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Using quantum chemistry calculations we shed fresh light on the electronic structure and magnetic properties of RuCl3, a proposed realization of the honeycomb Kitaev spin model. It is found that the nearest-neighbor Kitaev exchange K is…

Strongly Correlated Electrons · Physics 2017-01-19 Ravi Yadav , Nikolay A. Bogdanov , Vamshi M. Katukuri , Satoshi Nishimoto , Jeroen van den Brink , Liviu Hozoi

The Kitaev model on a honeycomb lattice may provide a robust topological quantum memory platform, but finding a material that realizes the unique spin liquid phase remains a considerable challenge. We demonstrate that an effective Kitaev…

Mesoscale and Nanoscale Physics · Physics 2024-06-19 Tessa Cookmeyer , Sankar Das Sarma

The Kitaev honeycomb model plays a pivotal role in the quest for quantum spin liquids, in which fractional quasiparticles would provide applications in decoherence-free topological quantum computing. The key ingredient is the bond-dependent…

Strongly Correlated Electrons · Physics 2024-10-11 Seong-Hoon Jang , Yukitoshi Motome

We study the exchange interactions and resulting magnetic phases in the honeycomb cobaltates. For a broad range of trigonal crystal fields acting on Co2+ ions, the low-energy pseudospin-1/2 Hamiltonian is dominated by bond-dependent Ising…

Strongly Correlated Electrons · Physics 2020-07-23 Huimei Liu , Jiri Chaloupka , Giniyat Khaliullin

The electronic ground state in many iridate materials is described by a complex wave-function in which spin and orbital angular momenta are entangled due to relativistic spin-orbit coupling (SOC). Such a localized electronic state carries…

Combining thermodynamic measurements with theoretical density functional and thermodynamic calculations we demonstrate that the honeycomb lattice iridates A2IrO3 (A = Na, Li) are magnetically ordered Mott insulators where the magnetism of…

Strongly Correlated Electrons · Physics 2012-03-26 Yogesh Singh , S. Manni , J. Reuther , T. Berlijn , R. Thomale , W. Ku , S. Trebst , P. Gegenwart

The low-temperature magnetic properties of \tcr{polycrystalline} Na$_2$IrO$_3$, a candidate material for the realization of a quantum spin-liquid state, were investigated by means of muon-spin relaxation and nuclear magnetic resonance…

The Kitaev model, which hosts a quantum spin liquid (QSL) in the ground state, was originally defined on a two-dimensional honeycomb lattice, but can be straightforwardly extended to any tricoordinate lattices in any spatial dimensions. In…

Strongly Correlated Electrons · Physics 2023-05-29 Kiyu Fukui , Yasuyuki Kato , Yukitoshi Motome

The Kitaev model predicts that quantum spin liquids (QSLs) will form at low temperatures under certain special conditions, and materials hosting the QSL state are frequently sought. The layered honeycomb lattice material {\alpha}-RuCl3 has…

Materials Science · Physics 2022-01-24 Danrui Ni , Xin Gui , Kelly M. Powderly , R. J. Cava

This paper reviews the current progress on searching the Kitaev spin liquid state in 3d electron systems. Honeycomb cobaltates were recently proposed as promising candidates to realize the Kitaev spin liquid state, due to the more localized…

Strongly Correlated Electrons · Physics 2021-10-05 Huimei Liu

The Kitaev quantum spin liquid (KSL) is a theoretically predicted state of matter whose fractionalized quasiparticles are distinct from bosonic magnons, the fundamental excitation in ordered magnets. The layered honeycomb antiferromagnet…

Metastable states with surprising properties abound in Hilbert space. We study unfrustrated isotropic spin-\half Heisenberg models in honeycomb lattice and find emergence of \textit{metastable Kitaev spin liquids having a 2-spin nematic…

Strongly Correlated Electrons · Physics 2023-09-14 Ganapathy Baskaran

The magnetic insulator $\alpha$-RuCl$_{3}$ is a promising candidate to realize Kitaev interactions on a quasi-2D honeycomb lattice. We perform extensive susceptibility measurements on single crystals of $\alpha$-RuCl$_{3}$, including…

Motivated by recent experiments on $\alpha$-RuCl$_3$, we investigate a possible quantum spin liquid ground state of the honeycomb-lattice spin model with bond-dependent interactions. We consider the $K-\Gamma$ model, where $K$ and $\Gamma$…

Strongly Correlated Electrons · Physics 2018-02-15 Matthias Gohlke , Gideon Wachtel , Youhei Yamaji , Frank Pollmann , Yong Baek Kim

Despite the exciting implications of the Kitaev spin-Hamiltonian, finding and confirming the quantum spin liquid state has proven incredibly difficult. Recently the applicability of the model has been expanded through the development of a…

Strongly Correlated Electrons · Physics 2022-09-23 K. M. Taddei , V. O. Garlea , A. M. Samarakoon , L. D. Sanjeewa , J. Xing , T. W. Heitmann , C. dela Cruz , A. S. Sefat , D. Parker

The spin S=$\frac{1}{2}$ Kitaev honeycomb model has attracted significant attention, since emerging candidate materials have provided a playground to test non-Abelian anyons. The Kitaev model with higher spins has also been theoretically…

Strongly Correlated Electrons · Physics 2019-07-24 P. Peter Stavropoulos , D. Pereira , Hae-Young Kee

We study a spin model on honeycomb lattice with two types of Heisenberg exchange couplings, $J$ and $\tilde J$, where $J$ is for the conventional spin and and $\tilde J$ for rotated spin. When $\tilde J=0$, this is the conventional…

Strongly Correlated Electrons · Physics 2015-06-04 Yue Yu , Long Liang , Qian Niu , Shaojing Qin

We present an analytical study of the exchange interactions between pseudospin one-half $d^{5}$ ions in honeycomb lattices with edge-shared octahedra. Various exchange channels involving Hubbard U, charge-transfer excitations, and cyclic…

Strongly Correlated Electrons · Physics 2022-06-10 Huimei Liu , Jiri Chaloupka , Giniyat Khaliullin

The exactly solvable Kitaev honeycomb lattice model is realized as the low energy effect Hamiltonian of a spin-1/2 model with spin rotation and time-reversal symmetry. The mapping to low energy effective Hamiltonian is exact, without…

Strongly Correlated Electrons · Physics 2010-05-20 Fa Wang

Recent proposals for spin-1 Kitaev materials, such as honeycomb Ni oxides with heavy elements of Bi and Sb, have shown that these compounds naturally give rise to antiferromagnetic (AFM) Kitaev couplings. Conceptual interest in such AFM…

Strongly Correlated Electrons · Physics 2020-06-22 Ciarán Hickey , Christoph Berke , Panagiotis Peter Stavropoulos , Hae-Young Kee , Simon Trebst
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