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We use a combination of optical spectra, first principles calculations, and energy dependent magneto-optical measurements to elucidate the electronic structure and to study the phase diagram of Ni$_3$V$_2$O$_8$. We find a remarkable…

Strongly Correlated Electrons · Physics 2007-05-23 R. C. Rai , J. Cao , S. Brown , J. L. Musfeldt , D. Kasinathan , D. J. Singh , G. Lawes , N. Rogado , R. J. Cava , X. Wei

Magneto-Raman spectroscopy is applied to study spin-phonon coupling in the layered two-dimensional (2D) van der Waals antiferromagnet CrSBr. We report on the effects of temperature and external magnetic field on Raman-active phonons of…

Materials Science · Physics 2025-03-20 Urszula D. Wdowik , Vaibhav Varade , Jana Vejpravova , Dominik Legut

Magneto-optical effect has been widely used in light modulation, optical sensing and information storage. Recently discovered two-dimensional (2D) van der Waals layered magnets are considered as promising platforms for investigating novel…

Direction-dependent charge transport and optical responses are characteristic of van der Waals (vdW) materials with strong in-plane anisotropy. While transition-metal trichalcogenides (TMTCs) exemplify this behavior, heavier analogs remain…

Transition metal phosphorous trichalcogenides, $M{\rm P}X_3$ ($M$ and $X$ being transition metal and chalcogen elements respectively), have been the focus of substantial interest recently because of their possible magnetism in the…

Strongly Correlated Electrons · Physics 2019-12-05 Heung-Sik Kim , David Vanderbilt , Kristjan Haule

The study of magnetism in two-dimensional materials has garnered significant interest, driven by fundamental investigations into low-dimensional magnetic phenomena and their potential for applications in spintronic devices. Through…

Strongly Correlated Electrons · Physics 2025-08-18 Yuanji Xu , Xintao Jin , Haoyuan Tang , Fuyang Tian

Tuning dimensionality in van der Waals materials with finite interlayer coupling has introduced various electronic phase transitions by conventional mechanical exfoliation. Particularly when the electronic order is tied to the modulation of…

Strongly Correlated Electrons · Physics 2023-01-12 Hyoung Kug Kim , So Young Kim , C. J. Won , Sang-Wook Cheong , Jonghwan Kim , Jun Sung Kim , Tae-Hwan Kim

Transition-metal dichalcogenides (TMDs) are layered compounds that support many electronic phases, including various charge density waves, superconducting, and Mott insulating states. Their intercalation with magnetic ions introduces…

Layered van der Waals materials have risen as powerful platforms to artificially engineer correlated states of matter. Here we show the emergence of a multiferroic order in a twisted dichalcogenide bilayer superlattice at quarter-filling.…

Strongly Correlated Electrons · Physics 2022-09-07 Mikael Haavisto , J. L. Lado , Adolfo O. Fumega

Resonant x-ray scattering at the Dy $M_5$ and Ni $L_3$ absorption edges was used to probe the temperature and magnetic field dependence of magnetic order in epitaxial LaNiO$_3$-DyScO$_3$ superlattices. For superlattices with 2 unit cell…

Strongly Correlated Electrons · Physics 2017-06-07 M. Bluschke , A. Frano , E. Schierle , M. Minola , M. Hepting , G. Christiani , G. Logvenov , E. Weschke , E. Benckiser , B. Keimer

FePS$_3$ is a prototype van der Waals layered antiferromagnet and a Mott insulator under ambient conditions, which has been recently reported to go through a pressure-induced dimensionality crossover and an insulator-to-metal transition.…

Strongly Correlated Electrons · Physics 2023-07-19 Shiyu Deng , Siyu Chen , Bartomeu Monserrat , Emilio Artacho , Siddharth S Saxena

Recent discovery of 2D van der Waals (vdW) magnetic materials has spurred progress in developing advanced spintronic devices. A central challenge lies in enhancing the spin-conversion efficiency for building spin-logic or spin-memory…

Materials Science · Physics 2023-08-30 Shuhan Liu , Shaojie Hu , Xiaomin Cui , Takashi Kimura

Antiferromagnetic FePS3 has recently gained significant interest in its potential applications in spin-related devices. Here, we show that in-plane structural anisotropy has a major impact in shaping the optical responses of FePS3…

The coupling between localized spins and phonons can lead to shifts in the dielectric constant of insulating materials at magnetic ordering transitions. Studies on isostructural SeCuO3 (ferromagnetic) and TeCuO3 (antiferromagnetic)…

Materials Science · Physics 2009-04-14 G. Lawes , T. Kimura , C. M. Varma , M. A. Subramanian , R. J. Cava , A. P. Ramirez

The new-found two-dimensional antiferromagnetic GdTe$_3$ is attractive owing to its highest carrier mobility among all known layered magnetic materials, as well as its potential application for novel magnetic twistronic and spintronic…

Materials Science · Physics 2020-10-28 J. S. Liu , S. C. Huan , Z. H. Liu , W. L. Liu , Z. T. Liu , X. L. Lu , Z. Huang , Z. C. Jiang , X. Wang , N. Yu , Z. Q. Zou , Y. F. Guo , D. W. Shen

We present a comprehensive $^{31}$P and $^{65}$Cu nuclear magnetic resonance (NMR) study of the layered van der Waals magnet CuCrP$_2$S$_6$. The compound exhibits a sequence of structural and magnetic phase transitions: a high-temperature…

Strongly Correlated Electrons · Physics 2026-04-06 C. S. Saramgi , L. F. Prager , S. Selter , Y. Shemerliuk , S. Aswartham , B. Büchner , H. -J. Grafe , K. M. Ranjith

Interest in van der Waals materials often stems from a desire to miniaturise existing technologies by exploiting their intrinsic layered structure to create near atomically-thin components that do not suffer from surface defects. One…

Mesoscale and Nanoscale Physics · Physics 2022-08-22 A. J. Healey , S. Rahman , S. C. Scholten , I. O. Robertson , G. J. Abrahams , N. Dontschuk , B. Liu , L. C. L. Hollenberg , Y. Lu , J. -P. Tetienne

The chiral magneto-electric compound Ni3TeO6 is investigated through temperature-dependent synchrotron-based powder x-ray diffraction and x-ray absorption spectroscopy between 15 to 300 K. Our work provides direct evidence for the…

Using a combination of density functional theory (DFT) and spin-wave theory methods, we investigate the magnetic interactions and spin excitations in semiconducting VI$_3$. Exchange parameters of monolayer, bilayer, and bulk forms are…

Materials Science · Physics 2021-09-24 Elijah Gordon , V. V. Mkhitaryan , Haijun Zhao , Y. Lee , Liqin Ke

Following the recent isolation of monolayer CrI3, there has been a surge of new two-dimensional van der Waals magnetic materials, whose incorporation in van der Waals heterostructures offers a new platform for spintronics, proximity…

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