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The slow relaxation and aging of glassy systems can be modelled as a Markov process on a simplified rough energy landscape: energy minima where the system tends to get trapped are taken as nodes of a random network, and the dynamics are…

Disordered Systems and Neural Networks · Physics 2020-01-29 Riccardo Giuseppe Margiotta , Reimer Kühn , Peter Sollich

We use colloidal suspensions encapsulated in emulsion droplets to model confined glass-forming liquids with tunable boundary mobility. We show dynamics in these idealized systems are governed by physical interactions with the boundary.…

Soft Condensed Matter · Physics 2014-05-29 Gary L. Hunter , Kazem V. Edmond , Eric R. Weeks

We study confined colloidal suspensions as a model system which approximates the behavior of confined small molecule glass-formers. Dense colloidal suspensions become glassier when confined between parallel glass plates. We use confocal…

Soft Condensed Matter · Physics 2015-03-13 Kazem V. Edmond , Carolyn R. Nugent , Eric R. Weeks

By characterizing the dynamics of idealized lattice models with a tunable kinetic constraint, we explore the different ways in which dynamical facilitation manifests itself within the local dynamics of glassy materials. Dynamical…

Statistical Mechanics · Physics 2012-06-25 Yael S. Elmatad , Aaron S. Keys

The interaction between passive and active/driven particles has introduced a new way to control colloidal suspension properties from particle aggregation to crystallization. Here, we focus on the hydrodynamic interaction between a single…

Soft Condensed Matter · Physics 2024-02-07 Shih-Yuan Chen , Hector Lopez-Rios , Monica Olvera de la Cruz , Michelle M. Driscoll

We demonstrate that an extended picture of kinetic constraints in glass-forming liquids is sufficient to explain dynamic anomalies observed in dense suspensions of strongly attracting colloidal particles. We augment a simple model of…

Statistical Mechanics · Physics 2009-11-10 Phillip L. Geissler , David R. Reichman

A binary mixture of super-paramagnetic colloidal particles is confined between glass plates such that the large particles become fixed and provide a two-dimensional disordered matrix for the still mobile small particles, which form a fluid.…

Aspects of the dynamical glass transition are considered within a mean field spin glass model. At the dynamical transition the the system condenses in a state of lower entropy. The difference, the information entropy or complexity, is…

Condensed Matter · Physics 2007-05-23 Th. M. Nieuwenhuizen

We study -- using molecular dynamics simulations -- the temperature dependence of the dynamics in a dense short-ranged attractive colloidal glass to find evidence of the kinetic glass-glass transition predicted by the ideal Mode Coupling…

Disordered Systems and Neural Networks · Physics 2009-11-10 Emanuela Zaccarelli , Giuseppe Foffi , Francesco Sciortino , Piero Tartaglia

One of the most controversial hypotheses for explaining the heterogeneous dynamics of glasses postulates the temporary coexistence of two phases characterized by a high and by a low diffusivity. In this scenario, two phases with different…

Soft Condensed Matter · Physics 2015-07-16 R. Pastore , A. Coniglio , M. Pica Ciamarra

We analyse the connections between structure and dynamics in two model glass-formers, using the mutual information between an initial configuration and the ensuing dynamics to compare the predictive value of different structural…

Statistical Mechanics · Physics 2014-09-05 Robert L. Jack , Andrew J. Dunleavy , C. Patrick Royall

We consider the problem of slow activation dynamics in glassy systems undergoing a random first order phase transition. Using an effective potential approach to supercooled liquids, we determine the spectrum of activation barriers for…

Disordered Systems and Neural Networks · Physics 2013-05-29 Maxim Dzero , Joerg Schmalian , Peter G. Wolynes

The transition into a glassy state of the ensemble of static, mechanically stable configurations of a tapped granular pile is explored using extensive molecular dynamics simulations. We show that different horizontal sub-regions ("layers")…

Soft Condensed Matter · Physics 2022-01-19 Paula A Gago , Stefan Boettcher

It has been recently shown that one can understand the Prigogine-Defay ratio at the glass transition in terms of freezing into one of the many inherent states of the undercooled liquid. In the present paper, the treatment is extended to the…

Disordered Systems and Neural Networks · Physics 2016-03-21 U. Buchenau

We study thermally activated dynamics using functional renormalization within the field theory of randomly pinned elastic systems, a prototype for glasses. It appears through an essentially non-perturbative boundary layer in the running…

Disordered Systems and Neural Networks · Physics 2007-05-23 Leon Balents , Pierre Le Doussal

We investigate the dynamics of kinetically constrained models of glass formers by analysing the statistics of trajectories of the dynamics, or histories, using large deviation function methods. We show that, in general, these models exhibit…

Statistical Mechanics · Physics 2009-01-21 J. P. Garrahan , R. L. Jack , V. Lecomte , E. Pitard , K. van Duijvendijk , F. van Wijland

Using video microscopy, we measure local spatial constraints in disordered binary colloidal samples, ranging from dilute fluids to jammed glasses, and probe their spatial and temporal correlations to local dynamics during the glass…

Soft Condensed Matter · Physics 2019-07-03 Xiunan Yang , Hua Tong , Wei-Hua Wang , Ke Chen

We review the field of the glass transition, glassy dynamics and aging from a statistical mechanics perspective. We give a brief introduction to the subject and explain the main phenomenology encountered in glassy systems, with a particular…

Statistical Mechanics · Physics 2020-10-12 Francesco Arceri , François P. Landes , Ludovic Berthier , Giulio Biroli

We review a theoretical perspective of the dynamics of glass forming liquids and the glass transition. It is a perspective we have developed with our collaborators during this decade. It is based upon the structure of trajectory space. This…

Soft Condensed Matter · Physics 2010-04-20 David Chandler , Juan P. Garrahan

We explore the glassy dynamics of soft colloids using microgels and charged particles interacting by steric and screened Coulomb interactions, respectively. In the supercooled regime, the structural relaxation time $\tau_\alpha$ of both…