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We develop a theoretical framework for high-harmonic generation (HHG) driven by quantum states of light based on a temporal-mode expansion of the electromagnetic field. This approach extends previous single plane-wave mode treatments to…

Quantum Physics · Physics 2025-12-09 Juan M. González-Monge , Johannes Feist

Harmonic generation from solid surfaces is a promising tool for producing high energy attosecond pulses. We report shaping of the harmonic spectrum to achieve the bandwidth necessary for attosecond pulse generation. The shaping is…

Plasma Physics · Physics 2019-03-27 A. Seyen , R. Kohn , U. Bovensiepen , D. von der Linde , A. Tarasevitch

The direct measurement of Berry phases is still a great challenge in condensed matter systems. The bottleneck has been the ability to adiabatically drive an electron coherently across a large portion of the Brillouin zone in a solid where…

We theoretically study the high-harmonic generation (HHG) in one-dimensional spin systems. While in electronic systems the driving by AC electric fields produces radiation from the dynamics of excited charges, we consider here the situation…

Strongly Correlated Electrons · Physics 2019-05-24 Shintaro Takayoshi , Yuta Murakami , Philipp Werner

This Letter brings together two topics that, until now, have been the focus of intense but non-overlapping research efforts. The first concerns high harmonic generation in solids, which occurs when intense light field excites highly…

Strongly Correlated Electrons · Physics 2022-04-06 R. E. F. Silva , Igor V. Blinov , Alexey N. Rubtsov , O. Smirnova , M. Ivanov

We theoretically investigate high-order harmonic generation (HHG) in Rydberg atoms driven by spatially inhomogeneous laser fields, induced, for instance, by plasmonic enhancement. It is well known that the laser intensity should to exceed…

Atomic Physics · Physics 2016-07-08 Y. Tikman , I. Yavuz , M. F. Ciappina , A. Chacon , Z. Altun , M. Lewenstein

We experimentally disentangle the contributions of different quantum paths in high-order harmonic generation (HHG) from the spectrally and spatially resolved harmonic spectra. By adjusting the laser intensity and focusing position, we…

Atomic Physics · Physics 2015-10-08 Lixin He , Pengfei Lan , Qingbin Zhang , Chunyang Zhai , Feng Wang , Wenjing Shi , Peixiang Lu

We consider noninteracting electrons coupled to laser fields, and study perturbatively the effects of the lattice potential involving disorder on the harmonic components of the electric current, which are sources of high-order harmonic…

Disordered Systems and Neural Networks · Physics 2020-01-15 Koki Chinzei , Tatsuhiko N. Ikeda

High harmonic generation (HHG) in crystals has revealed a wealth of perspectives such as all-optical mapping of the electronic band structure, ultrafast quantum information and the creation of novel all-solid-state attosecond sources.…

Breaking inversion symmetry in solids plays a central role in nonlinear optics because it can change material properties, such as producing even-order nonlinear optical (NLO) effects. Although a centrosymmetric diamond has been developed as…

Optics · Physics 2022-03-21 Aizitiaili Abulikemu , Yuta Kainuma , Toshu An , Muneaki Hase

High harmonic generation (HHG) is a striking phenomenon, which reflects the ultrafast dynamics of electrons. Recently, it has been demonstrated that HHG can be used to reconstruct not only the energy band structure but also the geometric…

Mesoscale and Nanoscale Physics · Physics 2024-09-10 Atsushi Ono , Shun Okumura , Shohei Imai , Yutaka Akagi

High-order harmonic generation (HHG) in solids - the frequency up-conversion of an optical signal - is governed by symmetries. At terahertz (THz) frequencies, HHG is a key technology to access high frequency spectral windows that are…

High-order harmonic generation (HHG) in gases leads to short-pulse extreme ultraviolet (XUV) radiation useful in a number of applications, for example, attosecond science and nanoscale imaging. However, this process depends on many…

We develop a multipolar theory of second-harmonic generation (SHG) by dielectric nanoparticles made of noncentrosymmetric materials with bulk quadratic nonlinearity. We specifically analyze two regimes of optical excitation: illumination by…

Highly nonlinear optical phenomena can provide access to properties of electronic systems which are otherwise difficult to access through conventional linear optical spectroscopies. In particular, high harmonic generation (HHG) in…

Optics · Physics 2021-04-28 K. Uchida , V. Pareek , K. Nagai , K. M. Dani , K. Tanaka

We propose a novel amplification mechanism for high harmonic generation (HHG) in solids by leveraging bandgap engineering with momentum k-gaps. By constructing a simple diatomic lattice featuring balanced, alternating gain and loss…

Optics · Physics 2025-03-28 Yiming Pan , Danni Chen , Xiaoxi Xu , Zhaopin Chen , Huaiqiang Wang

High-harmonic generation in solids allows probing and controlling electron dynamics in crystals on few femtosecond timescales, paving the way to lightwave electronics. In the spatial domain, recent advances in the real-space interpretation…

Light beams carrying orbital angular momentum (OAM) have led to stunning applications in various fields from quantum information to microscopy. In this letter, we examine OAM from the recently discovered high-harmonic generation (HHG) in…

High harmonic generation (HHG) is a highly nonlinear emission process in which systems driven by intense laser pulses emit integer multiples (harmonics) of the driving field. This feature is considered universal to all occurrences of HHG.…

The strong-field process of high-harmonic generation (HHG) has, in recent years, been treated from a quantum optical perspective in the emerging research area of strong-field quantum optics. These investigations show that HHG radiation is,…

Quantum Physics · Physics 2026-02-19 Christian Saugbjerg Lange , Lars Bojer Madsen