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In the quest for materials with unconventional quantum phases, the organic triangular-lattice antiferromagnet $\kappa$-(ET)$_2$Cu$_2$(CN)$_3$ has been extensively discussed as a quantum spin liquid (QSL) candidate. Recently, an intriguing…

Strongly Correlated Electrons · Physics 2019-06-13 Kira Riedl , Roser Valenti , Stephen M. Winter

Experimental quest for the hypothetical "quantum spin liquid" state has recently met a few promising candidate materials including organic salts \kappa-(ET)2Cu2(CN)3 and EtMe3Sb[Pd(dmit)2]2, S=1/2 triangular-lattice Heisenberg…

Strongly Correlated Electrons · Physics 2015-06-17 Ken Watanabe , Hikaru Kawamura , Hiroki Nakano , Toru Sakai

We report the discovery of a novel gapless quantum spin liquid in the S=1 honeycomb system Cu$_3$LiRu$_2$O$_6$ with Ru$^{4+}$ ($4d^4$) where moments remain dynamic down to 50 mK. Heat capacity measurements show no sign of magnetic ordering…

Actively shought since the turn of the century, two-dimensional quantum spin liquids (QSLs) are exotic phases of matter where magnetic moments remain disordered even at extremely low temperatures. Despite ongoing searches, QSLs remain…

Strongly Correlated Electrons · Physics 2015-07-22 Juan Carrasquilla , Zhihao Hao , Roger G. Melko

Quantum spin liquid (QSL) has become an exciting topic in interacting spin systems that do not order magnetically down to the lowest experimentally accessible temperature; however, conclusive experimental evidence remains lacking. Motivated…

Strongly Correlated Electrons · Physics 2023-10-26 Saikat Banerjee , Wei Zhu , Shi-Zeng Lin

Quantum fluctuations are expected to lead to highly entangled spin-liquid states in certain two-dimensional spin-1/2 compounds. We have synthesized and measured thermodynamic properties and muon spin relaxation rates in the copper-based…

Quantum spin liquids are a new class of magnetic ground state in which spins are quantum mechanically entangled over macroscopic scales. Motivated by recent advances in the control of polar molecules, we show that dipolar interactions…

Strongly Correlated Electrons · Physics 2018-04-23 Norman Y. Yao , Michael P. Zaletel , Dan M. Stamper-Kurn , Ashvin Vishwanath

Quantum fluctuations originating phase competition or geometrical frustration of spins lead to novel states such as a quantum critical point and a quantum spin liquid where the strong quantum fluctuations suppress any ordered states even at…

Strongly Correlated Electrons · Physics 2019-11-28 Y. Saito , H. Nakamura , M. Sawada , T. Yamazaki , S. Fukuoka , N. Matsunaga , K. Nomura , M. Dressel , A. Kawamoto

A quantum magnet, LiCuSbO4, with chains of edge-sharing S = 1/2 CuO6 octahedra is reported. While the Curie-Weiss constant is ferromagnetic, \theta = 30 K, no phase transition or spin freezing occurs down to 100 mK. Specific heat indicates…

Strongly Correlated Electrons · Physics 2012-05-04 S. E. Dutton , M. Kumar , M. Mourigal , Z. G. Soos , J. -J. Wen , C. L. Broholm , N. H. Andersen , Q. Huang , M. Zbiri , R. Toft-Petersen , R. J. Cava

The physics of interacting nuclear spins arranged in a crystalline lattice is typically described using a thermodynamic framework: a variety of experimental studies in bulk solid-state systems have proven the concept of a spin temperature…

Mesoscale and Nanoscale Physics · Physics 2009-07-21 P. Maletinsky , M. Kroner , A. Imamoglu

Quantum spin liquid (QSL), a state characterized by exotic low energy fractionalized excitations and statistics is still elusive experimentally and may be gauged via indirect experimental signatures. Remnant of QSL phase may reflect in the…

Strongly Correlated Electrons · Physics 2023-03-29 Vivek Kumar , Deepu Kumar , Birender Singh , Yuliia Shemerliuk , Mahdi Behnami , Bernd Buchner , Saicharan Aswartham , Pradeep Kumar

Quantum Spin Liquids (QSLs) are phases of interacting spins that do not order even at the absolute zero temperature, making it impossible to characterize them by a local order parameter. In this article, we review the unique view provided…

Strongly Correlated Electrons · Physics 2013-02-06 Tarun Grover , Yi Zhang , Ashvin Vishwanath

We found a plateau in the magnitude of the isolated magnetic moments as a function of the anisotropy of the transfer integral (t'/t) in the gapless quantum spin liquid (QSL) phase of an S=1/2 triangular lattice molecular solid X[Pd(dmit)2]2…

Strongly Correlated Electrons · Physics 2024-03-20 K. Ueda , S. Fujiyama , R. Kato

Quantum spin liquids (QSLs) represent exotic states of matter where quantum spins interact strongly yet evade long-range magnetic order down to absolute zero. Characterized by non-local quantum entanglement and resultant fractionalized…

Strongly Correlated Electrons · Physics 2025-12-05 Yuji Matsuda , Takasada Shibauchi , Hae-Young Kee

Quantum spin liquid is an exotic quantum state of matter in magnets. This state is a spin analogue of the liquid helium which does not solidify down to the lowest temperature due to strong quantum fluctuations. In conventional fluids,…

Strongly Correlated Electrons · Physics 2015-06-22 Joji Nasu , Masafumi Udagawa , Yukitoshi Motome

Quantum spin liquids (QSLs) are highly entangled, disordered magnetic states that arise in frustrated Mott insulators and host exotic fractional excitations such as spinons and chargons. Despite being charge insulators some QSLs are…

Pursuing fractionalized particles that do not bear properties of conventional measurable objects, exemplified by bare particles in the vacuum such as electrons and elementary excitations such as magnons, is a challenge in physics. Here we…

Strongly Correlated Electrons · Physics 2021-08-17 Yusuke Nomura , Masatoshi Imada

We report that a possible Z2 quantum spin liquid (QSL) can be observed in a new class of frustrated system: spinor bosons subject to a pi flux in a square lattice. We construct a new class of Ginsburg-Landau (GL) type of effective action to…

Strongly Correlated Electrons · Physics 2020-05-12 Fadi Sun , Jinwu Ye

Quantum spin liquids (QSL) are phases of matter which are distinguished not by the symmetries they break, but rather by the patterns of entanglement within them. Although these entanglement properties have been widely discussed for ground…

Strongly Correlated Electrons · Physics 2026-02-10 Snigdh Sabharwal , Matthias Gohlke , Paul Skrzypczyk , Nic Shannon

The Ce$^{3+}$ pseudospin-$\frac{1}{2}$ degrees of freedom in the pyrochlore magnet Ce$_2$Zr$_2$O$_7$ are known to possess dipole-octupole (DO) character, making it a candidate for novel quantum spin liquid (QSL) ground states at low…