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First-principles crystal structure search is performed to predict novel rubidium poly-nitrogen materials at high pressure by varying the stoichiometry, i. e. relative quantities of the constituent rubidium and nitrogen atoms. Three…

Materials Science · Physics 2017-11-29 Ashley S. Williams , Brad A. Steele , van I. Oleynik

Despite great technological importance and many investigations, a material with measured hardness comparable to that of diamond or cubic boron nitride has yet to be identified. Combined theoretical and experimental investigations led to the…

Materials Science · Physics 2009-07-10 L. S. Dubrovinsky , N. A. Dubrovinskaia , V. Swamy , J. Muscat , N. M. Harrison , R. Ahuja , B. Holm

Three new novel phases of carbon nitride (CN) bilayer, which are named as \alpha-C$_{2}$N$_{2}$, \beta-C$_{2}$N$_{2}$ and \gamma-C$_{4}$N$_{4}$, respectively, have been predicted in this paper. All of them are consisted of two CN sheets…

Materials Science · Physics 2019-02-01 Wanxing Lin , Shi-Dong Liang , Chunshan He , Wucheng Xie , Haiying He , Quanxiang Mai , Jiesen Li , D. X. Yao

Chromium nitride (CrN) is a thermoelectric transition metal nitride whose properties are strongly influenced by stoichiometry, substrate choice, and defect chemistry. CrN is routinely synthesized by physical vapor deposition (PVD), its…

Materials Science · Physics 2026-03-05 Lewis J. Adams , Sara Baserga , Laurent Souqui , Enji Sadek , Linus von Fieandt , Per Eklund

A multitude of observed boron-based materials have outstanding superconducting, mechanical, and refractory properties. Yet, the structure, the composition, and the very existence of some reported metal boride (M-B) compounds have been a…

Materials Science · Physics 2014-10-03 A. G. Van Der Geest , A. N. Kolmogorov

A computational search for stable structures among both $\alpha$ and $\beta$ phases of ternary ATB4 borides (A= Mg, Ca, Sr, Ba, Al, Ga, and Zn, T is 3d or 4d transition elements) has been performed. We found that $\alpha$-ATB4 compounds…

Materials Science · Physics 2023-10-31 Yang Sun , Zhen Zhang , Andrew P Porter , Kirill Kovnir , Kai-Ming Ho , Vladimir Antropov

Carbon nitride two-dimensional (2D) materials are among the most attractive class of nanomaterials, with wide range of application prospects. As a continuous progress, most recently, two novel carbon nitride 2D lattices of C3N5 and C3N4…

Single-atom-thick two-dimensional materials such as graphene usually have a hexagonal lattice while the square-planar lattice is uncommon in the family of two-dimensional materials. Here, we demonstrate that single-atom-thick transition…

Materials Science · Physics 2022-09-26 Dapeng Liu , Panjun Feng , Shuo Zhang , Miao Gao , Fengjie Ma , Xun-Wang Yan , Z. Y. Xie

Using an ab initio evolutionary algorithm combined with first-principles calculations, two metastable NaMnO$_2$ polymorphs, $I4_1/amd$ and Cmcm, are identified as promising cathode materials for sodium-ion batteries. Both phases exhibit…

Materials Science · Physics 2025-06-24 Fukuan Wang , Chen Zhou , Busheng Wang , Yong Liu

The basic known and hypothetic one- and two-element phases of the B-C-N-O system (both superhard phases having diamond and boron structures and precursors to synthesize them) are described. The attention has been given to the structure,…

Materials Science · Physics 2011-01-18 O. O. Kurakevych

We have performed first-principles evolutionary searches for all stable titanium nitrides and have found, in addition to the well-known rocksalt-type TiN, new ground states Ti$_3$N$_2$, Ti$_4$N$_3$, Ti$_6$N$_5$ at atmospheric pressure, and…

Materials Science · Physics 2014-11-07 Shuyin Yu , Qingfeng Zeng , Artem R. Oganov , Gilles Frapper , Litong Zhang

The immense interest in carbon nanomaterials continues to stimulate intense research activities aimed to realize carbon nanowires, since linear chains of carbon atoms are expected to display novel and technologically relevant optical,…

Materials Science · Physics 2010-11-02 Xing-Qiu Chen , C. L. Fu , C. Franchini

The 4d-transition-metals carbides (ZrC, NbC) and nitrides (ZrN, NbN) in the rocksalt structure, as well as their ternary alloys, have been recently studied by means of a first-principles full potential linearized augmented plane waves…

Materials Science · Physics 2017-04-26 Vassiliki Katsika-Tsigourakou

Layered Li(Ni,Mn,Co,)O$_2$ (NMC) presents an intriguing ternary alloy design space for optimization as a cathode material in Li-ion batteries. Recently, the high cost and resource limitations of Co have added a new design constraint and…

Materials Science · Physics 2020-02-17 Gregory Houchins , Venkatasubramanian Viswanathan

Rhombohedral dense forms of carbon, rh-C2 (or hexagonal h-C6), and boron nitride, rh-BN (or hexagonal h-B3N3), are derived from rhombohedral 3R graphite based on original crystal chemistry scheme backed with full cell geometry optimization…

Materials Science · Physics 2021-09-29 Samir F. Matar , Vladimir L. Solozhenko

Molybdenum borides were studied theoretically using first-principles calculations, empirical total energy model and global optimization techniques to determine stable crystal structures. Our calculations reveal the structures of known Mo-B…

Materials Science · Physics 2020-03-10 Dmitry V. Rybkovskiy , Alexander G. Kvashnin , Yulia A. Kvashnina , Artem R. Oganov

Polynitrogen compounds have attracted great interest due to their potential applications as high energy density materials. Most recently, a rich variety of alkali polynitrogens (R_{x}N_{y}; R=Li, Na, and Cs) have been predicted to be stable…

Materials Science · Physics 2018-02-07 Brad A. Steele , Ivan I. Oleynik

It is well known that pressure causes profound changes in the properties of atoms and chemical bonding, leading to the formation of many unusual materials. Here we systematically explore all stable calcium carbides at pressures from ambient…

Materials Science · Physics 2015-05-14 Yan-Ling Li , Sheng-Nan Wang , Artem R. Oganov , Huiyang Gou , Jesse S. Smith , Timothy A. Strobel

Carbon is likely the most fascinating element of the periodic table because of the diversity of its allotropes stemming from its variable (sp, sp2, and sp3) bonding motifs. Exploration of new forms of carbon has been an eternal theme of…

We have investigated by means of high-pressure x-ray diffraction the structural stability of Pd2Mo3N, Ni2Mo3C0.52N0.48, Co3Mo3C0.62N0.38, and Fe3Mo3C. We have found that they remain stable in their ambient-pressure cubic phase at least up…

Materials Science · Physics 2012-04-20 D. Errandonea , J. Ruiz-Fuertes , J. A. Sans , D. Santamaria-Perez , O. Gomis , A. Gomez , F. Sapina