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The 7.6-eV-isomer of Thorium-229 offers the opportunity to perform high resolution laser spectroscopy of a nuclear transition. We give a brief review of the investigations of this isomer. The nuclear resonance connecting ground state and…

Optics · Physics 2017-08-23 E. Peik , K. Zimmermann , M. Okhapkin , Chr. Tamm

We demonstrate coherent Doppler-free three-photon excitation of the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{0}$ optical clock transition and the $^{1}S_{0}$$\leftrightarrow$$^{3}P_{1}$ intercombination transition in free-space thermal clouds of…

Atomic Physics · Physics 2024-12-24 Guglielmo Panelli , Shaun C. Burd , Erik J. Porter , Mark Kasevich

We study the prospects of using the electric quadrupole transitions from the ground states of Cu, Ag and Au to the metastable state $^2{\rm D}_{5/2}$ as clock transitions in optical lattice clocks. We calculate lifetimes, transition rates,…

Atomic Physics · Physics 2021-02-24 V. A. Dzuba , Saleh O. Allehabi , V. V. Flambaum , Jiguang Li , S. Schiller

Recent developments in frequency metrology and optical clocks have been based on electronic transitions in atoms and singly charged ions as references. These systems have enabled relative frequency uncertainties at a level of a few parts in…

Atomic Physics · Physics 2018-12-06 M. G. Kozlov , M. S. Safronova , J. R. Crespo López-Urrutia , P. O. Schmidt

Ultra-stable, quasi-monochromatic laser light forms the basis for high-precision interferometric measurements, e.g. for observing gravitational waves and for time keeping with optical clocks. Optical frequency conversion enables access to…

An optical frequency comb generated with an electro-optic phase modulator and a chirped radiofrequency waveform is used to perform saturation and pump-probe spectroscopy on the $D_1$ and $D_2$ transitions of atomic potassium. With a comb…

Atomic Physics · Physics 2016-12-21 David A. Long , Adam J. Fleisher , David F. Plusquellic , Joseph T. Hodges

An optical atomic clock scheme is developed that utilizes two lasers to establish coherent coupling between the $5s^2 \phantom{}^1S_0$ ground state of $^{88}$Sr and the first excited state, $5s5p \phantom{}^3P_0$. The coupling is mediated…

Atomic Physics · Physics 2009-11-10 Robin Santra , Ennio Arimondo , Tetsuya Ido , Chris H. Greene , Jun Ye

We use complementary optical spectroscopy methods to directly measure the lowest crystal-field energies of the rare-earth quantum magnet LiY$_{1-x}$Ho$_{x}$F$_{4}$, including their hyperfine splittings, with more than 10 times higher…

We present a spectroscopy scheme for the 7-kHz-wide 689-nm intercombination line of strontium. We rely on shelving detection, where electrons are first excited to a metastable state by the spectroscopy laser before their state is probed…

We measure the spectrum of tellurium-130 in the vicinity of the 461~nm ${}^1\text{S}_0-{}^{1}\text{P}_1$ cycling transition in neutral strontium, a popular element for atomic clocks, quantum information, and quantum-degenerate gases. The…

Atomic Physics · Physics 2022-05-23 T. G. Akin , Bryan Hemingway , Steven Peil

We measured the transition frequencies of the hyperfine components in the four lines (P(34) 39-0, R(36) 39-0, P(33) 39-0, and R(35) 39-0) of the B-X transitions of molecular iodine at 520.2 nm. The 520.2 nm laser was generated by…

Chemical Physics · Physics 2024-09-26 Akiko Nishiyama , Sho Okubo , Takumi Kobayashi , Akio Kawasaki , Hajime Inaba

We perform laser spectroscopy of Yb+ ions on the 4f14 6s 2S_{1/2} - 4f13 5d 6s 3D[3/2]_{1/2} transition at 297 nm. The frequency measurements for 170Yb+, 172Yb+, 174Yb+, and 176Yb+ reveal the specific mass shift as well as the field shifts.…

We propose In-like Pr10+ as a candidate for the development of a high-accuracy optical clock with high sensitivity to a time variation of the fine-structure constant, (\dot alpha}/alpha, as well as favorable experimental systematics. We…

We perform spectroscopic observations of the 698-nm clock transition in $^{87}$Sr confined in an optical lattice using a laser linewidth transfer technique. A narrow-linewidth laser interrogating the clock transition is prepared by…

We have measured the frequency of the $6s^2S_{1/2} - 5d^2D_{3/2}$ electric-quadrupole transition of $^{171}$Yb$^+$ with a relative uncertainty of $1\times 10^{-14}$, $\nu_{Yb}$ = 688 358 979 309 312 Hz $\pm$ 6 Hz. A femtosecond frequency…

Optical atomic clocks using highly-charged ions hold an intriguing promise of metrology at the 19th significant figure. Here we study transitions within the $4f^{12}$ ground-state electronic configuration of highly charged ions. We consider…

Atomic Physics · Physics 2015-06-11 V. A. Dzuba , A. Derevianko , V. V. Flambaum

The complete second-order hyperfine-interaction correction is calculated for centroid energy levels of H, D, and $^3$He atoms. For $^3$He, the corrections of $-2.075$~kHz and $-0.305$~kHz beyond the leading hyperfine-mixing contribution are…

Atomic Physics · Physics 2024-12-10 Krzysztof Pachucki , Vojtěch Patkóš , Vladimir A. Yerokhin

Laser spectroscopic studies on minute samples of exotic radioactive nuclei require very efficient experimental techniques. In addition, high resolving powers are required to allow extraction of nu- clear structure information. Here we…

Instrumentation and Detectors · Physics 2017-04-14 R. P. de Groote , M. Verlinde , V. Sonnenschein , K. T. Flanagan , I. Moore , G. Neyens

We report detailed spectroscopic measurements of the X(0)$[^3\Sigma^+]$(v=0) to B(1)$[^3\Pi]$ (v=5) transition in PbO. Using a Stark-modulated laser absorption technique, we have measured the hyperfine constant of $^{207}$PbO in the B(1)…

Atomic Physics · Physics 2009-11-11 D. Kawall , Y. V. Gurevich , C. Cheung , S. Bickman , Y. Jiang , D. DeMille

A sharp resonance line that appears in three-photon transitions between the $^{1}S_{0}$ and $^{3}P_{0}$ states of alkaline earth and Yb atoms is proposed as an optical frequency standard. This proposal permits the use of the even isotopes,…

Optics · Physics 2007-05-23 Tao Hong , Claire Cramer , Warren Nagourney , E. N. Fortson