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We investigate theoretically the effect of injection of plasmonic carriers from an optically-excited metal nanocrystal to a semiconductor contact or to attached molecules. The distributions of optically-excited hot carriers are dramatically…

Mesoscale and Nanoscale Physics · Physics 2013-09-20 Alexander O. Govorov , Hui Zhang , Yurii K. Gounko

Space-time (ST) wave packets are propagation-invariant pulsed optical beams that travel freely in dielectrics at a tunable group velocity without diffraction or dispersion. Because ST wave packets maintain these characteristics even when…

Pump-probe spectroscopy is central for exploring ultrafast dynamics of fundamental excitations, collective modes and energy transfer processes. Typically carried out using conventional diffraction-limited optics, pump-probe experiments…

Localized surface plasmons are confined collective oscillations of electrons in metallic nanoparticles. When driven by light, the optical response is dictated by geometrical parameters and the dielectric environment and plasmons are…

Electron microscopy techniques such as electron energy-loss spectroscopy (EELS) facilitate the spatio-spectral characterization of plasmonic nanostructures. In this work, a time-dependent perspective is presented, which significantly…

We present a method to locally probe spatially varying chemical composition of soft matter systems by use of optically controlled and elastically self-assembled plasmonic nanoantennae. Disc-shaped metal particles with sharp irregular edges…

Two types of amorphous functional materials, based on lightsensitive inorganic compounds like Se and As20Se80 chalcogenide glass (ChG) were investigated with the aim to establish the influence of plasmonic fields, excited by the band-gap…

Materials Science · Physics 2015-02-06 M. L. Trunov , P. M. Lytvyn , P. M. Nagy , A. Csik , V. M. Rubish , S. Kokenyesi

We propose a plasmonic device consisting of a concentric ring grating acting as an efficient tool for directional launching and detection of surface plasmon-polaritons (SPPs). Numerical simulations and optical characterizations are used to…

Mesoscale and Nanoscale Physics · Physics 2016-01-05 N. Rahbany , W. Geng , R. Salas-Montiel , S. de la Cruz , E. R. Méndez , S. Blaize , R. Bachelot , C. Couteau

We combine ab-initio calculations based on many-body perturbation theory and the cumulant expansion with angle-resolved photoemission spectroscopy (ARPES) to quantify the electron-plasmon interaction in the highly-doped semiconducting…

Strongly Correlated Electrons · Physics 2023-07-12 Christoph Emeis , Sanjoy Kr Mahatha , Sebastian Rohlf , Kai Rossnagel , Fabio Caruso

We study light absorption by a dipolar absorber in a given environment, which can be a nanoantenna or any complex inhomogeneous medium. From first-principle calculations, we derive an upper bound for the absorption, which decouples the…

Surface charging is a phenomenon ubiquitously observable in in-situ transmission electron microscopy of non-conducting specimens as a result of electron beam/sample interactions or optical stimuli and often limits the achievable image…

Mesoscale and Nanoscale Physics · Physics 2024-08-27 Jonathan T. Weber , Sascha Schäfer

The recent generalised nonlocal optical response (GNOR) theory for plasmonics is analysed, and its main input parameter, namely the complex hydrodynamic convection-diffusion constant, is quantified in terms of enhanced Landau damping due to…

Mesoscale and Nanoscale Physics · Physics 2020-08-26 Mark. K. Svendsen , Christian Wolff , Antti-Pekka Jauho , N. Asger Mortensen , Christos Tserkezis

Plasmonic nanoparticles influence the absorption and emission processes of nearby emitters due to local enhancements of the illuminating radiation and the photonic density of states. Here, we use the plasmon resonance of metal nanoparticles…

A physically transparent unified theory of optically and plasmon induced hot carrier generation in metals is developed with all the relevant mechanisms included. Analytical expressions that estimate the carrier generation rates, their…

Optics · Physics 2019-06-19 Jacob B Khurgin

Using interplay between surface plasmons and metamaterials, we propose a new technique for novel metamaterial designs. We show that surface plasmons existing on thin metal surfaces can be used to "drive" non-resonant structures in their…

Optics · Physics 2011-04-12 Durdu O. Guney , Thomas Koschny , Costas M. Soukoulis

We provide the quantum mechanical description of the excitation of long-range surface plasmon polaritons (LRSPPs) on thin metallic strips. The excitation process consists of an attenuated-reflection setup, where efficient photon-to-LRSPP…

Quantum Physics · Physics 2013-12-25 D. Ballester , M. S. Tame , C. Lee , J. Lee , M. S. Kim

This paper is concerned with the analysis of time-harmonic electromagnetic scattering from plasmonic inclusions in the finite frequency regime beyond the quasi-static approximation. The electric permittivity and magnetic permeability in the…

Analysis of PDEs · Mathematics 2019-01-29 Hongjie Li , Shanqiang Li , Hongyu Liu , Xianchao Wang

Active nanoplasmonics has recently led to the emergence of many promising applications. One of them is spaser (surface plasmons amplification by stimulated emission of radiation) that has been shown to generate coherent and intense fields…

Optics · Physics 2019-05-27 Mariam Tohari , Andreas Lyras , Mohamad AlSalhi

We present a simple model to describe the lowest-subbands surface scattering in locally oxidized silicon nanowires grown in the [110] direction. To this end, we employ an atomistically scaled effective mass model projected from a…

Materials Science · Physics 2010-02-03 Panagiotis Drouvelis , Giorgos Fagas

High-performance osmotic energy conversion requires both large ionic throughput and high ionic selectivity, which can be significantly promoted by exterior surface charges simultaneously, especially for short nanopores. Here, we investigate…

Chemical Physics · Physics 2022-06-08 Long Ma , Xuan An , Fenhong Song , Yinghua Qiu