, group delay dispersion and temporal…

Multiphoton ionization of sodium by laser pulses of 800 nm wavelength and 57 fs duration is studied in the range of laser peak intensities belonging to over-the-barrier ionization regime. Photoelectron momentum distributions (PMD) and the…

Atomic Physics · Physics 2019-03-21 Andrej Bunac , Duška B. Popović , Nenad S. Simonović

Time-resolved investigations of ultrafast electronic and molecular dynamics were not possible until recently. The typical time scale of these processes is in the picosecond to attosecond realm. The tremendous technological progress in…

Atomic Physics · Physics 2013-05-14 Stefan Pabst

Realistic attosecond wave packets have complex profiles that, in dispersive conditions, rapidly broaden or split into multiple components. Such behaviors are encoded in sharp features of the wave packet spectral phase. Here, we exploit the…

Energy spectra and angular distributions have been measured of electrons that are emitted upon disassembly of $Xe_{150000}$ following irradiation by intense (10$^{15}-10^{16}$ W cm$^{-2}$) laser pulses whose durations are varied over the…

Atomic and Molecular Clusters · Physics 2009-11-07 V. Kumarappan , M. Krishnamurthy , D. Mathur

Optical pulses are routinely used to drive dynamical changes in the properties of solids. In quantum materials, many new phenomena have been discovered, including ultrafast transitions between electronic phases, switching of ferroic orders…

Strongly Correlated Electrons · Physics 2018-05-08 Michele Buzzi , Michael Först , Roman Mankowsky , Andrea Cavalleri

Streaking of photoelectrons has long been used for the temporal characterization of attosecond extreme ultraviolet pulses. When the time-resolved photoelectrons originate from a coherent superposition of electronic states, they carry an…

Chemical Physics · Physics 2016-07-27 Markus Kowalewski , Kochise Bennett , Jérémy R. Rouxel , Shaul Mukamel

The reflection, transmission and absorption of a symmetric electromagnetic pulse, which carrying frequency is close to the frequency of an interband transition in a QW (QW), are obtained. The energy levels of a QW are assumed discrete, one…

Mesoscale and Nanoscale Physics · Physics 2009-11-07 L. I. Korovin , I. G. Lang , D. A. Contreras-Solorio , S. T. Pavlov

Spectra of Thomson and Compton radiation, emitted during electron scattering off an intense laser beam, are calculated using the frameworks of classical and strong-field quantum electrodynamics, respectively. Both approaches use a…

Atomic Physics · Physics 2013-11-22 M Twardy , K Krajewska , J Z Kamiński

We describe a realistic model for a focused high-intensity laser pulse in three dimensions. Relativistic dynamics of an electron submitted to such pulse is described by equations of motion with ponderomotive potential depending on a single…

Quantum Physics · Physics 2009-11-07 N. B. Narozhny , M. S. Fofanov

We examine x-ray scattering from an isolated organic molecule from the linear to nonlinear absorptiveregime. In the nonlinear regime, we explore the importance of both the elastic and inelastic channelsand observe the onset of nonlinear…

Chemical Physics · Physics 2021-06-09 Phay J. Ho , Adam E. A. Fouda , Kai Li , Gilles Doumy , Linda Young

We study the emission spectrum and absorption spectrum of a quantum emitter when it is driven by various pulse sequences. We consider the Uhrig sequence of $\pi_x$ pulses, the periodic sequence of $\pi_x\pi_y$ pulses and the periodic…

Quantum Physics · Physics 2018-04-25 Herbert F Fotso

In ultrafast experiments with gas phase molecules, the alignment of the molecular axis relative to the polarization of the interacting laser pulses plays a crucial role in determining the dynamics following this light-matter interaction.…

Chemical Physics · Physics 2025-04-14 Shashank Kumar , Eric Liu , Liang Z. Tan , Varun Makhija , Niranjan Shivaram

The equations of motion of charged particles under the influence of short electromagnetic pulses are investigated. The subcycle regime is considered, and the delta function approximation is applied. The effects of the self force are also…

Optics · Physics 2007-05-23 Richard T Hammond

The dissociation spectrum of the hydrogen molecular ion by short intense pulses of infrared light is calculated. The time-dependent Schr\"odinger equation is discretized and integrated in position and momentum space. For few-cycle pulses…

Atomic Physics · Physics 2009-11-10 Liang-You Peng , I D Williams , J F McCann

We investigate an influence of the random external electric field on the 2D extremely short optical pulses propagation in the silicene. The random electric field is perpendicular to the silicene plane. An effective equation has the form of…

Mesoscale and Nanoscale Physics · Physics 2016-11-04 Natalia N. Konobeeva , Mikhail B. Belonenko

Previous theoretical studies have shown that attosecond electron dynamics can, in principle, be captured in electron momentum spectroscopy (EMS) using ultrashort electron pulses. By including further analytical considerations on the…

Atomic Physics · Physics 2026-02-23 Pieter Hessel Harkema , Lars Bojer Madsen