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Related papers: $GW$ vertex corrected calculations for molecular s…

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The GW self-energy method has long been recognized as the gold standard for quasiparticle (QP) calculations of solids in spite of the fact that the neglect of vertex corrections and the use of a DFT starting point lacks rigorous…

Materials Science · Physics 2017-12-06 Per S. Schmidt , Christopher E. Patrick , Kristian S. Thygesen

The $GW$ approximation is based on the neglect of vertex corrections, which appear in the exact self-energy and the exact polarizability. Here, we investigate the importance of vertex corrections in the polarizability only. We calculate the…

Materials Science · Physics 2019-04-16 Alan M. Lewis , Timothy C. Berkelbach

We report an all-electron, atomic orbital (AO) based, two-component (2C) implementation of the $GW$ approximation (GWA) for closed-shell molecules. Our algorithm is based on the space-time formulation of the GWA and uses analytical…

Chemical Physics · Physics 2023-09-11 Arno Förster , Erik van Lenthe , Edoardo Spadetto , Lucas Visscher

Atomic hydrogen provides a unique test case for computational electronic structure methods, since its electronic excitation energies are known analytically. With only one electron, hydrogen contains no electronic correlation and is…

Materials Science · Physics 2007-05-23 W. Nelson , P. Bokes , Patrick Rinke , R. W. Godby

A few approximate schemes to solve the Hedin equations self-consistently introduced in (Phys. Rev. B 94, 155101 (2016)) are explored and tested for the 3D electron gas at metallic densities. We calculate one electron spectra, dielectric…

Strongly Correlated Electrons · Physics 2017-07-12 A. L. Kutepov , G. Kotliar

The $GW$ approximation is considered to be the simplest approximation with Hedin's formulation of many-body perturbation theory. It is expected that some of the deficiencies of the $GW$ approximation can be overcome by adding the so-called…

Materials Science · Physics 2022-12-21 Yanyong Wang , Xinguo Ren

Self-consistent vertex corrected GW calculations have been performed to evaluate the equilibrium volume and corresponding bulk modulus of 3d transition metal vanadium. The study demonstrates the feasibility of this approach. The accuracy of…

Strongly Correlated Electrons · Physics 2018-10-10 Andrey L Kutepov

We provide the formal extension of Hedin's GW equations for single-particle Green's functions with electron-electron interaction onto the Keldysh time-loop contour. We show an application of our formalism to the plasmon model of a core…

Other Condensed Matter · Physics 2011-11-23 H. Ness , L. K. Dash , M. Stankovski , R. W. Godby

Starting with Hedins equations, simple expressions for the irreducible self-energy are derived. The derivation with vertex effects included in the self-energy results in a number of terms beyond GW such as second-order screened exchange…

Computational Physics · Physics 2024-12-17 Brian Cunningham

Diagrammatic perturbation theory is a powerful tool for the investigation of interacting many-body systems, the self-energy operator $\Sigma$ encoding all the variety of scattering processes. In the simplest scenario of correlated electrons…

Strongly Correlated Electrons · Physics 2020-07-22 Y. Pavlyukh , G. Stefanucci , R. van Leeuwen

We test the performance of self-consistent GW and several representative implementations of vertex corrected G0W0 (G0W0{\Gamma}). These approaches are tested on benchmark data sets covering full valence spectra (first ionization potentials…

Chemical Physics · Physics 2024-04-09 Ming Wen , Vibin Abraham , Gaurav Harsha , Avijit Shee , K. Birgitta Whaley , Dominika Zgid

We present a detailed account of the GW space-time method. The method increases the size of systems whose electronic structure can be studied with a computational implementation of Hedin's GW approximation. At the heart of the method is a…

Condensed Matter · Physics 2009-10-31 M. M. Rieger , L. Steinbeck , I. D. White , H. N. Rojas , R. W. Godby

In this work, we benchmark tensor hypercontraction (THC)-accelerated fully self-consistent $GW$ (sc$GW$) and vertex-corrected self-consistent $GW$ (sc$GW\Gamma$) methods for predicting molecular first ionization potentials (IPs). The vertex…

Strongly Correlated Electrons · Physics 2026-04-29 Munkhorgil Wang , Ming Wen , Pavel Pokhilko , Chia-Nan Yeh , Miguel A. Morales , Dominika Zgid

Using the simple (symmetric) Hubbard dimer, we analyze some important features of the $GW$ approximation. We show that the problem of the existence of multiple quasiparticle solutions in the (perturbative) one-shot $GW$ method and its…

Chemical Physics · Physics 2021-10-12 Stefano Di Sabatino , Pierre-François Loos , Pina Romaniello

Self-consistent solutions of Hedin's diagrammatic theory equations (HE) for the two-site Hubbard Model (HM) have been studied. They have been found for three-point vertices of increasing complexity ($\Gamma=1$ (GW approximation),…

Strongly Correlated Electrons · Physics 2016-05-27 A. L. Kutepov

Using a novel self-consistent implementation of Hedin's GW perturbation theory we calculate space and energy dependent self-energy for a number of materials. We find it to be local in real space and rapidly convergent on second-- to third--…

Strongly Correlated Electrons · Physics 2012-04-11 N. E. Zein , S. Y. Savrasov , G. Kotliar

While the well-established $GW$ approximation corresponds to a resummation of the direct ring diagrams and is particularly well suited for weakly-correlated systems, the $T$-matrix approximation does sum ladder diagrams up to infinity and…

Chemical Physics · Physics 2022-04-28 Pierre-François Loos , Pina Romaniello

We introduce a method that allows for the calculation of quasi-particle spectra in the GW approximation, yet avoiding any explicit reference to empty one-electron states. This is achieved by expressing the irreducible polarizability…

Materials Science · Physics 2015-05-14 P. Umari , G. Stenuit , S. Baroni

Using seven semiconductors/insulators with band gaps covering the range from 1 eV to 10 eV we systematically explore the performance of two different variants of self-consistency associated with famous Hedin's system of equations: the full…

Materials Science · Physics 2022-01-20 Andrey L. Kutepov

Electronic excitations and optical spectra of $CdF_{2}$ are calculated up to ultraviolet employing state-of-the-art techniques based on density functional theory and many-body perturbation theory. The GW scheme proposed by Hedin has been…

Materials Science · Physics 2015-06-15 Giancarlo Cappellini , Jürgen Furthmüller , Emiliano Cadelano , Friedhelm Bechstedt