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We apply ultrafast spectroscopy to establish a time-domain hierarchy between structural and electronic effects in a strongly-correlated electron system. We discuss the case of the model system VO2, a prototypical non-magnetic compound that…

Strongly Correlated Electrons · Physics 2007-05-23 A. Cavalleri , Th. Dekorsy , H. H. Chong , J. C. Kieffer , R. W. Schoenlein

We have investigated the electronic, vibrational, optical, thermal and piezoelectric properties of LiNbO$_3$, LiTaO$_3$ and Li$_2$NbTaO$_6$ using the first-principles calculation based on the density functional theory. It also shows…

Materials Science · Physics 2025-03-28 Debidutta Pradhan , Rojalin Swain , Souvagya Kumar Biswal , Jagadish Kumar

Thin films of VO$_2$ on different substrates, Al$_2$O$_3$ and SiO$_2$/Si, have been prepared and characterized from room temperature up to 360 K. From the band structure in the rutile metallic phase and in the monoclinic insulating phase…

Strongly Correlated Electrons · Physics 2016-09-21 Tobias Peterseim , Martin Dressel , Marc Dietrich , Angelika Polity

Vanadium dioxide (VO2) has drawn significant attention for its near room temperature insulator to metal transition and associated structural phase transition. The underlying Physics behind the temperature induced insulator to metal and…

Materials Science · Physics 2023-04-19 S. R. Sahu , S. S. Majid , A. Ahad , A. Tripathy , K. Dey , S. Pal , B. K. De , Wen-Pin Hsieh , R. Rawat , V. G. Sathe , D. K. Shukla

The quasi-particle spectra in the metallic rutile and insulating monoclinic phases of VO$_2$ are shown to be dominated by local Coulomb interactions. In the rutile phase the small orbital polarization among V 3d t_2g states leads to weak…

Strongly Correlated Electrons · Physics 2007-05-23 A. Liebsch , H. Ishida , G. Bihlmayer

In complex oxide materials, changes in electronic properties are often associated with changes in crystal structure, raising the question of the relative roles of the electronic and lattice effects in driving the metal-insulator transition.…

Strongly Correlated Electrons · Physics 2019-07-23 Alexandru B. Georgescu , Oleg E. Peil , Ankit Disa , Antoine Georges , Andrew J. Millis

Non-van der Waals two-dimensional (2D) materials derived from strongly bonded non-layered crystals have recently emerged as a novel and rising platform for nanoscale research. While uncovering and tuning their (opto-)electronic, catalytic,…

One of the distinguishing features of an altermagnet is that its spin-up and spin-down bands display a nodal momentum-dependent splitting even in the absence of spin-orbit coupling. While this property has been investigated in many…

Strongly Correlated Electrons · Physics 2026-05-28 Ina Park , Turan Birol , Antoine Georges , Rafael M. Fernandes

The large antiferromagnetic exchange coupling in the parent high-$T_{\rm c}$ cuprate superconductors is believed to play a crucial role in pairing the superconducting carriers. The recent observation of superconductivity in hole-doped…

Strongly Correlated Electrons · Physics 2020-12-22 Vamshi M. Katukuri , Nikolay A. Bogdanov , Oskar Weser , Jeroen van den Brink , Ali Alavi

The metal-insulator transition (MIT) of V6O11 is studied by means of electronic structure calculations using the augmented spherical wave method. The calculations are based on density functional theory and the local density approximation.…

Strongly Correlated Electrons · Physics 2009-11-07 U. Schwingenschloegl , V. Eyert , U. Eckern

Accurate high-energy electron diffraction measurements of structure factors of NiO have been carried out to investigate how strong correlations in the Ni 3d shell affect electron charge density in the interior area of nickel ions and…

Strongly Correlated Electrons · Physics 2009-10-31 S. L. Dudarev , L. -M. Peng , S. Y. Savrasov , J. -M. Zuo

Electronic correlations beyond static mean-field theories are of fundamental importance in describing the properties of complex materials - such as transition-metal oxides - where the low-energy physics is driven by localized d or f…

Strongly Correlated Electrons · Physics 2025-03-17 Mario Caserta , Tommaso Chiarotti , Marco Vanzini , Nicola Marzari

Using the DFT+dynamical mean-field theory method we revisit the pressure-temperature phase diagram of the prototypical correlated insulator NiO. We study the pressure-induced evolution of the electronic structure, magnetic state, and…

Strongly Correlated Electrons · Physics 2024-12-03 G. M. Gaifutdinov , I. V. Leonov

Hydrogen bond (H-bond) covalency has recently been observed in ice and liquid water, while the penetrating molecular orbitals (MOs) in the H-bond region of most typical water dimer system, (H2O)2, have also been discovered. However,…

Atomic and Molecular Clusters · Physics 2016-11-08 Zhiyuan Zhang , Wanrun Jiang , Bo Wang , Zhigang Wang

The electronic structure of the CuO monolayer is investigated taking into account the intra- and interatomic Coulomb interactions on copper and oxygen atoms. Local Coulomb interactions and covalence effects are treated exactly when…

Strongly Correlated Electrons · Physics 2025-03-28 I. A. Makarov , A. A. Slobodchikov , I. A. Nekrasov , Yu. S. Orlov , L. V. Begunovich , M. M. Korshunov , S. G. Ovchinnikov

With their broad range of magnetic, electronic and structural properties, transition metal perovskite oxides ABO3 have long served as a platform for testing condensed matter theories. In particular, their insulating character - found in…

Materials Science · Physics 2019-05-28 Julien Varignon , Manuel Bibes , Alex Zunger

We carry out a detailed study of the role of electronic interaction on $p$ oxygen orbitals in a Mott insulator oxide (UO$_2$) and a charge transfer oxide (TiO$_2$). First, we calculate values of effective interactions \Uff, \Upp{} and…

Strongly Correlated Electrons · Physics 2023-06-21 Robinson Outerovitch , Bernard Amadon

Appropriate consideration of the electron correlation is essential to reproduce the intriguing metal-insulator transition accompanying the Peierls-type structural transition in VO$_2$. In the density functional theory-based approach, this…

Strongly Correlated Electrons · Physics 2021-03-16 Sooran Kim

We report a theoretical study of the effects of electron correlations and structural confinement on the electronic properties and magnetic state of LaNiO3 (LNO) thin films epitaxially deposited on the (001) LaAlO3 (LAO) substrate. Using the…

Strongly Correlated Electrons · Physics 2024-02-01 N. O. Vambold , G. A. Sazhaev , I. V. Leonov

We study the interplay between electronic correlations and hybridization in the low-energy electronic structure of CaMn$_2$Bi$_2$, a candidate hybridization-gap semiconductor. Utilizing a DFT+$U$ approach we find both the antiferromagnetic…

Strongly Correlated Electrons · Physics 2021-02-18 Christopher Lane , M. M. Piva , P. F. S. Rosa , Jian-Xin Zhu