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High-harmonic generation driven by temporal-mode quantum states of light

Quantum Physics 2025-12-09 v1 Atomic Physics

Abstract

We develop a theoretical framework for high-harmonic generation (HHG) driven by quantum states of light based on a temporal-mode expansion of the electromagnetic field. This approach extends previous single plane-wave mode treatments to realistic pulse configurations, resolving conceptual inconsistencies arising from non-normalizable infinite plane waves and establishing consistency between analytical and numerical methods. We derive a correction factor that quantifies deviations from the single-mode approximation and show that it remains below 10410^{-4} for intensities typical of HHG (1014 \sim 10^{14}~W/cm2^2). This result confirms that free-space HHG driven by any quantum state of light is accurately described by averaging semi-classical calculations over the Husimi distribution, with no observable genuine quantum effects. The absence of such effects is attributed to the large photon numbers (1011\sim 10^{11}) required to reach HHG intensities in free space, which render quantum fluctuations negligible. We discuss nanophotonic environments with ultrasmall mode volumes as potential platforms where few-photon strong-field processes could exhibit genuine quantum signatures.

Keywords

Cite

@article{arxiv.2512.06602,
  title  = {High-harmonic generation driven by temporal-mode quantum states of light},
  author = {Juan M. González-Monge and Johannes Feist},
  journal= {arXiv preprint arXiv:2512.06602},
  year   = {2025}
}
R2 v1 2026-07-01T08:13:16.802Z