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We report measurements performed on a polycrystalline sample of the pyrochlore compound Nd2Sn2O7. It undergoes a second order magnetic phase transition at Tc ~ 0.91 K to a noncoplanar all-in-all-out magnetic structure of the Nd3+ magnetic…

Strongly Correlated Electrons · Physics 2015-11-04 A. Bertin , P. Dalmas de Reotier , B. Fak , C. Marin , A. Yaouanc , A. Forget , D. Sheptyakov , B. Frick , C. Ritter , A. Amato , C. Baines , P. J. C. King

Muon spin rotation and relaxation experiments in the pyrochlore iridate Eu2Ir2O7 yield a well-defined muon spin precession frequency below the metal-insulator/antiferromagnetic transition temperature TM = 120 K, indicative of long-range…

Strongly Correlated Electrons · Physics 2015-03-19 Songrui Zhao. J. M. Mackie , D. E. MacLaughlin , O. O. Bernal , J. J. Ishikawa , Y. Ohta , S. Nakatsuji

We present a muon spin relaxation study on the Ising pyrochlore Nd$_2$Zr$_2$O$_7$ which develops an "all-in-all-out" magnetic order below 0.4~K. At 20~mK far below the ordering transition temperature, the zero-field muon spin relaxation…

Materials Science · Physics 2016-09-07 J. Xu , C. Balz , C. Baines , H. Luetkens , B. Lake

Neutron scattering has been used to study the magnetic order and spin dynamics of the colossal magnetoresistive pyrochlore Tl_2Mn_2O_7. On cooling from the paramagnetic state, magnetic correlations develop and appear to diverge at T_C (123…

Strongly Correlated Electrons · Physics 2009-10-31 J. W. Lynn , L. Vasiliu-Doloc , M. A. Subramanian

Muon spin rotation (muSR) experiments reveal unconventional spin freezing and dynamics in the two-dimensional (2D) triangular lattice antiferromagnet NiGa2S4. Long-lived disordered Ni-spin freezing (correlation time > 10-6 s at 2 K) sets in…

Strongly Correlated Electrons · Physics 2009-11-13 D. E. MacLaughlin , Y. Nambu , S. Nakatsuji , R. H. Heffner , Lei Shu , O. O. Bernal , K. Ishida

The spin dynamics of geometrically frustrated pyrochlore antiferromagnets Y2Mo2O7 and Tb2Mo2O7 have been investigated using muon spin relaxation. A dramatic slowing down of the moment fluctuations occurs as one approaches the spin freezing…

Nd2Hf2O7, belonging to the family of geometrically frustrated cubic rare earth pyrochlore oxides, was recently identified to order antiferromagnetically below T_N = 0.55 K with an all-in/all-out arrangement of Nd3+ moments, however with a…

Strongly Correlated Electrons · Physics 2017-12-15 V. K. Anand , D. L. Abernathy , D. T. Adroja , A. D. Hillier , P. K. Biswas , B. Lake

We investigate the temperature dependence of the spin dynamics in the pyrochlore magnet Nd$_2$Zr$_2$O$_7$ by neutron scattering experiments. At low temperature, this material undergoes a transition towards an "all in - all out"…

Strongly Correlated Electrons · Physics 2021-07-22 M. Léger , E. Lhotel , M. Ciomaga Hatnean , J. Ollivier , A. R. Wildes , S. Raymond , E. Ressouche , G. Balakrishnan , S. Petit

Muon spin relaxation measurements on Bi2Ir2O7 show that it undergoes a bulk magnetic transition at 1.84(3) K. This is accompanied by increases in the muon spin relaxation rate and the amplitude of the non-relaxing part of the signal. The…

Strongly Correlated Electrons · Physics 2013-06-13 P. J. Baker , J. S. Moeller , F. L. Pratt , W. Hayes , S. J. Blundell , T. Lancaster , T. F. Qi , G. Cao

We report on the muon spin rotation/relaxation study of a pyrochlore oxide, Cd2Os2O7, which exhibits a metal-insulator (MI) transition at T_{MI}~225 K without structural phase transition. It reveals strong spin fluctuation (>10^8/s) below…

Strongly Correlated Electrons · Physics 2009-11-13 A. Koda , R. Kadono , K. Ohishi , S. R. Saha , W. Higemoto , S. Yonezawa , Y. Muraoka , Z. Hiroi

We report a combined muon spin relaxation/rotation, bulk magnetization, neutron scattering, and transport study of the electronic properties of the pyrochlore iridate Nd2Ir2O7. We observe the onset of strongly hysteretic behavior in the…

Er2Ti2O7 is believed to be a realization of an XY antiferromagnet on a frustrated lattice of corner-sharing regular tetrahedra. It is presented as an example of the order-by-disorder mechanism in which fluctuations lift the degeneracy of…

Strongly Correlated Electrons · Physics 2012-09-28 P. Dalmas de Reotier , A. Yaouanc , Y. Chapuis , S. H. Curnoe , B. Grenier , E. Ressouche , C. Marin , J. Lago , C. Baines , S. R. Giblin

Magnetic systems with spins sitting on a lattice of corner sharing regular tetrahedra have been particularly prolific for the discovery of new magnetic states for the last two decades. The pyrochlore compounds have offered the playground…

Strongly Correlated Electrons · Physics 2017-10-05 P. Dalmas de Reotier , C. Marin , A. Yaouanc , C. Ritter , A. Maisuradze , B. Roessli , A. Bertin , P. J. Baker , A. Amato

Magnetic susceptibility and muon spin relaxation (muSR) experiments have been carried out on the quasi-2D triangular-lattice spin S = 2 antiferromagnet FeGa2S4. The muSR data indicate a sharp onset of a frozen or nearly-frozen spin state at…

Strongly Correlated Electrons · Physics 2015-06-11 Songrui Zhao , P. Dalmas de R/'eotier , A. Yaouanc , D. E. MacLaughlin , J. M. Mackie , O. O. Bernal , Y. Nambu , T. Higo , S. Nakatsuji

Building a full understanding of the complex magnetism in the rare-earth pyrochlore iridates, A2Ir2O7, is an ongoing issue in condensed matter physics. The possibility of two interpenetrating and interacting frustrated magnetic pyrochlore…

Strongly Correlated Electrons · Physics 2021-01-01 Ross H. Colman , Kristina Vlaskova , Adam Berlie , Milan Klicpera

We report a neutron diffraction and muon spin relaxation muSR study of static and dynamical magnetic properties of BaCo2V2O8, a quasi-one-dimensional spin-chain system. A proposed model for the antiferromagnetic structure includes: a…

We report magnetic susceptibility, specific heat and muon spin relaxation (muSR) experiments on the triangular antiferromagnet La2Ca2MnO7 which develops a genuine two-dimensional, three-sublattice \sqrt{3} \times \sqrt{3} magnetic order…

Strongly Correlated Electrons · Physics 2015-07-08 P. Dalmas de Réotier , C. Marin , A. Yaouanc , T. Douce , A. Sikora , A. Amato , C. Baines

Muon spin relaxation on Nd$_2$Ti$_2$O$_7$ (NTO) and NdLaTi$_2$O$_7$ (NLTO) compounds are presented. The time spectra for both compounds are as expected for the paramagnetic state at high temperatures, but deviate from the exponential…

Strongly Correlated Electrons · Physics 2014-10-21 Hanjie Guo , Hui Xing , Jun Tong , Qian Tao , Isao Watanabe , Zhu-an Xu

Longitudinal-field muon spin relaxation experiments have been carried out in the paramagnetic state of single-crystal Gd_2Ti_2O_7 just above the phase transition at T_m = 1.0 K. At high applied fields the exponential relaxation time T_1 is…

Strongly Correlated Electrons · Physics 2009-11-11 D. E. MacLaughlin , M. S. Rose , J. E. Anderson , Lei Shu , R. H. Heffner , T. Kimura , G. D. Morris , O. O. Bernal

The very low temperature properties of two pyrochlore compounds, Yb2Ti2O7 and Gd2Sn2O7, were investigated using an ensemble of microscopic and bulk techniques. In both compounds, a first order transition is evidenced, as well as spin…

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