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While various structural and dynamical precursors to vitrification have been identified, a predictive and quantitative description of how subtle changes at the microscopic scale give rise to the steep growth in macroscopic viscosity is…

Soft Condensed Matter · Physics 2016-12-05 Ruben Higler , Johannes Krausser , Jasper van der Gucht , Alessio Zaccone , Joris Sprakel

Despite the enormous theoretical and application interests, a fundamental understanding of the glassy dynamics remains elusive. The static properties of glassy and ordinary liquids are similar, but their dynamics are dramatically different.…

Soft Condensed Matter · Physics 2023-11-21 Puneet Pareek , Monoj Adhikari , Chandan Dasgupta , Saroj Kumar Nandi

As approaching the glass transition, particle motion in liquids becomes highly heterogeneous and regions with virtually no mobility coexist with liquid-like domains. This complex dynamics is believed to be responsible for different…

Soft Condensed Matter · Physics 2018-03-28 F. Puosi , N. Jakse , A. Pasturel

Dense assemblies of self-propelled particles undergo a nonequilibrium form of glassy dynamics. Physical intuition suggests that increasing departure from equilibrium due to active forces fluidifies a glassy system. We falsify this belief by…

Soft Condensed Matter · Physics 2017-12-08 Ludovic Berthier , Elijah Flenner , Grzegorz Szamel

The emergence of nanoscience has increased the importance of experiments able to probe the very local structure of materials, especially for disordered and heterogeneous systems. This is technologically important; for example, the nanoscale…

Soft Condensed Matter · Physics 2015-05-13 R. Casalini , C. M. Roland

We have considered the dynamical evolution of cellular patterns controlled by a stochastic Glauber process determined by the deviations of local cell topology from that of a crystalline structure. Above a critical temperature evolution is…

Disordered Systems and Neural Networks · Physics 2009-10-31 Tomaso Aste , David Sherrington

Systems in which a short-ranged attraction and long-ranged repulsion compete are intrinsically frustrated, leading their structure and dynamics to be dominated either by mesoscopic order or by metastable disorder. Here we report the latter…

Soft Condensed Matter · Physics 2017-12-27 Christian L. Klix , C. Patrick Royall , Hajime Tanaka

We study the aging dynamics in a model for dense simple liquids, in which particles interact through a hard-core repulsion complemented by a short-ranged attractive potential, of the kind found in colloidal suspensions. In this system, at…

Statistical Mechanics · Physics 2007-05-23 G. Foffi , E. Zaccarelli , S. Buldyrev , F. Sciortino , P. Tartaglia

We propose an interacting lattice gas model of structural glass characterized by particle distinguishability and site-particle-dependent random nearest-neighboring particle interactions. This incorporates disorder quenched in the…

Statistical Mechanics · Physics 2017-05-24 Ling-Han Zhang , Chi-Hang Lam

With molecular dynamics simulations of a fluid mixture of classical particles interacting with pair-wise additive Weeks-Chandler-Andersen potentials, we consider the time series of particle displacements and thereby determine distributions…

Statistical Mechanics · Physics 2011-11-10 Lester O. Hedges , Lutz Maibaum , David Chandler , Juan P. Garrahan

Glasses are structurally liquid-like, but mechanically solid-like. Most attempts to understand glasses start from liquid state theory. Here we take the opposite point of view, and use concepts from solid state physics. We determine the…

Soft Condensed Matter · Physics 2015-05-14 Antina Ghosh , Vijayakumar K. Chikkadi , Peter Schall , Jorge Kurchan , Daniel Bonn

The history dependence of the glasses formed from flow-melted steady states by a sudden cessation of the shear rate $\dot\gamma$ is studied in colloidal suspensions, by molecular dynamics simulations, and mode-coupling theory. In an ideal…

Aging in an attraction-driven colloidal glass is studied by computer simulations. The system is equilibrated without attraction and instantaneously ``quenched'', at constant colloid volume fraction, to one of two states beyond the glass…

Soft Condensed Matter · Physics 2015-06-25 Antonio M. Puertas , Matthias Fuchs , Michael E. Cates

We use the swap Monte Carlo algorithm to analyse the glassy behaviour of sticky spheres in equilibrium conditions at densities where conventional simulations and experiments fail to reach equilibrium, beyond predicted phase transitions and…

Soft Condensed Matter · Physics 2020-12-21 Christopher J. Fullerton , Ludovic Berthier

We conduct a numerical study of the dynamical behavior of a system of three-dimensional crosses, particles that consist of three mutually perpendicular line segments rigidly joined at their midpoints. In an earlier study [W. van Ketel et…

Disordered Systems and Neural Networks · Physics 2009-11-13 Patrick Charbonneau , Chinmay Das , Daan Frenkel

The dynamic behavior of a hard-sphere colloidal suspension was studied by X-ray Photon Correlation Spectroscopy and Small Angle X-ray Scattering over a wide range of particle volume fractions. The short-time mobility of the particles was…

The slow dynamics in a glassy hard-sphere system is dominated by cage breaking events, i.e., rearrangements where a particle escapes from the cage formed by its neighboring particles. We study such events for an overdamped colloidal system…

Soft Condensed Matter · Physics 2016-10-26 Matthias Kohl , Andreas Härtel , Michael Schmiedeberg

The transport properties of colloidal particles in active liquids have been studied extensively. It has led to a deeper understanding of the interactions between passive and active particles. However, the phase behavior of colloidal…

Soft Condensed Matter · Physics 2023-01-30 Pragya Kushwaha , Vivek Semwal , Sayan Maity , Shraddha Mishra , Vijayakumar Chikkadi

We present a computer simulation study of a disordered two-dimensional system of localized interacting electrons at thermal equilibrium. It is shown that the configuration of occupied sites within the Coulomb gap persistently changes at…

Disordered Systems and Neural Networks · Physics 2007-05-23 D. Menashe , O. Biham , B. D. Laikhtman , A. L. Efros

Aging dynamics in glassy systems is investigated by considering the hopping motion in a rugged energy landscape whose deep minima are characterized by an exponential density of states. In particular we explore the behavior of a generic…

Statistical Mechanics · Physics 2009-11-07 Bernd Rinn , Philipp Maass , Jean-Philippe Bouchaud