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Iridates supply fertile grounds for unconventional phenomena and exotic electronic phases. With respect to well-studied octahedrally-coordinated iridates, we pay our attention to a rather unexplored iridate, Na4IrO4, showing an unusual…

Strongly Correlated Electrons · Physics 2017-12-13 Xing Ming , Carmine Autieri , Kunihiko Yamauchi , Silvia Picozzi

The magnetic properties of (Ca,Sr)RuO_3 and Sr_2YRuO_6 are studied within the context of band structure based Stoner theory. LSDA calculations without recourse to strong correlation effects yield the correct magnetic behavior and order in…

Materials Science · Physics 2009-10-30 I. I. Mazin , D. J. Singh

We present a model describing the lattice distortion and incommensurate magnetic order in the spinel CdCr2O4, a good realization of the Heisenberg "pyrochlore" antiferromagnet. The magnetic frustration is relieved through the spin-Peierls…

Strongly Correlated Electrons · Physics 2007-05-23 Gia-Wei Chern , C. J. Fennie , O. Tchernyshyov

Double perovskite-based magnets wherein frustration and competition between emergent degrees of freedom are at play can lead to novel electronic and magnetic phenomena. Herein, we report the electronic structure and magnetic properties of…

While it was speculated that 5$d^4$ systems would possess non-magnetic $J$~=~0 ground state due to strong Spin-Orbit Coupling (SOC), all such systems have invariably shown presence of magnetic moments so far. A puzzling case is that of…

We investigate the temperature dependence of the spin dynamics in the pyrochlore magnet Nd$_2$Zr$_2$O$_7$ by neutron scattering experiments. At low temperature, this material undergoes a transition towards an "all in - all out"…

Strongly Correlated Electrons · Physics 2021-07-22 M. Léger , E. Lhotel , M. Ciomaga Hatnean , J. Ollivier , A. R. Wildes , S. Raymond , E. Ressouche , G. Balakrishnan , S. Petit

The complex metal oxides Ni2InSbO6 (NISO) and Ni2ScSbO6 (NSSO) have been prepared in form of polycrystalline powders by a solid state reaction route. The crystal structure and magnetic properties of the compounds were investigated using a…

From a microscopic model for the pyrochlore antiferromagnet Tb2Sn2O7, including the crystal field Hamiltonian and interactions between the angular momenta, we compute an effective pseudospin-1/2 Hamiltonian Heff$ that incorporates…

Statistical Mechanics · Physics 2010-11-30 Paul A. McClarty , Pawel Stasiak , Michel J. P. Gingras

Physical properties of a pyrohafnate compound Pr2Hf2O7 have been investigated by ac magnetic susceptibility \chi_ ac(T), dc magnetic susceptibility \chi(T), isothermal magnetization M(H) and heat capacity C_p(T) measurements on…

It is well known that if a crystal structure has no inversion symmetry, it may allow for Dzyaloshinskii-Moriya magnetic interactions, operating between different crystallographic unit cells, which in turn should lead to the formation of…

Materials Science · Physics 2012-03-19 I. V. Solovyev

Geometrically frustrated magnetic systems, such as those based on the Shastry-Sutherland lattice (SSL), offer a rich playground for exploring unconventional magnetic states. The delicate balance between competing interactions in these…

We report a comprehensive investigation of the triple perovskite iridate Ba$_{3}$CoIr$_{2}$O$_{9}$. Stabilizing in the hexagonal $P6_{3}/mmc$ symmetry at room temperature, this system transforms to a monoclinic $C2/c$ symmetry at the…

Strongly Correlated Electrons · Physics 2021-02-03 Charu Garg , Deepak Roy , Martin Lonsky , Pascal Manuel , Antonio Cervellino , Jens Müller , Mukul Kabir , Sunil Nair

Muon-spin relaxation results on the pyrochlore iridate Nd$_2$Ir$_2$O$_7$ are reported. Spontaneous coherent muon-spin precession below the metal-insulator transition (MIT) temperature of about 33 K is observed, indicating the appearance of…

Strongly Correlated Electrons · Physics 2013-09-03 Hanjie Guo , Kazuyuki Matsuhira , Ikuto Kawasaki , Makoto Wakeshima , Yukio Hinatsu , Isao Watanabe , Zhu-an Xu

We report a magnetic and neutron diffraction study on the ground state magnetism and field evolution of single crystal van der Waals multiferroic CuCrP2S6. The ordered moments align along the b axis in the A-type antiferromagnetic…

Strongly Correlated Electrons · Physics 2026-03-30 Jiasen Guo , Ryan P. Siebenaller , Michael A. Susner , Jiaqiang Yan , Zachary Morgan , Feng Ye

Electron correlation strength is predicted to be weak in 5d transition metal oxides and hence, various anomalous electronic properties observed in these systems are often attributed to the large spin-orbit interaction strength. Employing…

Strongly Correlated Electrons · Physics 2009-07-17 Kalobaran Maiti

Spin-orbit coupling (SOC) plays a crucial role in magnetic and electronic properties of 5$d$ iridates. In this paper we have experimentally investigated the structural and physical properties of a series of Ir-based double perovskite…

Strongly Correlated Electrons · Physics 2019-10-02 Abhisek Bandyopadhyay , I. Carlomagno , L. Simonelli , M. Moretti Sala , A. Efimenko , C. Meneghini , Sugata Ray

A2Ir2O7 iridates were proven to crystallise in the geometrically frustrated pyrochlore structure, which remains stable upon rare-earth cation substitution, temperature variation, and external pressure application. However, the change of…

Strongly Correlated Electrons · Physics 2024-08-05 Daniel Staško , Petr Proschek , Jiří Prchal , Milan Klicpera

In order to understand magnetic behavior observed in CmO$_2$ with non-magnetic ground state, we numerically evaluate magnetic susceptibility on the basis of a seven-orbital Anderson model with spin-orbit coupling. Naively we do not expect…

Strongly Correlated Electrons · Physics 2014-05-30 Fumiaki Niikura , Takashi Hotta

We report a neutron scattering study of the metallic triangular lattice antiferromagnet PdCrO$_2$. Powder neutron diffraction measurements confirm that the crystalline space group symmetry remains $R\bar{3}m$ below $T_N$. This implies that…

Neutron inelastic scattering and diffraction techniques have been used to study the MnV2O4 spinel system. Our measurements show the existence of two transitions to long-range ordered ferrimagnetic states; the first collinear and the second…

Strongly Correlated Electrons · Physics 2009-11-13 V. O. Garlea , R. Jin , D. Mandrus , B. Roessli , Q. Huang , M. Miller , A. J. Schultz , S. E. Nagler